Quantum control of molecular orientation by two-color laser fields.

We demonstrate molecular orientation by using phase-controlled two-color omega+2omega laser pulses with an intensity of 1.0x10(12) W/cm(2) and a pulse duration of 130 fs. The orientation of three iodine-containing molecules (IBr, CH(3)I, and C(3)H(5)I) was monitored by the directional asymmetries of the photofragment angular distribution in dissociative ionization.

Coherent control of photofragment separation in the dissociative ionization of IBr.

We have investigated coherent control of the dissociative ionization of IBr using phase-controlled two-color omega+2omega laser pulses with an intensity of 1.0 x 10(12) W/cm and a pulse duration of 130 fs. The directional asymmetries of the photofragment angular distributions showed oscillation behavior dependent on the relative phase difference between the omega and 2omega pulses.