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Phase diagrams and dynamical evolution of the triple-pathway electro-oxidation of formic acid on platinum.
Phys Chem Chem Phys
January 2020
Max-Planck Institute for the Physics of Complex Systems, Nöthnitzer Str. 38, 01187 Dresden, Germany and Instituto de Altos Estudos da Paraíba, Rua Silvino Lopes 419-2502, 58039-190 João Pessoa, Brazil and Complexity Sciences Center, 9225 Collins Avenue Suite 1208, Surfside, FL 33154-3001, USA.
Recently, an electro-kinetic model based on a specified reaction scheme for the electro-oxidation of formic acid on platinum was reported. The model evaluated three reaction pathways towards the production of CO2: the dehydrogenation and the dehydration of formic acid, and the third and most active pathway includes fast oxidation of the formate ion. Numerical integrations showed that the model is well-suited to describe the experimental results in voltammetric and oscillatory regimes.
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