Gold doping of tin clusters: exo- vs. endohedral complexes.

We present molecular beam electric deflection experiments on neutral gold-doped tin clusters. The experimental SnAu (N = 6-16) cluster beam profiles are interpreted by means of classical trajectory simulations supplied, with cluster structures generated by a genetic algorithm based on density functional theory. The combined experimental and theoretical analysis confirms that at least nine tin atoms are necessary to form a cage that is capable of encapsulating a gold atom, with high symmetry only marginally distorted by the gold atom.

Cavity Cooling of a Levitated Nanosphere by Coherent Scattering.

We report three-dimensional (3D) cooling of a levitated nanoparticle inside an optical cavity. The cooling mechanism is provided by cavity-enhanced coherent scattering off an optical tweezer. The observed 3D dynamics and cooling rates are as theoretically expected from the presence of both linear and quadratic terms in the interaction between the particle motion and the cavity field.

Measurement of quantum back action in the audio band at room temperature.

Quantum mechanics places a fundamental limit on the precision of continuous measurements. The Heisenberg uncertainty principle dictates that as the precision of a measurement of an observable (for example, position) increases, back action creates increased uncertainty in the conjugate variable (for example, momentum). In interferometric gravitational-wave detectors, higher laser powers reduce the position uncertainty created by shot noise (the photon-counting error caused by the quantum nature of the laser) but necessarily do so at the expense of back action in the form of quantum radiation pressure noise (QRPN).

Photoelectrical imaging and coherent spin-state readout of single nitrogen-vacancy centers in diamond.

Nitrogen-vacancy (NV) centers in diamond have become an important instrument for quantum sensing and quantum information science. However, the readout of NV spin state requires bulky optical setups, limiting fabrication of miniaturized compact devices for practical use. Here we realized photoelectrical detection of magnetic resonance as well as Rabi oscillations on a single-defect level.

On the origin of second harmonic generation in silicon waveguides with silicon nitride cladding.

Strained silicon waveguides have been proposed to break the silicon centrosymmetry, which inhibits second-order nonlinearities. Even if electro-optic effect and second harmonic generation (SHG) were measured, the published results presented plenty of ambiguities due to the concurrence of different effects affecting the process. In this work, the origin of SHG in a silicon waveguide strained by a silicon nitride cladding is investigated in detail.

Quantum mechanics and the covariance of physical laws in quantum reference frames.

In physics, every observation is made with respect to a frame of reference. Although reference frames are usually not considered as degrees of freedom, in all practical situations it is a physical system which constitutes a reference frame. Can a quantum system be considered as a reference frame and, if so, which description would it give of the world? Here, we introduce a general method to quantise reference frame transformations, which generalises the usual reference frame transformation to a "superposition of coordinate transformations".

Four Wave Mixing control in a photonic molecule made by silicon microring resonators.

Four Wave Mixing (FWM) is the main nonlinear interaction in integrated silicon devices, which finds diffuse use in all-optical signal processing and wavelength conversion. Despite the numerous works on coupled resonator devices, which showed record conversion efficiencies and broadband operation, the possibility to coherently control the strength of the stimulated FWM interaction on a chip has received very limited attention. Here, we demonstrate both theoretically and experimentally, the manipulation of FWM in a photonic molecule based on two side coupled silicon microring resonators.

Optomechanical Bell Test.

Over the past few decades, experimental tests of Bell-type inequalities have been at the forefront of understanding quantum mechanics and its implications. These strong bounds on specific measurements on a physical system originate from some of the most fundamental concepts of classical physics-in particular that properties of an object are well-defined independent of measurements (realism) and only affected by local interactions (locality). The violation of these bounds unambiguously shows that the measured system does not behave classically, void of any assumption on the validity of quantum theory.

Polarization Entanglement by Time-Reversed Hong-Ou-Mandel Interference.

Sources of entanglement are an enabling resource in quantum technology, and pushing the limits of generation rate and quality of entanglement is a necessary prerequisite towards practical applications. Here, we present an ultrabright source of polarization-entangled photon pairs based on time-reversed Hong-Ou-Mandel interference. By superimposing four pair-creation possibilities on a polarization beam splitter, pairs of identical photons are separated into two spatial modes without the usual requirement for wavelength distinguishability or noncollinear emission angles.

Experimental Determination of Irreversible Entropy Production in out-of-Equilibrium Mesoscopic Quantum Systems.

By making use of a recently proposed framework for the inference of thermodynamic irreversibility in bosonic quantum systems, we experimentally measure and characterize the entropy production rates in the nonequilibrium steady state of two different physical systems-a micromechanical resonator and a Bose-Einstein condensate-each coupled to a high finesse cavity and hence also subject to optical loss. Key features of our setups, such as the cooling of the mechanical resonator and signatures of a structural quantum phase transition in the condensate, are reflected in the entropy production rates. Our work demonstrates the possibility to explore irreversibility in driven mesoscopic quantum systems and paves the way to a systematic experimental assessment of entropy production beyond the microscopic limit.

Integrated Optomechanical Arrays of Two High Reflectivity SiN Membranes.

Multielement cavity optomechanics constitutes a direction to observe novel effects with mechanical resonators. Several exciting ideas include superradiance, increased optomechanical coupling, and quantum effects between distinct mechanical modes among others. Realizing these experiments has so far been difficult, because of the need for extremely precise positioning of the elements relative to one another due to the high-reflectivity required for each element.

A No-Go Theorem for Observer-Independent Facts.

In his famous thought experiment, Wigner assigns an entangled state to the composite quantum system made up of Wigner's friend and her observed system. While the two of them have different accounts of the process, each Wigner and his friend can in principle verify his/her respective state assignments by performing an appropriate measurement. As manifested through a click in a detector or a specific position of the pointer, the outcomes of these measurements can be regarded as reflecting directly observable "facts".

Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators.

We present quantum yield measurements of single layer WSe (1L-WSe) integrated with high-Q ( Q > 10) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission is achieved by placing 1L-WSe in the evanescent cavity field. This preserves the microresonator high intrinsic quality factor ( Q > 10) below the bandgap of 1L-WSe.

Comparative study of afterpulsing behavior and models in single photon counting avalanche photo diode detectors.

Single-photon avalanche diode (SPAD) detectors, have a great importance in fields like quantum key distribution, laser ranging, florescence microscopy, etc. Afterpulsing is a non-ideal behavior of SPADs that adversely affects any application that measures the number or timing of detection events. Several studies based on a few individual detectors, derived distinct mathematical models from semiconductor physics perspectives.

Two-Way Communication with a Single Quantum Particle.

In this Letter we show that communication when restricted to a single information carrier (i.e., single particle) and finite speed of propagation is fundamentally limited for classical systems.

Proposal for a Quantum Test of the Weak Equivalence Principle with Entangled Atomic Species.

We propose an experiment to test the weak equivalence principle (WEP) with a test mass consisting of two entangled atoms of different species. In the proposed experiment, a coherent measurement of the differential gravity acceleration between the two atomic species is considered, by entangling two atom interferometers operating on the two species. The entanglement between the two atoms is heralded at the initial beam splitter of the interferometers through the detection of a single photon emitted by either of the atoms, together with the impossibility of distinguishing which atom emitted the photon.

High-Dimensional Single-Photon Quantum Gates: Concepts and Experiments.

Transformations on quantum states form a basic building block of every quantum information system. From photonic polarization to two-level atoms, complete sets of quantum gates for a variety of qubit systems are well known. For multilevel quantum systems beyond qubits, the situation is more challenging.

Distribution of high-dimensional entanglement via an intra-city free-space link.

Quantum entanglement is a fundamental resource in quantum information processing and its distribution between distant parties is a key challenge in quantum communications. Increasing the dimensionality of entanglement has been shown to improve robustness and channel capacities in secure quantum communications. Here we report on the distribution of genuine high-dimensional entanglement via a 1.

Experimental test of photonic entanglement in accelerated reference frames.

The unification of the theory of relativity and quantum mechanics is a long-standing challenge in contemporary physics. Experimental techniques in quantum optics have only recently reached the maturity required for the investigation of quantum systems under the influence of non-inertial motion, such as being held at rest in gravitational fields, or subjected to uniform accelerations. Here, we report on experiments in which a genuine quantum state of an entangled photon pair is exposed to a series of different accelerations.

Orbital angular momentum of photons and the entanglement of Laguerre-Gaussian modes.

The identification of orbital angular momentum (OAM) as a fundamental property of a beam of light nearly 25 years ago has led to an extensive body of research around this topic. The possibility that single photons can carry OAM has made this degree of freedom an ideal candidate for the investigation of complex quantum phenomena and their applications. Research in this direction has ranged from experiments on complex forms of quantum entanglement to the interaction between light and quantum states of matter.

Stable Optical Trap from a Single Optical Field Utilizing Birefringence.

We report a stable double optical spring effect in an optical cavity pumped with a single optical field that arises as a result of birefringence. One end of the cavity is formed by a multilayer Al_{0.92}Ga_{0.

Automated Search for new Quantum Experiments.

Quantum mechanics predicts a number of, at first sight, counterintuitive phenomena. It therefore remains a question whether our intuition is the best way to find new experiments. Here, we report the development of the computer algorithm Melvin which is able to find new experimental implementations for the creation and manipulation of complex quantum states.

Proposal to Test Bell's Inequality in Electromechanics.

Optomechanical and electromechanical systems offer an effective platform to test quantum theory and its predictions at macroscopic scales. To date, all experiments presuppose the validity of quantum mechanics, but could in principle be described by a hypothetical local statistical theory. Here we suggest a Bell test using the electromechanical Einstein-Podolski-Rosen entangled state recently generated by Palomaki et al.

Non-classical correlations between single photons and phonons from a mechanical oscillator.

Interfacing a single photon with another quantum system is a key capability in modern quantum information science. It allows quantum states of matter, such as spin states of atoms, atomic ensembles or solids, to be prepared and manipulated by photon counting and, in particular, to be distributed over long distances. Such light-matter interfaces have become crucial to fundamental tests of quantum physics and realizations of quantum networks.