1,550 results match your criteria: "Collaborative Innovation Center of Quantum Matter[Affiliation]"

Synthesis and structure of a non-van-der-Waals two-dimensional coordination polymer with superconductivity.

Nat Commun

October 2024

National Key Laboratory of Advanced Micro and Nano Manufacture Technology, School of Materials Science and Engineering, Peking University, Beijing, 100871, China.

Article Synopsis
  • Two-dimensional conjugated coordination polymers, like copper-based benzenehexathiol (Cu-BHT), are notable for their exceptional charge transport characteristics, with Cu-BHT being a rare superconductor.
  • Researchers successfully synthesized high-quality single crystals of Cu-BHT, revealing a unique quasi-two-dimensional kagome structure characterized by strong Cu-S covalent bonds between layers.
  • The crystals demonstrated significant metallic conductivity at both high (10S/cm at 300 K) and low (10S/cm at 2 K) temperatures, and achieved superconductivity at 0.25 K, highlighting an important link between the crystal structure and electrical behavior that could influence the future of quantum technologies.
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Incoherence-to-coherence crossover observed in charge-density-wave material 1T-TiSe.

Nat Commun

October 2024

International Center for Quantum Materials, School of Physics, Peking University, 100871, Beijing, China.

Analogous to the condensation of Cooper pairs in superconductors, the Bose-Einstein condensation (BEC) of electron-hole pairs in semiconductors and semimetals leads to an emergence of an exotic ground state - the excitonic insulator state. In this paper, we study the electronic structure of 1T-TiSe utilizing angle-resolved photoemission spectroscopy and alkali-metal deposition. Alkali-metal adatoms are deposited in-situ on the sample surface, doping the system with electrons.

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Coherent optical spin Hall transport for polaritonics at room temperature.

Nat Mater

January 2025

State Key Laboratory of Low-Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, People's Republic of China.

Spin or valley degrees of freedom hold promise for next-generation spintronics. Nonetheless, the macroscopic coherent spin current formations are still hindered by rapid dephasing due to electron scattering, specifically at room temperature. Exciton polaritons offer excellent platforms for spin-optronic devices via the optical spin Hall effect.

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Molecular Pairing in Twisted Bilayer Graphene Superconductivity.

Phys Rev Lett

October 2024

International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, China.

We propose a theory for how the weak phonon-mediated interaction (J_{A}=1-4  meV) wins over the prohibitive Coulomb repulsion (U=30-60  meV) and leads to a superconductor in magic-angle twisted bilayer graphene (MATBG). We find the pairing mechanism akin to that in the A_{3}C_{60} family of molecular superconductors: Each AA stacking region of MATBG resembles a C_{60} molecule, in that optical phonons can dynamically lift the degeneracy of the moiré orbitals, in analogy to the dynamical Jahn-Teller effect. Such induced J_{A} has the form of an intervalley anti-Hund's coupling and is less suppressed than U by the Kondo screening near a Mott insulator.

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We present a lattice QCD calculation of the nucleon electric polarizabilities at the physical pion mass. Our findings reveal the substantial contributions of the Nπ states to these polarizabilities. Without considering these contributions, the lattice results fall significantly below the experimental values, consistent with previous lattice studies.

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Coherent growth of high-Miller-index facets enhances perovskite solar cells.

Nature

November 2024

State Key Laboratory for Artificial Microstructure and Mesoscopic Physics, School of Physics, Frontiers Science Center for Nano-optoelectronics and Collaborative Innovation Center of Quantum Matter, Peking University, Beijing, China.

Obtaining micron-thick perovskite films of high quality is key to realizing efficient and stable positive (p)-intrinsic (i)-negative (n) perovskite solar cells, but it remains a challenge. Here we report an effective method for producing high-quality, micron-thick formamidinium-based perovskite films by forming coherent grain boundaries, in which high-Miller-index-oriented grains grow on the low-Miller-index-oriented grains in a stabilized atmosphere. The resulting micron-thick perovskite films, with enhanced grain boundaries and grains, showed stable material properties and outstanding optoelectronic performances.

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Emergent Berezinskii-Kosterlitz-Thouless and Kugel-Khomskii Physics in the Triangular Lattice Bilayer Colbaltate.

Phys Rev Lett

September 2024

International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, China and Collaborative Innovation Center of Quantum Matter, 100871 Beijing, China.

Motivated by the experiments on the triangular lattice bilayer colbaltate K_{2}Co_{2}(SeO_{3})_{3}, we consider an extended XXZ model to explore the underlying physics. The model is composed of interacting Co^{2+} dimers on the triangular lattice, where the Co^{2+} ion provides an effective spin-1/2 local moment via the spin-orbit coupling and the crystal field effect. The intradimer interaction is dominant and would simply favor the local spin singlet, and the interdimer interactions compete with the interdimer interaction, leading to rich behaviors.

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Probing fragile topology with dislocations.

Sci Bull (Beijing)

December 2024

School of Physical Science and Technology, and Collaborative Innovation Center of Suzhou Nano Science and Technology, Soochow University, Suzhou 215006, China; Suzhou Institute for Advanced Research, University of Science and Technology of China, Suzhou 215123, China. Electronic address:

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Observation of Circular Dichroism Induced by Electronic Chirality.

Phys Rev Lett

September 2024

International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, China.

Chiral phases of matter, characterized by a definite handedness, abound in nature, ranging from the crystal structure of quartz to spiraling spin states in helical magnets. In 1T-TiSe_{2} a source of chirality has been proposed that stands apart from these classical examples as it arises from combined electronic charge and quantum orbital fluctuations. This may allow its chirality to be accessed and manipulated without imposing either structural or magnetic handedness.

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Eliminating performance loss from perovskite films to solar cells.

Sci Adv

September 2024

State Key Lab for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, Beijing 100871, China.

Article Synopsis
  • * The process of creating metal electrodes through high-vacuum thermal evaporation can damage the perovskite films, causing defects and reducing the effectiveness of the optimization.
  • * To address these issues, a dual-layer structure with graphene oxide and graphite flakes was developed, leading to PSCs with a power conversion efficiency of 25.55% and stable performance after 2000 hours of operation.
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High discrimination ratio, broadband circularly polarized light photodetector using dielectric achiral nanostructures.

Light Sci Appl

September 2024

State Key Laboratory for Mesoscopic Physics, Collaborative Innovation Center of Quantum Matter, Frontiers Science Center for Nano-Optoelectronics, School of Physics, Peking University, Beijing, China.

Article Synopsis
  • On-chip measurement of polarization states is essential for advanced sensing and imaging, but current circularly polarized light (CPL) photodetectors lack effective discrimination.
  • This study introduces a new broadband CPL photodetector using achiral all-dielectric nanostructures, achieving a high discrimination ratio of ~107 at 405 nm without needing intensity calibration.
  • The device works by exciting different near-field modes depending on the chirality of the light, leading to distinct photovoltage outputs, and offers a compact and versatile solution for high-performance CPL detection across various materials and wavelengths.
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Cascade Enhancement and Efficient Collection of Single Photon Emission under Topological Protection.

Nano Lett

October 2024

State Key Laboratory for Mesoscopic Physics, Department of Physics, Peking University, Beijing 100871, China.

High emission rate, high collection efficiency, and immunity to defects are the requirements of implementing on-chip single photon sources. Here, we theoretically demonstrate that both cascade enhancement and high collection efficiency of emitted photons from a single emitter can be achieved simultaneously in a topological photonic crystal containing a resonant dielectric nanodisk. The nanodisk excited by a magnetic emitter can be regarded as a large equivalent magnetic dipole.

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Bidirectional Peptide Translocation through Ultrasmall Solid-State Nanopores.

Langmuir

October 2024

State Key Lab for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics School of Physics, Peking University, Beijing 100871, China.

It is important to obtain the configuration of polypeptides and the sequence information on amino acids for understanding various life processes and many biological applications. Nanopores, as a newly developed single-molecule detection technology, exhibit unique advantages in real-time dynamics detection. Here, we designed a special peptide chain with 10 arginine in the head and achieved successful single-molecule detection by ultrasmall solid-state nanopores (2-3 nm).

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Exact work distribution and Jarzynski's equality of a relativistic particle in an expanding piston.

Phys Rev E

August 2024

School of Physics, Peking University, Beijing 100871, China; Collaborative Innovation Center of Quantum Matter, Beijing 100871, China and Frontiers Science Center for Nano-optoelectronics, Peking University, Beijing 100871, China.

We study the nonequilibrium work in a pedagogical model of relativistic ideal gas. We obtain the exact work distribution and verify Jarzynski's equality. In the nonrelativistic limit, our results recover the nonrelativistic results of Lua and Grosberg [J.

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Spin-Enhanced Self-Powered Light Helicity Detecting Based on Vertical WSe-CrI Heterojunction.

ACS Nano

September 2024

State Key Lab for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, Beijing 100871, China.

Two-dimensional (2D) magnetic semiconductors offer an intriguing platform for investigating magneto-optoelectronic properties and hold immense potential in developing prospective devices when they are combined with valley electronic materials like 2D transition-metal dichalcogenides. Herein, we report various magneto-optoelectronic response features of the vertical hBN-FLG-CrI-WSe-FLG-hBN van der Waals heterostructure. Through a sensible layout and exquisite manipulation, an hBN-FLG-CrI-FLG-hBN heterostructure was also fabricated on identical CrI and FLGs for better comparison.

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Suppressed Ion Migration by Heterojunction Layer for Stable Wide-Bandgap Perovskite and Tandem Photovoltaics.

Molecules

August 2024

State Key Laboratory for Artificial Microstructure and Mesoscopic Physics, School of Physics, Peking University, Beijing 100871, China.

Wide-bandgap (WBG) perovskite has demonstrated great potential in perovskite-based tandem solar cells. The power conversion efficiency (PCE) of such devices has surpassed 34%, signifying a new era for renewable energy development. However, the ion migration reduces the stability and hinders the commercialization, which is yet to be resolved despite many attempts.

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Monolayer SnS Schottky barrier field effect transistors: effects of electrodes.

Nanoscale

October 2024

State Key Laboratory of Mesoscopic Physics and Department of Physics, Peking University, Beijing 100871, P. R. China.

Achieving Ohmic contacts with low resistance is quite desirable for two-dimensional (2D) Schottky barrier field effect transistors (SBFETs). We verify the electrode effect on monolayer (ML) SnS SBFETs using calculations. With the aforeselected ML electrodes from matching lattices and work functions, we obtain n-type Ohmic contacts or quasi-Ohmic contacts to ML SnS with ML 1T-NbTe, ScNF, MoNF, NbCF, and graphene electrodes.

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Effect of ion-specific water structures at metal surfaces on hydrogen production.

Nat Commun

September 2024

International Center for Quantum Materials, School of Physics, Peking University, Beijing, P. R. China.

Article Synopsis
  • Water structures at electrolyte/electrode interfaces significantly influence electrochemical reaction selectivity and kinetics, yet detailed atomic-level information remains elusive.
  • Using advanced microscopy techniques, the study visualizes water layers with alkali metal cations on a charged Au(111) surface, showing Li cations are elevated and create an ice-like layer, while K and Cs cations are directly on the surface.
  • The research reveals various water network arrangements based on the cation type, which affects hydrogen evolution reaction kinetics, emphasizing the importance of spectator ions in electrochemical processes.
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Evolution from a charge-ordered insulator to a high-temperature superconductor in BiSr(Ca,Dy)CuO.

Nat Commun

September 2024

International Center for Quantum Materials, School of Physics, Peking University, Beijing, China.

How Cooper pairs form and condense has been the main challenge in the physics of copper-oxide high-temperature superconductors. Great efforts have been made in the 'underdoped' region of the phase diagram, through doping a Mott insulator or cooling a strange metal. However, there is still no consensus on how superconductivity emerges when electron-electron correlations dominate and the Fermi surface is missing.

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Electrical Contacts in Monolayer MoSiN Transistors.

ACS Appl Mater Interfaces

September 2024

State Key Laboratory for Mesoscopic Physics and Department of Physics, Peking University, Beijing 100871, P. R. China.

The latest synthesized monolayer (ML) MoSiN material exhibits stability in ambient conditions, suitable bandgap, and high mobilities. Its potential as a next-generation transistor channel material has been demonstrated through quantum transport simulations. However, in practical two-dimensional (2D) material transistors, the electrical contacts formed by the channel and the electrode must be optimized, as they are crucial for determining the efficiency of carrier injection.

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The Promise and Challenges of Inverted Perovskite Solar Cells.

Chem Rev

October 2024

State Key Laboratory for Artificial Microstructure and Mesoscopic Physics, School of Physics, Frontiers Science Center for Nano-optoelectronics & Collaborative Innovation Center of Quantum Matter, Peking University, Beijing 100871, China.

Article Synopsis
  • Inverted perovskite solar cells (PSCs) are being studied a lot because they are really stable, efficient, cheap, and can be made at low temperatures, which helps them work well in future solar tech.
  • The best single-junction PSCs have reached over 26% efficiency, while a combination of PSCs and silicon can reach nearly 34%, making them great for real-world use.
  • To make these solar cells even better, scientists are looking into different methods of improving their design and figuring out how to make them more environmentally friendly and cost-effective.
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Utilizing full-spectrum sunlight for ammonia decomposition to hydrogen over GaN nanowires-supported Ru nanoparticles on silicon.

Nat Commun

August 2024

Key Laboratory for Power Machinery and Engineering of Ministry of Education, Research Center for Renewable Synthetic Fuel, School of Mechanical Engineering, Shanghai Jiao Tong University, 800 Dongchuan Road, Shanghai, China.

Photo-thermal-coupling ammonia decomposition presents a promising strategy for utilizing the full-spectrum to address the H storage and transportation issues. Herein, we exhibit a photo-thermal-catalytic architecture by assembling gallium nitride nanowires-supported ruthenium nanoparticles on a silicon for extracting hydrogen from ammonia aqueous solution in a batch reactor with only sunlight input. The photoexcited charge carriers make a predomination contribution on H activity with the assistance of the photothermal effect.

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Solvent-Engineering-Assisted Ligand Exchange Strategy for High-Efficiency AgBiS Quantum Dot Solar Cells.

Angew Chem Int Ed Engl

December 2024

State Key Laboratory for Artificial Microstructure and Mesoscopic Physics, School of Physics, Frontiers Science Center for Nano-optoelectronics & Collaborative Innovation Center of Quantum Matter, Peking University, Beijing, 100871, China.

As the initial synthesized colloidal quantum dots (CQDs) are generally capped with insulating ligands, ligand exchange strategies are essential in the fabrication of CQD films for solar cells, which can regulate the surface chemical states of CQDs to make them more suitable for thin-film optoelectronic devices. However, uncontrollable surface adsorption of water molecules during the ligand exchange process introduces new defect sites, thereby impairing the resultant device performance, which attracts more efforts devoted to it but remains a puzzle. Here, we develop a solvent-engineering-assisted ligand exchange strategy to revamp the surface adsorption, improve the exchange efficiency, and modulate the surface chemistry for the environmentally friendly lead-free silver bismuth disulfide (AgBiS) CQDs.

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Article Synopsis
  • Researchers used varied experimental searches with and without missing transverse momentum to analyze a Two-Higgs-Doublet Model (2HDM) augmented by a pseudo-scalar that mediates interactions between ordinary and dark matter.
  • The analysis utilized data from proton-proton collisions at 13 TeV collected by the ATLAS detector at the Large Hadron Collider between 2015 and 2018, totaling up to 139 fb.
  • Three key searches were statistically combined, focusing on large missing transverse momentum along with decaying Z bosons, Higgs bosons decaying to bottom quarks, and charged Higgs bosons interacting with top and bottom quarks, to derive constraints for various benchmark scenarios in the 2HDM+a
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Strong light-matter coupling in van der Waals materials.

Light Sci Appl

August 2024

State Key Laboratory of Low-Dimensional Quantum Physics, Department of Physics, Tsinghua University, Beijing, 100084, China.

Article Synopsis
  • Two-dimensional (2D) van der Waals materials, particularly transition metal dichalcogenides (TMDs), are gaining popularity for their unique electronic and optical properties.
  • The review highlights advances in strong light-matter coupling with TMDs when integrated with optical structures like Fabry-Perot cavities and photonic crystals.
  • The paper also discusses potential applications of TMD polaritons and suggests future research directions in the study of light-matter interactions within van der Waals materials.
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