Correlated Dirac Fermions in Twisted Bilayers of MoS.

Artificial honeycomb lattices are essential for understanding exotic quantum phenomena arising from the interplay between Dirac physics and electron correlation. This work shows that the top two moiré valence bands in rhombohedral-stacked twisted MoS bilayers (tb-MoS) form a honeycomb lattice with massless Dirac fermions. The hopping and Coulomb interaction parameters are explicitly determined based on large-scale ab initio calculations.

Disorder-order transition-induced unusual bandgap bowing effect of tin-lead mixed perovskites.

Owing to the predominant merit of tunable bandgaps, tin-lead mixed perovskites have shown great potentials in realizing near-infrared optoelectronics and are receiving increasing attention. However, despite the merit, there is still a lack of fundamental understanding of the bandgap variation as a function of Sn/Pb ratio, mainly because the films are easy to segregate in terms of both composition and phase. Here, we report a fully stoichiometric synthesis of monocrystalline FAPbSnI nanocrystals as well as their atomic-scale imaging.

Experimental revival of an unknown state from the past in quantum walks.

The physical process in the macroscopic world unfolds along a single time direction, while the evolution of a quantum system is reversible in principle. How to recover a quantum system to its past state is a complex issue of both fundamental and practical interests. In this article, we experimentally demonstrate a novel method for recovering the state in quantum walks (QWs), also known as full-state revival.

Observing quantum coherent oscillations in a three-level atom via electromagnetically induced transparency by two-dimensional spectroscopy.

Two-dimensional electronic spectroscopy (2DES) has high spectral resolution and is a useful tool for studying atomic dynamics. In this paper, we show a smallest unit of electromagnetically induced transparency (EIT) for 2DES, i.e.

Competition between Bipolar Conduction Modes in Extrinsically -Doped MoS: Interaction with Gate Dielectric Matters.

With reduced dimensionality and a high surface area-to-volume ratio, two-dimensional (2D) semiconductors exhibit intriguing electronic properties that are exceptionally sensitive to surrounding environments, including directly interfacing gate dielectrics. These influences are tightly correlated to their inherent behavior, making it critical to examine when extrinsic charge carriers are intentionally introduced to the channel for complementary functionality. This study explores the physical origin of the competitive transition between intrinsic and extrinsic charge carrier conduction in extrinsically -doped MoS, highlighting the central role of interactions of the channel with amorphous gate dielectrics.

Length-dependent water permeation through a graphene channel.

Water confined in two-dimensional channels exhibits unique properties, such as rich morphology, specific phase transition and a low dielectric constant. In this work, molecular dynamics simulations have been used to study the water transport in two-dimensional graphene channels. The structures and dynamics of water under confinement show strong dependence on the channel length and thickness of the channels.

Nature of Disordering in γ-Ga_{2}O_{3}.

Polymorphs commonly exist for various materials, enabling phase engineering for diverse material properties. While the crystal structures of different polymorphs can, in principle, be experimentally characterized, interpreting and understanding complex crystal structures can be very challenging. Using Ga_{2}O_{3} as a prototype, here we show that the crystal structure of γ-Ga_{2}O_{3} has long been misinterpreted from either theory or experiment.

Bio-inspired multi-dimensional deep fusion learning for predicting dynamical aerospace propulsion systems.

Rapid and precise forecasting of dynamical systems is critical to ensuring safe aerospace missions. Previous forecasting research has primarily concentrated on global trend analysis using full-scale inputs. However, time series arising from real-world applications such as aerospace propulsion, exhibit a distinct dynamical periodicity over a limited timeframe.

Oxygen Defect Site Filling Strategy Induced Moderate Enrichment of Reactants for Efficient Electrocatalytic Biomass Upgrading.

The electrocatalytic oxidation of 5-hydroxymethylfurfural (HMF) provides a feasible approach for the efficient utilization of biomass. Defect regulation is an effective strategy in the field of biomass upgrading to enhance the adsorption capacity of reactants and thus increase the activity. However, how to select appropriate strategies to regulate the over-enrichment of reactants induced by excessive oxygen vacancy is still a huge challenge.

Charge stripe manipulation of superconducting pairing symmetry transition.

Charge stripes have been widely observed in many different types of unconventional superconductors, holding varying periods ( ) and intensities. However, a general understanding on the interplay between charge stripes and superconducting properties is still incomplete. Here, using large-scale unbiased numerical simulations on a general inhomogeneous Hubbard model, we discover that the charge-stripe period , which is variable in different real material systems, could dictate the pairing symmetries-d wave for and d waves for .

Oxide-Metal Hybrid Glass Nanomembranes with Exceptional Thermal Stability.

Contrary to oxide or polymeric glasses, metallic glasses are infamously known for their relatively limited thermal stability, which is often characterized by their narrow supercooled liquid regions. Nonetheless, we successfully fabricated metallic-glass based nanomembranes with an ultrahigh thermal ability by a polymer surface buckling enabled exfoliation technique. These nanomembranes exhibit a distinctive nanostructure with nanosized metallic-glasses encapsulated within an interconnected nanoamorphous-oxide network.

Understanding solvent polarity effects on the separation of uranyl porphyrin-derivative complexes.

Solvation is a crucial task in developing efficient and selective extractants for actinide elements, but an understanding and perspective of solvent effects on the extraction of uranyl are still lacking. Herein, we present investigations into solvent effects on the geometry, stability and bonding properties of five uranyl porphyrin derivative complexes (UO(L)) in four solvents relativistic quantum chemical calculations, and reveal some trends in the influence of solvent polarity on uranyl compounds. All five [L] ligands equatorially coordinate [UO] in a hexa-dentate (κ) fashion.

Interpretable and Physicochemical-Intuitive Deep Learning Approach for the Design of Thermal Resistance of Energetic Compounds.

Thermal resistance of energetic materials is critical due to its impact on safety and sustainability. However, developing predictive models remains challenging because of data scarcity and limited insights into quantitative structure-property relationships. In this work, a deep learning framework, named EM-thermo, was proposed to address these challenges.

Minimum Tracking Linear Response Hubbard and Hund Corrected Density Functional Theory in CP2K.

We present the implementation of the Hubbard () and Hund () corrected Density Functional Theory (DFT + + ) functionality in the Quickstep program, which is part of the CP2K suite. The tensorial and Löwdin subspace representations are implemented and compared. Full analytical DFT + + forces are implemented and benchmarked for the tensorial and Löwdin representations.

Diagnosing Quantum Phase Transition Order and Deconfined Criticality via Entanglement Entropy.

We study the scaling behavior of the Rényi entanglement entropy with smooth boundaries at the putative deconfined critical point separating the Néel antiferromagnetic and valence-bond-solid states of the two-dimensional J-Q_{3} model. We observe a subleading logarithmic term with a coefficient indicating the presence of four Goldstone modes, signifying the presence of an SO(5) symmetry at the transition point, which spontaneously breaks into an O(4) symmetry in the thermodynamic limit. This result supports the conjecture that an SO(5) symmetry emerges at the transition point, but reveals the transition to be weakly first-order.

Incognizant 1T/1H Charge-Density-Wave Phases in Monolayer NbTe.

While experimental realization of multiple charge-density waves (CDWs) has been ascribed to monolayer 1T-NbTe, their atomic structures are still largely unclear, preventing a deep understanding of their novel electronic structures. Here, comparing first-principles-calculated orbital textures with reported STM measurements, we successfully identify multiple CDWs in monolayer NbTe. Surprisingly, we reveal that both 1T/1H phases could exist in monolayer NbTe, which was incognizant before.