2 results match your criteria: "Japan and The Graduate University for Advanced Studies (SOKENDAI)[Affiliation]"
Erratum: "Unraveling the dynamic slowdown in supercooled water: The role of dynamic disorder in jump motions" [J. Chem. Phys. 160, 194506 (2024)].
J Chem Phys
July 2024
Institute for Molecular Science, Myodaiji, Okazaki, Aichi 444-8585, Japan and The Graduate University for Advanced Studies (SOKENDAI), Myodaiji, Okazaki, Aichi , 444-8585, Japan.
Unraveling the dynamic slowdown in supercooled water: The role of dynamic disorder in jump motions.
J Chem Phys
May 2024
Institute for Molecular Science, Myodaiji, Okazaki, Aichi 444-8585, Japan and The Graduate University for Advanced Studies (SOKENDAI), Myodaiji, Okazaki, Aichi 444-8585, Japan.
Article Synopsis
- Rapid cooling of water below its melting point leads to a significant slowdown in its dynamics without obvious structural changes, posing a challenge to understand this phenomenon.
- Molecular dynamics simulations reveal that the jump dynamics of water molecules behave differently than expected at lower temperatures, influenced by slow variables that disrupt regular motion, described as dynamic disorder.
- As temperature decreases, jumping molecules become trapped in stable low-density regions, increasing the number of slow variables involved and resulting in even slower and more intermittent dynamics, which may eventually lead to a glass transition.