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Flexible lithium-ion batteries have attracted considerable interest for next-generation bendable, implantable and wearable electronics devices. Here, we have successfully grown CrO nanosheets on carbon cloth (CC) as freestanding anodes for Li-ion batteries (LIBs). Density functional theory (DFT) calculations verify an optimal structure of two-dimensional CrO nanosheets on the carbon fiber surface and a strong interaction between the O edges of CrO and the carbon.

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