Shape characterization of a large nonspherical particle by use of its Fraunhofer diffraction pattern.

We characterize the shape of a large nonspherical particle by means of the two-dimensional Fourier transformation of its diffraction pattern, called the S function. The main properties of S functions are considered. Some ways in which to retrieve the geometric parameters of a particle by use of its S function are discussed.

Retrieval of cloud optical parameters from space-based backscatter lidar data.

We present an approach to estimating the multiple-scattering (MS) contribution to lidar return signals from clouds recorded from space that enables us to describe in more detail the return formation at the depth where first orders of scattering dominate. Estimates made have enabled us to propose a method for correcting solutions of single-scattering lidar equations for the MS contribution. We also describe an algorithm for reconstructing the profiles of the cloud scattering coefficient and the optical thickness tau under conditions of a priori uncertainties.

Cross-wind profiling based on the scattered wave scintillation in a telescope focus.

The problem of wind profile reconstruction from scintillation of an optical wave scattered off a rough surface in a telescope focus plane is considered. Both the expression for the spatiotemporal correlation function and the algorithm of cross-wind velocity and direction profiles reconstruction based on the spatiotemporal spectrum of intensity of an optical wave scattered by a diffuse target in a turbulent atmosphere are presented. Computer simulations performed under conditions of weak optical turbulence show wind profiles reconstruction by the developed algorithm.

Wind profiling based on the optical beam intensity statistics in a turbulent atmosphere.

Reconstruction of the wind profile from the statistics of intensity fluctuations of an optical beam propagating in a turbulent atmosphere is considered. The equations for the spatiotemporal correlation function and the spectrum of weak intensity fluctuations of a Gaussian beam are obtained. The algorithms of wind profile retrieval from the spatiotemporal intensity spectrum are described and the results of end-to-end computer experiments on wind profiling based on the developed algorithms are presented.

Wind velocity profile reconstruction from intensity fluctuations of a plane wave propagating in a turbulent atmosphere.

Reconstruction of a wind profile based on the statistics of plane-wave intensity fluctuations in a turbulent atmosphere is considered. The algorithm for wind profile retrieval from the spatiotemporal spectrum of plane-wave weak intensity fluctuations is described, and the results of end-to-end computer experiments on wind profiling based on the developed algorithm are presented. It is shown that the reconstructing algorithm allows retrieval of a wind profile from turbulent plane-wave intensity fluctuations with acceptable accuracy.

Pulsed light field of a point source in a scattering medium.

Pulsed radiation propagating through a layer of a scattering medium undergoes distortions caused by multiple scattering. The results of numerical calculations of pulse waveforms for media with different scattering phase functions are presented. It is demonstrated that the scattered radiation waveform is not described by diffusion theories even for sufficiently large optical thicknesses (tau approximately 10-20) but is described, as a rule, by a bimodal distribution.

Two-channel opto-acoustic diode laser spectrometer and fine structure of methane absorption spectra in 6070-6180 cm-1 region.

We describe the hardware and software of the high-sensitive two-channel opto-acoustic spectrometer with a near infrared diode laser. A semiconductor TEC-100 laser with outer resonator generates a continuous single-frequency radiation in the range of 6040-6300 cm-1 with spectral resolution better that 10 MHz. The newly designed model of photo-acoustic cells in the form of a ring type resonator was used in the spectrometer, and the system allows the measurement of a weak absorption coefficient equal to 1.

Spatial distribution of methane over Lake Baikal surface.

The results of application of a high sensitivity methane laser detector to investigations of the methane concentration in the atmosphere over Baikal lake are presented as well as methane flows from the water into the atmosphere. The measurements were conducted at a stationary station and aboard the research vessel "Vereschagin" during two summer expeditions in 2003 and 2004. Mean background concentration was equal to (2.

Statistical approach to light scattering by convex ice crystals.

Within the geometric optics approximation, the phase functions of randomly oriented ice crystals are calculated as a series relative to multiplicity of internal collisions of light inside the particles. In the case of convex crystals, it is shown that the coefficients of the series provide the most information about the crystal shapes, while the angular functions of this series are weakly dependent on the shapes. The prevailing role of the term corresponding to one internal collision is emphasized.

Two level metal vapor lasers with thermal creation of population inversion.

We present a new technique for direct conversion of thermal energy into coherent radiation. The near-surface layer of evaporated excited atoms of rare earth metals is proposed to be used as a converter. There is an inverted population in this layer.

Influence of the air-water interface on hydrosol lidar operation.

The results of seawater sensing by use of an airborne lidar with a changeable field of view (FOV) are presented, together with the results of numerical simulation of lidar operation by the Monte Carlo method. It is demonstrated that multiple scattering and wind-driven sea waves have opposite effects on the measured attenuation coefficient. At small FOVs the wind-driven sea waves cause the lidar signal decay rate to increase compared with the size of the plane surface and hence result in an overestimation of the retrieved attenuation coefficient.

Method for reconstructing atmospheric optical parameters from the data of polarization lidar sensing.

Inversion of polarization lidar sensing data based on the form of the lidar sensing equation with allowance for contributions from multiple-scattering calls for a priori information on the scattering phase matrix. In the present study the parameters of the Stokes vectors for various propagation media, including those with the scattering phase matrices that vary along the measuring range, are investigated. It is demonstrated that, in spaceborne lidar sensing, a simple parameterization of the multiple-scattering contribution is applicable and the polarization signal's characteristics depend mainly on the lidar and depolarization ratios, whereas differences in the angular dependences of the matrix components are no longer determining factors.

Polarization structure of lidar signals reflected from ice crystal clouds.

Polarization characteristics of signals of a monostatic lidar intended for sensing of homogeneous ice crystal clouds are calculated by the Monte Carlo method. Clouds are modeled as monodisperse ensembles of randomly oriented hexagonal ice crystals. The polarization state of multiply scattered lidar signal components is analyzed for different scattering orders depending on the crystal shapes and sizes as well as on the optical and geometrical conditions of observation.

Investigating particle orientation in cirrus clouds by measuring backscattering phase matrices with lidar.

The relation between the orientation of particles in ice-crystal clouds and backscattering phase matrices (BSPMs) is considered. Parameters characterizing the predominant orientation of particles in the azimuthal direction and in the horizontal position are presented. The parameters are expressed through BSPM elements.

Photo-acoustic measurements of gas and aerosol absorption with diode lasers.

The results of designing multipurpose high-sensitive photo-acoustic (PA) detectors and their application to high-resolution diode laser spectroscopy of molecular gases, gas analysis, and aerosol absorption measurements are summarized in this paper. The hardware and software of the diode laser spectrometer with a Helmholtz resonant PA detector providing an absorption sensitivity limit of better than 10(-7)Wm(-1)Hz(-1/2) are described. A procedure is proposed for an experiment involving the measurements of the rotational structure of hot vibrational bands of molecules.

Scattering matrices for large ice crystal particles.

The problem of light scattering by ice crystal particles whose sizes are essentially larger than the incident wavelength is divided into two parts. First, the scattered field is represented as a set of plane-parallel outgoing beams in the near zone of the particle. Then, in the far zone the scattered field is represented as a result of both diffraction and interference of these beams within the framework of physical optics.

On the extinction of radiation by a homogeneous but spatially correlated random medium: comment.

Some extinction laws for radiation transmitted through inhomogeneous random media were discussed by Kostinski [J. Opt. Soc.

Optimisation of photoacoustic resonant cells with commercial microphones for diode laser gas detection.

The theoretical and experimental study of the differential Helmholtz resonant (DHR) cell sensitivity under variation of the total gas pressure is made for various commercial microphones. Near-infrared lasers (room-temperature diode lasers) were used to measure the response of DHR cell versus pressure of the absorbing gas and frequency of the laser radiation modulation. Several molecular absorbers like H2O, CH4, mixed with molecular buffer gases were used to investigate the behavior of the photoacoustic (PA) signal characteristics with a DHR cell.

Phase-correction of turbulent distortions of an optical wave propagating under conditions of strong intensity fluctuations.

Phase correction of a plane wave and a spatiolimited beam propagating through a turbulent layer of atmosphere were considered. The required adaptive corrector element size and the system bandwidth were found by numerical simulation. These requirements were determined to be the same as for a weak-intensity scintillation approximation.

Optimal method of linear regression in laser remote sensing.

Remote lidar sensing in the photon-counting mode is now the commonly accepted method for studying atmospheric processes in the lower and free atmosphere. However, when processing signals obtained from lidar measurements, investigators necessarily face the problem of achieving accuracy in reconstructing the atmospheric parameters despite the presence of inhomogeneous noise in the measured signals. We propose an optimal method of linear regression (OMLR) of signals.

Expanding the dynamic range of a lidar receiver by the method of dynode-signal collection.

A method of lidar data collection by simultaneous registration of signals from the anode and several dynodes of the photomultiplier is suggested. The dynamic range of the receiver has been extended as many as 5 orders of magnitude in the case of cloud sensing. The stable operation under strong background illumination is possible without losses in fine signal structure.

Theory of singular-phase reconstruction for an optical speckle field in the turbulent atmosphere.

Analytical expressions are derived and computational algorithms are constructed for retrieving optical-field phase distribution under strong scintillation. The input data for the phase reconstruction are the wave-front slopes registered by a Hartmann sensor or shearing interferometer. The theory is based on representing the slope-vector field as the sum of its potential and solenoid components; it introduces the concept of phase-source and phase-vortex density and uses strict integral expressions relating these quantities to the wave-front slopes.

Fourth-Order Rotational Corrections to the Effective Dipole Moments of Nonrigid Asymmetric Rotors.

An expression for the fourth-order rotational correction terms of the effective dipole moments of nonrigid asymmetric rotors has been derived using the method of contact transformation. The treatment takes into account the large-amplitude bending motion. The correction terms have been calculated for the different bending states of the H(2)O molecule.

Dipole-Moment Derivatives of Nitrous Oxide.

The equations relating the q(2)J-type parameters of the matrix elements of the effective dipole-moment operator with the force field constants and the dipole-moment derivatives have been established by means of contact transformations in the case of nitrous oxide molecule. The effective dipole-moment operator corresponds to the reduced effective Hamiltonian derived by J.-L.

High-Order Resonances in the Water Molecule.

The water-vapor spectra in the near-infrared and visible region were reanalyzed with the purpose of finding experimental evidences of unusual high-order resonance between "dark" high-bending and "bright" stretch vibration states. About 70 transitions to the (050), (060), (070), (080), (160), (061), (170), (071), and, even (0 10 0) bending states, and their resonating partners were assigned in the spectra that gives the experimental energy levels lying near or above the potential energy barrier to linearity. The assignments were confirmed by combination differences and simultaneous observation of both perturbed and perturbing levels.