289 results match your criteria: "Scottish Universities Physics Alliance[Affiliation]"

Dipole toroidal modes appear in many fields of physics. In nuclei, such a mode was predicted more than 50 years ago, but clear experimental evidence was lacking so far. Using a combination of high-resolution inelastic scattering experiments with photons, electrons, and protons, we identify for the first time candidates for toroidal dipole excitations in the nucleus ^{58}Ni and demonstrate that transverse electron scattering form factors represent a relevant experimental observable to prove their nature.

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Intercellular friction and motility drive orientational order in cell monolayers.

Proc Natl Acad Sci U S A

October 2024

Scottish Universities Physics Alliance, School of Physics and Astronomy, University of Edinburgh, Edinburgh EH9 3FD, United Kingdom.

Spatiotemporal patterns in multicellular systems are important to understanding tissue dynamics, for instance, during embryonic development and disease. Here, we use a multiphase field model to study numerically the behavior of a near-confluent monolayer of deformable cells with intercellular friction. Varying friction and cell motility drives a solid-liquid transition, and near the transition boundary, we find the emergence of local nematic order of cell deformation driven by shear-aligning cellular flows.

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Radio-frequency particle accelerators are engines of discovery, powering high-energy physics and photon science, but are also large and expensive due to their limited accelerating fields. Plasma-wakefield accelerators (PWFAs) provide orders-of-magnitude stronger fields in the charge-density wave behind a particle bunch travelling in a plasma, promising particle accelerators of greatly reduced size and cost. However, PWFAs can easily degrade the beam quality of the bunches they accelerate.

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We report on a new technique for measuring the dynamic Young's modulus, E, of quantum materials at low temperatures as a function of static tuning strain, ϵ, in piezoactuator-driven pressure cells. In addition to a static tuning of stress and strain, we apply a small-amplitude, finite-frequency AC (1 Hz ≲ ω ≲ 1000 Hz) uniaxial stress, σac, to the sample and measure the resulting AC strain, ϵac, using a capacitive sensor to obtain the associated modulus E. We demonstrate the performance of the new technique through proof-of-principle experiments on the unconventional superconductor Sr2RuO4, which is known for its rich temperature-strain phase diagram.

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Piezoelectric Charge Coefficient of Halide Perovskites.

Materials (Basel)

June 2024

Energy Harvesting Research Group, School of Physics & Astronomy, Scottish Universities Physics Alliance (SUPA), University of St Andrews, North Haugh, St Andrews KY16 9SS, UK.

Halide perovskites are an emerging family of piezoelectric and ferroelectric materials. These materials can exist in bulk, single-crystal, and thin-film forms. In this article, we review the piezoelectric charge coefficient (d) of single crystals, thin films, and dimension-tuned halide perovskites based on different measurement methods.

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Predicted hot superconductivity in LaScH under pressure.

Proc Natl Acad Sci U S A

June 2024

Key Laboratory of Material Simulation Methods and Software of Ministry of Education, College of Physics, Jilin University, Changchun 130012, China.

The recent theory-driven discovery of a class of clathrate hydrides (e.g., CaH, YH, YH, and LaH) with superconducting critical temperatures () well above 200 K has opened the prospects for "hot" superconductivity above room temperature under pressure.

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π-π stacking are omnipresent interactions, crucial in many areas of chemistry, and often studied using quantum chemical methods. Here, we report a simple and computationally efficient method of estimating the binding energies of stacked polycyclic aromatic hydrocarbons based on steered molecular dynamics. This method leverages the force field parameters for accurate calculation.

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Embryo quality is an important determinant of successful implantation and a resultant live birth. Current clinical approaches for evaluating embryo quality rely on subjective morphology assessments or an invasive biopsy for genetic testing. However, both approaches can be inherently inaccurate and crucially, fail to improve the live birth rate following the transfer of in vitro produced embryos.

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Phase-Transition-Promoted Thermoelectric Textiles Based on Twin Surface-Modified CNT Fibers.

ACS Appl Mater Interfaces

April 2024

Department of Light Chemical Engineering, Jiangnan University, Wuxi 214122, PR China.

With the fast development of new science and technology, wearable devices are in great demand in modern human daily life. However, the energy problem is a long-lasting issue to achieve real smart, wearable, and portable devices. Flexible thermoelectric generators (TEGs) based on thermoelectric conversion systems can convert body waste heat into electricity with excellent flexibility and wearability, which shows a new direction to solving this issue.

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Impact of the Crystal Structure of Silica Nanoparticles on Rhodamine 6G Adsorption: A Molecular Dynamics Study.

ACS Omega

January 2024

Photophysics Group, Department of Physics, University of Strathclyde, Scottish Universities Physics Alliance, 107 Rottenrow, Glasgow G4 0NG, U.K.

Understanding the mechanism of adsorption of Rhodamine 6G (R6G) to various crystal structures of silica nanoparticles (SNPs) is important to elucidate the impact of dye size when measuring the size of the dye-SNP complex via the time-resolved fluorescence anisotropy method. In this work, molecular dynamics (MD) simulations were used to get an insight into the R6G adsorption process, which cannot be observed using experimental methods. It was found that at low pH, α-Cristobalite structured SNPs have a strong affinity to R6G; however, at high pH, more surface silanol groups undergo ionization when compared with α-Quartz, preventing the adsorption.

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Fate of Quasiparticles at High Temperature in the Correlated Metal Sr_{2}RuO_{4}.

Phys Rev Lett

December 2023

Department of Quantum Matter Physics, University of Geneva, 24 Quai Ernest-Ansermet, 1211 Geneva 4, Switzerland.

We study the temperature evolution of quasiparticles in the correlated metal Sr_{2}RuO_{4}. Our angle resolved photoemission data show that quasiparticles persist up to temperatures above 200 K, far beyond the Fermi liquid regime. Extracting the quasiparticle self-energy, we demonstrate that the quasiparticle residue Z increases with increasing temperature.

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We have investigated the low-temperature local magnetic properties in the bulk of molten salt-flux (MSF)-grown single crystals of the candidate odd-parity superconductor UTe_{2} by zero-field muon spin relaxation (μSR). In contrast to previous μSR studies of UTe_{2} single crystals grown by a chemical vapor transport method, we find no evidence of magnetic clusters or electronic moments fluctuating slow enough to cause a discernible relaxation of the zero-field μSR asymmetry spectrum. Consequently, our measurements on MSF-grown single crystals rule out the generation of spontaneous magnetic fields in the bulk that would occur near impurities or lattice defects if the superconducting state of UTe_{2} breaks time-reversal symmetry.

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Progress in magnetoelectric materials is hindered by apparently contradictory requirements for time-reversal symmetry broken and polar ferroelectric electronic structure in common ferromagnets and antiferromagnets. Alternative routes can be provided by recent discoveries of a time-reversal symmetry breaking anomalous Hall effect (AHE) in noncollinear magnets and altermagnets, but hitherto reported bulk materials are not polar. Here, the authors report the observation of a spontaneous AHE in doped AgCrSe , a layered polar semiconductor with an antiferromagnetic coupling between Cr spins in adjacent layers.

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The interplay of electronic and structural degrees of freedom in solids is a topic of intense research. More than 60 years ago, Lifshitz discussed a counterintuitive possibility: lattice softening driven by conduction electrons at topological Fermi surface transitions. The effect that he predicted, however, was small and has not been convincingly observed.

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The layered delafossite metal PdCrO[Formula: see text] is a natural heterostructure of highly conductive Pd layers Kondo coupled to localized spins in the adjacent Mott insulating CrO[Formula: see text] layers. At high temperatures, , it has a -linear resistivity which is not seen in the isostructural but nonmagnetic PdCoO[Formula: see text]. The strength of the Kondo coupling is known, as-grown crystals are extremely high purity and the Fermi surface is both very simple and experimentally known.

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Compass-like manipulation of electronic nematicity in SrRuO.

Proc Natl Acad Sci U S A

September 2023

Scottish Universities Physics Alliance, School of Physics and Astronomy, University of St Andrews, North Haugh, St Andrews, KY16 9SS, United Kingdom.

Electronic nematicity has been found in a wide range of strongly correlated electron materials, resulting in the electronic states having-4.5pc]Please note that the spelling of the following author name(s) in the manuscript differs from the spelling provided in the article metadata: Izidor Benedičič. The spelling provided in the manuscript has been retained; please confirm.

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The largest Fermi surface sheet of the correlated metal Sr_{2}RuO_{4} can be driven through a Lifshitz transition between an electronlike and an open geometry by uniaxial stress applied along the [100] lattice direction. Here, we investigate the effect of this transition on the longitudinal resistivity ρ_{xx} and the Hall coefficient R_{H}. ρ_{xx}(T), when Sr_{2}RuO_{4} is tuned to this transition, is found to have a T^{2}logT form, as expected for a Fermi liquid tuned to a Lifshitz transition.

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We report the preparation and spectroscopic characterization of a highly elusive copper site bound exclusively to oxygen donor atoms within a protein scaffold. Despite copper generally being considered unsuitable for use in MRI contrast agents, which in the clinic are largely Gd(III) based, the designed copper coiled coil displays relaxivity values equal to, or superior than, those of the Gd(III) analog at clinical field strengths. The creation of this new-to-biology proteinaceous CuO-binding site demonstrates the power of the de novo peptide design approach to access chemistry for abiological applications, such as for the development of MRI contrast agents.

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Machine learning (ML) is an effective tool to interrogate complex systems to find optimal parameters more efficiently than through manual methods. This efficiency is particularly important for systems with complex dynamics between multiple parameters and a subsequent high number of parameter configurations, where an exhaustive optimisation search would be impractical. Here we present a number of automated machine learning strategies utilised for optimisation of a single-beam caesium (Cs) spin exchange relaxation free (SERF) optically pumped magnetometer (OPM).

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The crucial role of adhesion in the transmigration of active droplets through interstitial orifices.

Nat Commun

February 2023

Istituto per le Applicazioni del Calcolo CNR, via dei Taurini 19, 00185, Rome, Italy.

Active fluid droplets are a class of soft materials exhibiting autonomous motion sustained by an energy supply. Such systems have been shown to capture motility regimes typical of biological cells and are ideal candidates as building-block for the fabrication of soft biomimetic materials of interest in pharmacology, tissue engineering and lab on chip devices. While their behavior is well established in unconstrained environments, much less is known about their dynamics under strong confinement.

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Attosecond-Angstrom free-electron-laser towards the cold beam limit.

Nat Commun

February 2023

Department of Physics, Scottish Universities Physics Alliance, University of Strathclyde, Glasgow, UK.

Electron beam quality is paramount for X-ray pulse production in free-electron-lasers (FELs). State-of-the-art linear accelerators (linacs) can deliver multi-GeV electron beams with sufficient quality for hard X-ray-FELs, albeit requiring km-scale setups, whereas plasma-based accelerators can produce multi-GeV electron beams on metre-scale distances, and begin to reach beam qualities sufficient for EUV FELs. Here we show, that electron beams from plasma photocathodes many orders of magnitude brighter than state-of-the-art can be generated in plasma wakefield accelerators (PWFAs), and then extracted, captured, transported and injected into undulators without significant quality loss.

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Core-Shell Nanorods as Ultraviolet Light-Emitting Diodes.

Nano Lett

February 2023

Department of Physics, Scottish Universities Physics Alliance (SUPA), University of Strathclyde, Glasgow G4 0NG, United Kingdom.

Existing barriers to efficient deep ultraviolet (UV) light-emitting diodes (LEDs) may be reduced or overcome by moving away from conventional planar growth and toward three-dimensional nanostructuring. Nanorods have the potential for enhanced doping, reduced dislocation densities, improved light extraction efficiency, and quantum wells free from the quantum-confined Stark effect. Here, we demonstrate a hybrid top-down/bottom-up approach to creating highly uniform AlGaN core-shell nanorods on sapphire repeatable on wafer scales.

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Stabilization of SO at high pressure: implications for the sulfur-excess paradox.

Sci Bull (Beijing)

May 2022

State Key Laboratory of Superhard Materials & International Center of Computational Method and Software, College of Physics, Jilin University, Changchun 130012, China. Electronic address:

The amount of sulfur in SO discharged in volcanic eruptions exceeds that available for degassing from the erupted magma. This geological conundrum, known as the "sulfur excess", has been the subject of considerable interests but remains an open question. Here, in a systematic computational investigation of sulfur-oxygen compounds under pressure, a hitherto unknown SO compound containing a mixture of sulfur oxidation states +II and +IV is predicted to be stable at pressures above 79 GPa.

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Gold nanorods (GNRs) have emerged as the most efficient photothermal agent in cancer therapy and photocatalysis. Understanding the influence of the surrounding medium, particle size, and excitation wavelength is critical to optimising the photothermal conversion rate. Here, three pairs of large and small gold nanorods of different aspect ratios and their heat generation under laser radiation at on and off surface plasmon resonance wavelengths in aqueous solution and gel-like media are investigated.

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Keratin intrinsic fluorescence as a mechanism for non-invasive monitoring of its glycation.

Methods Appl Fluoresc

December 2022

Photophysics Group, Department of Physics, University of Strathclyde, Scottish Universities Physics Alliance, Glasgow G4 0NG, United Kingdom.

We have studied the evolution of keratin intrinsic fluorescence as an indicator of its glycation. Steady-state and time-resolved fluorescence of free keratin and keratin-glucose samples were detected in PBS solutions. The changes in the fluorescence response demonstrate that the effect of glucose is manifest in the accelerated formation of fluorescent cross-links with an emission peak at 460 nm and formation of new cross-links with emission peaks at 525 nm and 575 nm.

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