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Surface phonon polaritons (SPhPs) are coupled photon-phonon excitations that emerge at the surfaces of nanostructured materials. Although they strongly influence the optical and thermal behavior of nanomaterials, no technique has been able to reveal the complete three-dimensional (3D) vectorial picture of their electromagnetic density of states. Using a highly monochromated electron beam in a scanning transmission electron microscope, we could visualize varying SPhP signatures from nanoscale MgO cubes as a function of the beam position, energy loss, and tilt angle.

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