1,273 results match your criteria: "Center for Functional Materials[Affiliation]"
Nat Commun
February 2024
Physics Department, Sapienza University of Rome, Piazzale Aldo Moro 5, 00185, Rome, Italy.
Moiré excitons (MXs) are electron-hole pairs localised by the periodic (moiré) potential forming in two-dimensional heterostructures (HSs). MXs can be exploited, e.g.
View Article and Find Full Text PDFNano Lett
March 2024
Max-Planck-Institut für Festköperforschung, Stuttgart 70569, Germany.
Due to Landau quantization, the conductance of two-dimensional electrons exposed to a perpendicular magnetic field exhibits oscillations that generate a fan of linear trajectories when plotted in the parameter space spanned by density and field. This fan looks identical, irrespective of the dispersion and field dependence of the Landau level energy. This is no surprise because the position of conductance minima depends solely on the level degeneracy that is linear in flux.
View Article and Find Full Text PDFChem Commun (Camb)
February 2024
Research Center for Functional Materials, National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba 305-0044, Ibaraki, Japan.
Nanoarchitectonics, as a post-nanotechnology concept, constructs functional materials and structures using nanounits of atoms, molecules, and nanomaterials as materials. With the concept of nanoarchitectonics, asymmetric structures, and hierarchical organization, rather than mere assembly and organization of structures, can be produced, where rational physical and chemical communications will lead to the development of more advanced functional materials. Layer-by-layer assembly can be a powerful tool for this purpose, as exemplified in this feature paper.
View Article and Find Full Text PDFNat Commun
January 2024
QuTech and Kavli Institute of Nanoscience, Delft University of Technology, 2600 GA, Delft, The Netherlands.
Bilayer graphene encapsulated in tungsten diselenide can host a weak topological phase with pairs of helical edge states. The electrical tunability of this phase makes it an ideal platform to investigate unique topological effects at zero magnetic field, such as topological superconductivity. Here we couple the helical edges of such a heterostructure to a superconductor.
View Article and Find Full Text PDFNat Nanotechnol
May 2024
Department of Physics, University of California at Berkeley, Berkeley, CA, USA.
Transition metal dichalcogenide-based moiré superlattices exhibit strong electron-electron correlations, thus giving rise to strongly correlated quantum phenomena such as generalized Wigner crystal states. Evidence of Wigner crystals in transition metal dichalcogenide moire superlattices has been widely reported from various optical spectroscopy and electrical conductivity measurements, while their microscopic nature has been limited to the basic lattice structure. Theoretical studies predict that unusual quasiparticle excitations across the correlated gap between upper and lower Hubbard bands can arise due to long-range Coulomb interactions in generalized Wigner crystal states.
View Article and Find Full Text PDFACS Nano
February 2024
School of Electrical Engineering, Korea Advanced Institute of Science and Technology (KAIST), Daejeon 34141, Republic of Korea.
Applying a drain bias to a strongly gate-coupled semiconductor influences the carrier density of the channel. However, practical applications of this drain-bias-induced effect in the advancement of switching electronics have remained elusive due to the limited capabilities of its current modulation known to date. Here, we show strategies to largely control the current by utilizing drain-bias-induced carrier type switching in an ambipolar molybdenum disulfide (MoS) field-effect transistor with Pt bottom contacts.
View Article and Find Full Text PDFNat Mater
April 2024
Centre for Advanced 2D Materials, National University of Singapore, Singapore, Singapore.
In anisotropic crystals, the direction-dependent effective mass of carriers can have a profound impact on spin transport dynamics. The puckered crystal structure of black phosphorus leads to direction-dependent charge transport and optical response, suggesting that it is an ideal system for studying anisotropic spin transport. To this end, we fabricate and characterize high-mobility encapsulated ultrathin black-phosphorus-based spin valves in a four-terminal geometry.
View Article and Find Full Text PDFACS Nano
January 2024
Instituto de Ciencias de Materiales de Sevilla (Consejo Superior de Investigaciones Científicas-Universidad de Sevilla), C/Américo Vespucio, 49, Sevilla 41092, Spain.
Quantum-dot (QD) solids are being widely exploited as a solution-processable technology to develop photovoltaic, light-emission, and photodetection devices. Charge transport in these materials is the result of a compromise between confinement at the individual QD level and electronic coupling among the different nanocrystals in the ensemble. While this is commonly achieved by ligand engineering in colloidal-based systems, ligand-free QD assemblies have recently emerged as an exciting alternative where nanostructures can be directly grown into porous matrices with optical quality as well as control over their connectivity and, hence, charge transport properties.
View Article and Find Full Text PDFNanomaterials (Basel)
December 2023
Department of Applied Mechanics and Project Engineering, Mining and Industrial Engineering School of Almaden, University of Castilla-La Mancha, 13400 Almadén, Spain.
This study focuses on the fabrication of polymer nanocomposite films using polyvinyl alcohol (PVA)/graphene quantum dots (GQDs). We investigate the relationship between the structural, thermal, and nanoscale morphological properties of these films and their photoluminescent response. Although according to X-ray diffraction (XRD), Fourier-transform infrared spectroscopy (FT-IR), and differential thermal analysis (DTA), the incorporation of GQDs does not significantly affect the percentage crystallinity of the PVA matrix, for a range of added GQD concentrations, atomic force microscopy (AFM) showed the formation of islands with apparent crystalline morphology on the surface of the PVA/GQD films.
View Article and Find Full Text PDFPhys Rev Lett
December 2023
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
Moiré superlattices have emerged as an exciting condensed-matter quantum simulator for exploring the exotic physics of strong electronic correlations. Notable progress has been witnessed, but such correlated states are achievable usually at low temperatures. Here, we report evidence of possible room-temperature correlated electronic states and layer-hybridized SU(4) model simulator in AB-stacked MoS_{2} homobilayer moiré superlattices.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2024
Hubei Engineering & Technology Research Center for Functional Materials from Biomass, School of Chemistry and Material Science, Hubei Engineering University, Xiaogan, Hubei 432000, China.
Anion exchange membranes (AEMs) are increasingly becoming a popular research area due to their ability to function with nonprecious metals in electrochemical devices. Nevertheless, there is a challenge to simultaneously optimize the dimensional stability and ionic conductivity of AEMs due to the "trade-off" effect. Herein, we adopted a novel strategy of combining filling and cross-linking using functionalized bacterial cellulose (PBC) as a dual-functional porous support and brominated poly(phenylene oxide) (Br-PPO) as the cross-linking agent and filler.
View Article and Find Full Text PDFNat Mater
February 2024
Department of Physics, University of California at Berkeley, Berkeley, CA, USA.
Electron superlattices allow the engineering of correlated and topological quantum phenomena. The recent emergence of moiré superlattices in two-dimensional heterostructures has led to exciting discoveries related to quantum phenomena. However, the requirement for the moiré pattern poses stringent limitations, and its potential cannot be switched on and off.
View Article and Find Full Text PDFNat Mater
February 2024
Department of Physics, University of Washington, Seattle, WA, USA.
Moiré excitons are emergent optical excitations in two-dimensional semiconductors with moiré superlattice potentials. Although these excitations have been observed on several platforms, a system with dynamically tunable moiré potential to tailor their properties is yet to be realized. Here we present a continuously tunable moiré potential in monolayer WSe, enabled by its proximity to twisted bilayer graphene (TBG) near the magic angle.
View Article and Find Full Text PDFHeliyon
January 2024
School of Materials Science and Engineering, Shanghai University, Shanghai 200444, China.
Copper-doped Zinc Tellurium (ZnTe:Cu) films were deposited on borosilicate glass using magnetron co-sputtering technique. The influence of the substrate temperature on the structural, morphological, optical and electrical properties of ZnTe:Cu films was investigated by X-ray diffraction (XRD), Raman spectroscopy, X-ray photoelectron spectroscopy (XPS), atomic force microscopy (AFM), UV-Vis spectrophotometer and Hall effect measurement system. The results indicate that substrate temperature significantly affects the properties of the ZnTe:Cu films.
View Article and Find Full Text PDFNat Mater
May 2024
Department of Physics, University of California at Berkeley, Berkeley, CA, USA.
J Am Chem Soc
January 2024
Hoffmann Institute of Advanced Materials, Shenzhen Polytechnic University, 7098 Liuxian Boulevard, Shenzhen, Guangdong 518055, P. R. China.
Alkali metal-based metal-organic frameworks (MOFs) with permanent porosity are scarce because of their high tendency to coordinate with solvents such as water. However, these MOFs are lightweight and bear gravimetric benefits for gas adsorption related applications. In this study, we present the successful construction of a microporous MOF, designated as HIAM-111, built solely on sodium ions by using an octacarboxylate linker.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2024
School of Materials and Chemical Technology, Tokyo Institute of Technology, Yokohama 226-8502, Japan.
Tetragonal (1-)(Bi,Na)TiO-BaTiO films exhibit enhanced piezoelectric properties due to domain switching over a wide composition range. These properties were observed over a significantly wider composition range than the morphotropic phase boundary (MPB), which typically has a limited composition range of 1-2%. The polarization axis was found to be along the in-plane direction for the tetragonal composition range = 0.
View Article and Find Full Text PDFNano Lett
January 2024
Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Shenyang National Laboratory for Materials Science, School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China.
Graphene nanoribbons (GNRs), quasi one-dimensional (1D) narrow strips of graphene, have shown promise for high-performance nanoelectronics due to their exceptionally high carrier mobility and structurally tunable bandgaps. However, producing chirality-uniform GNRs on insulating substrates remains a big challenge. Here, we report the successful growth of bilayer GNRs with predominantly armchair chirality and ultranarrow widths (<5 nm) on insulating hexagonal boron nitride (h-BN) substrates using chemical vapor deposition (CVD).
View Article and Find Full Text PDFNature
December 2023
Department of Materials Science and Engineering, Northwestern University, Evanston, IL, USA.
Moiré quantum materials host exotic electronic phenomena through enhanced internal Coulomb interactions in twisted two-dimensional heterostructures. When combined with the exceptionally high electrostatic control in atomically thin materials, moiré heterostructures have the potential to enable next-generation electronic devices with unprecedented functionality. However, despite extensive exploration, moiré electronic phenomena have thus far been limited to impractically low cryogenic temperatures, thus precluding real-world applications of moiré quantum materials.
View Article and Find Full Text PDFNat Commun
December 2023
Department of Physics, University of California, Berkeley, CA, 94720, USA.
Coupled two-dimensional electron-hole bilayers provide a unique platform to study strongly correlated Bose-Fermi mixtures in condensed matter. Electrons and holes in spatially separated layers can bind to form interlayer excitons, composite Bosons expected to support high-temperature exciton condensates. The interlayer excitons can also interact strongly with excess charge carriers when electron and hole densities are unequal.
View Article and Find Full Text PDFMater Adv
December 2023
Physics and Center for Functional Materials, Faculty of Science and Engineering, Åbo Akademi University Turku 20500 Finland
Organic electrochemical transistors (OECTs) are widely employed in several bioelectronic applications such as biosensors, logic circuits, and neuromorphic engineering, providing a seamless link between the realm of biology and electronics. More specifically, OECTs are endowed with remarkable signal amplification, the ability to operate in an aqueous environment, and the effective transduction of ionic to electrical signals. One main limiting factor preventing OECTs' wide use is the need for microfabrication processes, typically requiring specialized equipment.
View Article and Find Full Text PDFLight Sci Appl
December 2023
School of Physics and Technology, Center for Nanoscience and Nanotechnology, and Key Laboratory of Artificial Micro- and Nanostructures of Ministry of Education, Wuhan University, 430072, Wuhan, China.
Various exciton species in transition metal dichalcogenides (TMDs), such as neutral excitons, trions (charged excitons), dark excitons, and biexcitons, have been individually discovered with distinct light-matter interactions. In terms of valley-spin locked band structures and electron-hole configurations, these exciton species demonstrate flexible control of emission light with degrees of freedom (DOFs) such as intensity, polarization, frequency, and dynamics. However, it remains elusive to fully manipulate different exciton species on demand for practical photonic applications.
View Article and Find Full Text PDFNat Nanotechnol
February 2024
Department of Physics, University of Regensburg, Regensburg, Germany.
Nano Lett
December 2023
Photonics Laboratory, ETH Zürich, 8093 Zürich, Switzerland.
Tunneling light-emitting devices (LEDs) based on transition metal dichalcogenides (TMDs) and other two-dimensional (2D) materials are a new platform for on-chip optoelectronic integration. Some of the physical processes underlying this LED architecture are not fully understood, especially the emission at photon energies higher than the applied electrostatic potential, so-called overbias emission. Here we report overbias emission for potentials that are near half of the optical bandgap energy in TMD-based tunneling LEDs.
View Article and Find Full Text PDFNat Commun
November 2023
JARA-FIT and 2nd Institute of Physics, RWTH Aachen University, 52074, Aachen, Germany.
The coherent dynamics of a quantum mechanical two-level system passing through an anti-crossing of two energy levels can give rise to Landau-Zener-Stückelberg-Majorana (LZSM) interference. LZSM interference spectroscopy has proven to be a fruitful tool to investigate charge noise and charge decoherence in semiconductor quantum dots (QDs). Recently, bilayer graphene has developed as a promising platform to host highly tunable QDs potentially useful for hosting spin and valley qubits.
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