Polarization-Resolved Near-Infrared PdSe p-i-n Homojunction Photodetector.

Constructing high-quality homojunctions plays a pivotal role for the advancement of two-dimensional transition metal sulfide (TMDC) based optoelectronic devices. Here, a lateral PdSe p-i-n homojunction is constructed by electrostatic doping. Electrical measurements reveal that the homojunction diode exhibits a strong rectifying characteristic with a rectification ratio exceeding 10 and an ideality factor approaching 1.

Dynamic Homogenization of Internal Strain in Multi-Principal Element Alloy via High-Concentration Doping of Oxygen with Large Mobility.

Internal strain and its distribution within the crystal lattice play crucial roles in modulating dislocation activities, thereby affecting mechanical properties of materials. Through the synergistic application of integrated differential phase contrast, in situ transmission electron microscopy characterizations, and computational simulations, a method is unveiled for homogenizing dislocation pinning in NiCoCr multi-principal element alloy (MPEA) through the introduction of a high concentration of oxygen atoms with high diffusion mobility. The doping of massive oxygen atoms creates a high density of strong local pinning points for dislocation motion.

Prevailing Charge Order in Overdoped La_{2-x}Sr_{x}CuO_{4} beyond the Superconducting Dome.

The extremely overdoped cuprates are generally considered to be Fermi liquid metals without exotic orders, whereas the underdoped cuprates harbor intertwined states. Contrary to this conventional wisdom, using Cu L_{3}-edge and O K-edge resonant x-ray scattering, we reveal a charge order (CO) correlation in overdoped La_{2-x}Sr_{x}CuO_{4} (0.35≤x≤0.

Full electrical control of multiple resistance states in van der Waals sliding multiferroic tunnel junctions.

The recent development of two-dimensional magnetic and sliding-ferroelectric van der Waals (vdW) materials opens a new way to realize vdW sliding multiferroic tunnel junctions (MFTJs) for low-power nonvolatile memory applications. Here, we propose and investigate full electrical control of four nonvolatile resistance states in sliding MFTJs, Au/CrI/bilayer -BN/CrI-MnBiTe/Au, first principles. We found four stable states associated with different polarization orientations in bilayer -BN and magnetization alignment in two CrI magnetic layers, which can be controlled purely by electrical voltage and current, respectively.

Magnetically-dressed CrSBr exciton-polaritons in ultrastrong coupling regime.

Over the past few decades, exciton-polaritons have attracted substantial research interest due to their half-light-half-matter bosonic nature. Coupling exciton-polaritons with magnetic orders grants access to rich many-body phenomena, but has been limited by the availability of material systems that exhibit simultaneous exciton resonances and magnetic ordering. Here we report magnetically-dressed microcavity exciton-polaritons in the van der Waals antiferromagnetic (AFM) semiconductor CrSBr coupled to a Tamm plasmon microcavity.

Universal Quantum Optimization with Cold Atoms in an Optical Cavity.

Cold atoms in an optical cavity have been widely used for quantum simulations of many-body physics, where the quantum control capability has been advancing rapidly in recent years. Here, we show the atom cavity system is universal for quantum optimization with arbitrary connectivity. We consider a single-mode cavity and develop a Raman coupling scheme by which the engineered quantum Hamiltonian for atoms directly encodes number partition problems.

Full counting statistics, fluctuation relations, and linear response properties in a one-dimensional Kitaev chain.

We analytically calculate the cumulant generating function of energy and particle transport in an open one-dimensional Kitaev chain at finite temperature by utilizing the Keldysh technique. The joint distribution of particle and energy currents satisfies different fluctuation relations in different regions of the parameter space as a result of U(1) symmetry breaking and energy conservation. Furthermore, we investigate the linear response behavior of the Kitaev chain within the framework of three-terminal systems, deriving the expressions for the Seebeck coefficient and thermal conductance.

Harvesting Energy from Changes in Relative Humidity Using Nanoscale Water Capillary Bridges.

We show that nanoscale water capillary bridges (WCB) formed between patchy surfaces can extract energy from the environment when subjected to changes in relative humidity (RH). Our results are based on molecular dynamics simulations combined with a modified version of the Laplace-Kelvin equation, which is validated using the nanoscale WCB. The calculated energy density harvested by the nanoscale WCB is relevant, ≈1700 kJ/m, and is comparable to the energy densities harvested using available water-responsive materials that expand and contract due to changes in RH.

Synergistic correlated states and nontrivial topology in coupled graphene-insulator heterostructures.

Graphene has aroused great attention due to the intriguing properties associated with its low-energy Dirac Hamiltonian. When graphene is coupled with a correlated insulating substrate, electronic states that cannot be revealed in either individual layer may emerge in a synergistic manner. Here, we theoretically study the correlated and topological states in Coulomb-coupled and gate-tunable graphene-insulator heterostructures.

Unraveling the Ultrafast Coherent Dynamics of Exciton Polariton Propagation at Room Temperature.

Exciton polaritons are widely considered as promising platforms for developing room-temperature polaritonic devices, owing to the high-speed propagation and nonlinear interactions. However, it remains challenging to explore the dynamics of exciton polaritons specifically at room temperature, where the lifetime could be as small as a few picoseconds and the prevailing time-averaged measurement cannot give access to the true nature of it. Herein, by using the time-resolved photoluminescence, we have successfully traced the ultrafast coherent dynamics of a moving exciton polariton condensate in a one-dimensional perovskite microcavity.

Manipulating nonlinear exciton polaritons in an atomically-thin semiconductor with artificial potential landscapes.

Exciton polaritons in atomically thin transition-metal dichalcogenide microcavities provide a versatile platform for advancing optoelectronic devices and studying the interacting Bosonic physics at ambient conditions. Rationally engineering the favorable properties of polaritons is critically required for the rapidly growing research. Here, we demonstrate the manipulation of nonlinear polaritons with the lithographically defined potential landscapes in monolayer WS microcavities.

Buried-Metal-Grid Electrodes for Efficient Parallel-Connected Perovskite Solar Cells.

The limited conductivity of existing transparent conducting oxide (TCO) greatly restricts the further performance improvement of perovskite solar cells (PSCs), especially for large-area devices. Herein, buried-metal-grid tin-doped indium oxide (BMG ITO) electrodes are developed to minimize the power loss caused by the undesirable high sheet resistance of TCOs. By burying 140-nm-thick metal grids into ITO using a photolithography technique, the sheet resistance of ITO is reduced from 15.

Detecting Bell Correlations in Multipartite Non-Gaussian Spin States.

We expand the toolbox for studying Bell correlations in multipartite systems by introducing permutationally invariant Bell inequalities (PIBIs) involving few-body correlators. First, we present around twenty families of PIBIs with up to three- or four-body correlators, that are valid for an arbitrary number of particles. Compared to known inequalities, these show higher noise robustness, or the capability to detect Bell correlations in highly non-Gaussian spin states.

Strongly Localized Moiré Exciton in Twisted Homobilayers.

Artificially molding exciton flux is the cornerstone for developing promising excitonic devices. In the emerging hetero/homobilayers, the spatial separated charges prolong exciton lifetimes and create out-plane dipoles, facilitating electrically control exciton flux on a large scale, and the nanoscale periodic moiré potentials arising from twist-angle or/and lattice mismatch can substantially alter exciton dynamics, which are mainly proved in the heterostructures. However, the spatially indirect excitons dynamics in homobilayers without lattice mismatch remain elusive.

Spin Coherence and Spin Relaxation in Hybrid Organic-Inorganic Lead and Mixed Lead-Tin Perovskites.

Metal halide perovskites make up a promising class of materials for semiconductor spintronics. Here we report a systematic investigation of coherent spin precession, spin dephasing and spin relaxation of electrons and holes in two hybrid organic-inorganic perovskites MAFAPbI and MAFAPbSnI using time-resolved Faraday rotation spectroscopy. With applied in-plane magnetic fields, we observe robust Larmor spin precession of electrons and holes that persists for hundreds of picoseconds.

Intrinsic Nonlinear Hall Detection of the Néel Vector for Two-Dimensional Antiferromagnetic Spintronics.

The respective unique merit of antiferromagnets and two-dimensional (2D) materials in spintronic applications inspires us to exploit 2D antiferromagnetic spintronics. However, the detection of the Néel vector in 2D antiferromagnets remains a great challenge because the measured signals usually decrease significantly in the 2D limit. Here we propose that the Néel vector of 2D antiferromagnets can be efficiently detected by the intrinsic nonlinear Hall (INH) effect which exhibits unexpected significant signals.

Correlation of rattlers with thermal transport and thermoelectric performance.

The presence of rattlers in the host-guest structure has sparked great interest in the field of thermoelectrics, as it allows for the suppression of thermal transport in materials through vigorous anharmonic vibrations. This work predicts a ternary half-Heusler compound, LiAgTe, with good thermoelectric properties and high-temperature stability, which possesses a host-guest structure. Furthermore, it provides a detailed analysis of the role of rattlers in the transport process.

Proposal for Observing XUV-Induced Rabi Oscillation Using Superfluorescent Emission.

Intense x-ray and extreme ultraviolet (XUV) light sources have been available for decades, however, due to weak nonlinear interaction in the XUV photon energy range, observation of Rabi oscillation induced by XUV pulse remains a very challenging experimental task. Here we suggest a scheme where photoionization of a He medium by an intense XUV pump pulse is followed by a strong population inversion and Rabi oscillation at the He^{+}(1s-3p) transition and is accompanied by superfluorescence (SF) of the 7.56 eV pulse at the He^{+}(3p-2s) transition.

Revealing low-loss dielectric near-field modes of hexagonal boron nitride by photoemission electron microscopy.

Low-loss dielectric modes are important features and functional bases of fundamental optical components in on-chip optical devices. However, dielectric near-field modes are challenging to reveal with high spatiotemporal resolution and fast direct imaging. Herein, we present a method to address this issue by applying time-resolved photoemission electron microscopy to a low-dimensional wide-bandgap semiconductor, hexagonal boron nitride (hBN).

Approaching Ohmic Contacts for Ideal Monolayer MoS Transistors Through Sulfur-Vacancy Engineering.

Field-effect transistors (FETs) made of monolayer 2D semiconductors (e.g., MoS ) are among the basis of the future modern wafer chip industry.

First-principle calculation of the η→2γ decay width from lattice QCD.

We perform a lattice QCD calculation of the η→2γ decay width using a model-independent method that requires no momentum extrapolation of the off-shell form factors. This method also provides a straightforward and simple way to examine the finite-volume effects. The calculation is accomplished using N=2 twisted mass fermion ensembles.

Four-dimensional electron energy-loss spectroscopy.

Recent advances in scanning transmission electron microscopy have enabled atomic-scale focused, coherent, and monochromatic electron probes, achieving nanoscale spatial resolution, meV energy resolution, sufficient momentum resolution, and a wide energy detection range in electron energy-loss spectroscopy (EELS). A four-dimensional EELS (4D-EELS) dataset can be recorded with a slot aperture selecting the specific momentum direction in the diffraction plane and the beam scanning in two spatial dimensions. In this paper, the basic principle of the 4D-EELS technique and a few examples of its application are presented.

Deciphering Vacancy Defect Evolution of 2D MoS for Reliable Transistors.

Two-dimensional (2D) MoS is an excellent candidate channel material for next-generation integrated circuit (IC) transistors. However, the reliability of MoS is of great concern due to the serious threat of vacancy defects, such as sulfur vacancies (V). Evaluating the impact of vacancy defects on the service reliability of MoS transistors is crucial, but it has always been limited by the difficulty in systematically tracking and analyzing the changes and effects of vacancy defects in the service environment.