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Domino intramolecular Diels-Alder reactions to construct a 6/6/5/5 fused tetracyclic framework.
Chem Commun (Camb)
December 2015
State Key Laboratory of Applied Organic Chemistry, Department of Chemistry, Lanzhou University, Lanzhou, 730000, China. and Collaborative Innovation Center of Chemical Science and Engineering (Tianjin), Tianjin, 30071, China.
Domino intramolecular Diels-Alder (IMDA) reactions towards the 6/6/5/5 fused tetracyclic natural products were developed in satisfactory yield and high stereoselectivity. Four rings, six contiguous stereocenters and four C-C bonds were formed in a single operation. 4-epi-Hydromitchellene B was also synthesised efficiently via this strategy.
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