High-speed asynchronous optical sampling with sub-50fs time resolution.

We report an ultrafast time-domain spectroscopy system based on high-speed asynchronous optical sampling operating without mechanical scanner. The system uses two 1 GHz femtosecond oscillators that are offset-stabilized using high-bandwidth feedback electronics operating at the tenth repetition rate harmonics. Definition of the offset frequency, i.

Terahertz emission from lateral photo-Dember currents.

The photo-Dember effect is a source of impulsive THz emission following femtosecond pulsed optical excitation. This emission results from the ultrafast spatial separation of electron-hole pairs in strong carrier gradients due to their different diffusion coefficients. The associated time dependent polarization is oriented perpendicular to the excited surface which is inaptly for efficient out coupling of THz radiation.

Efficient nonlinear light emission of single gold optical antennas driven by few-cycle near-infrared pulses.

Individual nanometer-sized plasmonic antennas are excited resonantly with few-cycle laser pulses in the near infrared. Intense third-harmonic emission of visible light prevails for fundamental photon energies below 1.1 eV.

Rapid-scanning terahertz precision spectrometer with more than 6 THz spectral coverage.

We report a terahertz time-domain spectrometer with more than 6 THz spectral coverage and 1 GHz resolution based on high-speed asynchronous optical sampling. It operates at 2 kHz scan rate without mechanical delay stage. The frequency error of the system at 60 s acquisition time is determined by comparing a measured water vapor absorption spectrum to data reported in the HITRAN database.

10-GHz self-referenced optical frequency comb.

The femtosecond laser-based frequency comb has played a key role in high-precision optical frequency metrology for a decade. Although often referred to as a precise optical frequency ruler, its tick marks are in fact too densely spaced for direct observation and individual use, limiting important applications in spectroscopy, astronomy, and ultrafast electromagnetic waveform control. We report on a femtosecond laser frequency comb with a 10-gigahertz repetition rate that creates a stabilized output spectrum with coverage from 470 to 1130 nanometers.

Compact coherent anti-Stokes Raman scattering microscope based on a picosecond two-color Er:fiber laser system.

We present a compact coherent anti-Stokes Raman scattering microscope based on a widely tunable picosecond Er:fiber laser. Intense and bandwidth-limited 1 ps pump pulses at a center wavelength of 775 nm are generated via frequency mixing within the broadband fundamental at 1.55 microm.

Highly versatile confocal microscopy system based on a tunable femtosecond Er:fiber source.

The performance of a confocal microscopy setup based on a single femtosecond fiber system is explored over a broad range of pump wavelengths for both linear and nonlinear imaging techniques. First, the benefits of a laser source in linear fluorescence excitation that is continuously tunable over most of the visible spectrum are demonstrated. The influences of subpicosecond pulse durations on the bleaching behavior of typical fluorophores are discussed.

Sub-cycle switch-on of ultrastrong light-matter interaction.

Controlling the way light interacts with material excitations is at the heart of cavity quantum electrodynamics (QED). In the strong-coupling regime, quantum emitters in a microresonator absorb and spontaneously re-emit a photon many times before dissipation becomes effective, giving rise to mixed light-matter eigenmodes. Recent experiments in semiconductor microcavities reached a new limit of ultrastrong coupling, where photon exchange occurs on timescales comparable to the oscillation period of light.

Dynamics of photoinduced charge-density-wave to metal phase transition in K0.3MoO3.

We present the first systematic studies of the photoinduced phase transition from the ground charge density wave (CDW) state to the normal metallic state in the prototype quasi-1D CDW system K0.3MoO3. Ultrafast nonthermal CDW melting is achieved at the absorbed energy density that corresponds to the electronic energy difference between the metallic and CDW states.

8-fs pulses from a compact Er:fiber system: quantitative modeling and experimental implementation.

We demonstrate an all-fiber turnkey source of extremely stable 2-cycle pulses at a center wavelength of 1.17 microm. Taylor-cut highly nonlinear germano-silica bulk fibers (HNFs) provide smooth supercontinua with a bandwidth of 560 nm and a spectral shape precisely controlled by the dispersion of the fiber and the phase of the 1.

Phase-locked generation and field-resolved detection of widely tunable terahertz pulses with amplitudes exceeding 100 MV/cm.

Phase-locked terahertz transients with peak electric fields of 108 MV/cm and center frequencies continuously tunable from 10 to 72 THz are generated via difference-frequency mixing of two parametrically amplified pulse trains from a single white-light seed. Free space electro-optic sampling with 8 fs gating pulses from a two-branch Er:fiber laser allows us to monitor all transients directly in the time domain. We identify extreme terahertz nonlinearities in the detector crystal with subcycle resolution.

Colloidal ZnO quantum dots in ultraviolet pillar microcavities.

Three dimensional light confinement and distinct pillar microcavity modes in the ultraviolet have been observed in pillar resonators with embedded colloidal ZnO quantum dots fabricated by focused ion beam milling. Results from a waveguide model for the mode patterns and their spectral positions are in excellent agreement with the experimental data.

Ultrafast spin dynamics in colloidal ZnO quantum dots.

Time-resolved Faraday rotation measurements in the ultraviolet have been performed to reveal the ultrafast spin dynamics of electrons in colloidal ZnO quantum dots. Oscillating Faraday rotation signals are detected at frequencies corresponding to an effective g factor of g = 1.96.

1-GHz repetition rate femtosecond OPO with stabilized offset between signal and idler frequency combs.

We report an optical parametric oscillator (OPO) based on periodically poled lithium niobate (PPLN) that is synchronously pumped by a femtosecond Ti:sapphire laser at 1 GHz repetition rate. The signal output has a center wavelength of 1558 nm and its spectral bandwidth amounts to 40 nm. The OPO operates in a regime where the signal- and idler frequency combs exhibit a partial overlap around 1600 nm.

Attosecond relative timing jitter and 13 fs tunable pulses from a two-branch Er:fiber laser.

We present what is believed to be the first direct measurement of the relative timing jitter between the two parallel pulse trains of a two-branch femtosecond erbium-doped fiber laser, operated without active stabilization. The system provides independently tunable pulses in the near infrared with durations down to 13 fs. Using an interferometric optical cross-correlator, the phase-noise spectral density is measured with high sensitivity in a range from 1 Hz up to the Nyquist frequency of 24.

Coherent structural dynamics and electronic correlations during an ultrafast insulator-to-metal phase transition in VO2.

We directly trace the multi-THz conductivity of VO2 during an insulator-metal transition triggered by a 12-fs light pulse. The femtosecond dynamics of lattice and electronic degrees of freedom are spectrally discriminated. A coherent wave packet motion of V-V dimers at 6 THz modulates the lattice polarizability for approximately 1 ps.

Colloidal quantum dots in all-dielectric high-Q pillar microcavities.

We have fabricated all-dielectric high-Q optical pillar resonators with embedded colloidal CdSe/ZnS quantum dots or rods as light emitters by focused ion beam milling. Three-dimensional light confinement and distinct pillar microcavity modes are observed. Results from a waveguide model for the mode patterns and their spectral positions are in excellent agreement with the experimental data.

Ultrafast time-domain spectroscopy based on high-speed asynchronous optical sampling.

High-speed asynchronous optical sampling (ASOPS) is a novel technique for ultrafast time-domain spectroscopy (TDS). It employs two mode-locked femtosecond oscillators operating at a fixed repetition frequency difference as sources of pump and probe pulses. We present a system where the 1 GHz pulse repetition frequencies of two Ti:sapphire oscillators are linked at an offset of Deltaf(R)=10 kHz.

A surface phase transition of supported gold nanoparticles.

A thermal phase transition has been resolved in gold nanoparticles supported on a surface. By use of asynchronous optical sampling with coupled femtosecond oscillators, the Lamb vibrational modes could be resolved as a function of annealing temperature. At a temperature of 104 degrees C the damping rate and phase changes abruptly, indicating a structural transition in the particle, which is explained as the onset of surface melting.

Multimilliwatt ultrashort pulses continuously tunable in the visible from a compact fiber source.

We report on a single-pass device that efficiently converts the broadband near-infrared output from a femtosecond fiber laser into a narrow spectrum in the visible. With fan-out poled MgO:LiNbO3 we obtain sub-picosecond, continuously tunable pulses in the 520-700 nm range. Conversion efficiencies as high as 30% are observed at typical pump power levels of 30 mW, corresponding to average output powers up to 9.