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Adsorption of selenium wires in silicalite-1 zeolite: a first order transition in a microporous system.
Phys Rev Lett
July 2002
Centre de Recherches sur les Mécanismes de la Croissance Cristalline CNRS, Campus de Luminy, Case 913, 13288, Marseille, Cedex 9, France.
A tight binding grand canonical Monte Carlo simulation of the adsorption of selenium in silicalite-1 zeolite is presented. The calculated adsorption-desorption isotherms exhibit characteristic features of a first order transition, unexpected for adsorption in a microporous system with pore size of the order of 0.5 to 0.
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