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Solvatochromism and cis-trans isomerism in azobenzene-4-sulfonyl chloride.
Photochem Photobiol Sci
January 2025
CQC-IMS, Department of Chemistry, University of Coimbra, 3004-535, Coimbra, Portugal.
Solvatochromism exhibited by azobenzene-4-sulfonyl chloride (here abbreviated as Azo-SCl) has been investigated in a series of non-polar, polar-aprotic and polar-protic solvents. The UV-vis spectra of Azo-SCl exhibit two long-wavelength bands, observed at 321-330 nm (band-I) and 435-461 nm (band-II), which are ascribed to the π*-π (S ← S) and π*-n (S ← S) transitions, respectively. The shorter wavelength band indicates a reversal in solvatochromism, from negative to positive solvatochromism, for a solvent with a dielectric constant of 32.
View Article and Find Full Text PDFField-particle energy transfer during chorus emissions in space.
Nature
January 2025
Southwest Research Institute, San Antonio, TX, USA.
Chorus waves are some of the strongest electromagnetic emissions naturally occurring in space and can cause radiation that is hazardous to humans and satellites. Although chorus waves have attracted extreme interest and been intensively studied for decades, their generation and evolution remain highly debated. Here, in contrast to the conventional expectation that chorus waves are governed by planetary magnetic dipolar fields, we report observations of repetitive, rising-tone chorus waves in the terrestrial neutral sheet, where the effects of the magnetic dipole are absent.
View Article and Find Full Text PDFA 1D coordination compound made of a photochromic dithienylethene linker and [Dy(Tp2-py)F]+ units (with Tp2-py = tris(3-(2-pyridyl)pyrazolyl)hydroborate) and having tetrakis[3,5-bis(trifluoromethyl)phenyl]borate counterions is reported. Full photoconversion from the closed isomer to the open isomer of the dithienyethene within single crystals allow for monitoring of the transformation by photocrystallography. Magnetic slow relaxation as well as magnetic hysteresis are observed and can be both modulated upon light irradiation.
View Article and Find Full Text PDFDipolar wavevector interference induces a polar skyrmion lattice in strained BiFeO films.
Nat Nanotechnol
January 2025
Bay Area Center for Electron Microscopy, Songshan Lake Materials Laboratory, Dongguan, China.
Skyrmions can form regular arrangements, so-called skyrmion crystals (SkXs). A mode with multiple wavevectors q then describes the arrangement. While magnetic SkXs, which can emerge in the presence of Dzyaloshinskii-Moriya interaction, are well established, polar skyrmion lattices are still elusive.
View Article and Find Full Text PDFLong-Range Charge Transport Facilitated by Electron Delocalization in MoS and Carbon Nanotube Heterostructures.
ACS Nano
January 2025
Department of Chemistry, Purdue University, West Lafayette, Indiana 47907, United States.
Controlling charge transport at the interfaces of nanostructures is crucial for their successful use in optoelectronic and solar energy applications. Mixed-dimensional heterostructures based on single-walled carbon nanotubes (SWCNTs) and transition metal dichalcogenides (TMDCs) have demonstrated exceptionally long-lived charge-separated states. However, the factors that control the charge transport at these interfaces remain unclear.
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