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Facile Aqueous Route to Large-Scale Superhydrophilic TiO-Incorporated Graphitic Carbon Nitride-Coated Ni(OH) and NiP Nano-Architecture Arrays as Efficient Electrocatalysts for Enhanced Hydrogen Production.
Langmuir
January 2025
Department of Chemistry, Faculty of Science, University of Kurdistan, Pasdaran Boulevard, Sanandaj 66177-15175, Iran.
Water splitting by an electrochemical method to generate hydrogen gas is an economic and green approach to resolve the looming energy and environmental crisis. Designing a composite electrocatalyst having integrated multichannel charge separation, robust stability, and low-cost facile scalability could be considered to address the issue of electrochemical hydrogen evolution. Herein, we report a superhydrophilic, noble-metal-free bimetallic nanostructure TiO/NiP coated on graphitic polyacrylonitrile carbon fibers (g-C/TiO/NiP) using a facile hydrothermal method followed by phosphorylation.
View Article and Find Full Text PDFComparative study of single-port single-channel and single-port multi-channel adrenalectomy in various maximum tumor diameters.
BMC Surg
January 2025
The First Affiliated Hospital of Nanjing Medical University, 300 Guangzhou Road, Nanjing, 210029, China.
Background: Investigating the application of single-port single-channel and single-port multi-channel adrenalectomy in various maximum tumor diameters.
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Semiconductive Coordination Polymer with Multi-Channel Charge Transfer for High-Performance Direct X-ray Detection.
Angew Chem Int Ed Engl
December 2024
State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun, 130012, P. R. China.
Coordination polymers (CPs) are promising for direct X-ray detection and imaging owing to higher designability and outstanding stability, however, it remains a challenge to achieve highly X-ray detection performance, particularly both high sensitivity and low detection limit at the same operating voltage. Herein, we construct a new conjugated CP {[Co(BPTTz)(DIPA)] ⋅ DMA} (1, BPTTz=2,5-bis(pyridine-4-yl)thiazolo[5,4-d]thiazole, HDIPA=2,5-diiodoterephthalic acid, DMA=N, N'-dimethylacetamide), with multi-channel charge transfer by regulating the linker mediated electronic-state, which reduces carrier losses resulting from recombination or quenching, enhances the efficiency of charge separation and transfer, thus further optimizes X-ray detection performance. The semiconductor prepared based on this strategy achieves record values including the highest mobility-lifetime product (μτ, 8.
View Article and Find Full Text PDFA press-actuated slidable microfluidic colorimetric biosensor for Salmonella detection utilizing nickel mesh sheet and MIL-88@Pd/Pt nanoparticles.
Food Chem
March 2025
Key Laboratory of Agricultural Information Acquisition Technology, Ministry of Agriculture and Rural Affairs, China Agricultural University, Beijing 100083, China. Electronic address:
A press-actuated slidable microfluidic colorimetric biosensor was designed for rapid, sensitive and multi-channel detection of Salmonella. The nickel mesh sheet (NMS) modified with capture antibodies was employed for capturing target bacteria, and metal organic frameworks decorated with palladium (Pd) and platinum (Pt) nanoparticles (MIL-88@Pd/Pt NPs) modified with detection antibodies were used for amplifying colorimetric signals. The capture efficiency of the immune NMS reached 83 %, and the detection limit of this colorimetric biosensor was 35 CFU/mL in 20 min.
View Article and Find Full Text PDFEstimating global phase synchronization by quantifying multivariate mutual information and detecting network structure.
Neural Netw
November 2024
Beijing Institute of Functional Neurosurgery, Xuanwu Hospital, Capital Medical University, Beijing 100053, China. Electronic address:
In neuroscience, phase synchronization (PS) is a crucial mechanism that facilitates information processing and transmission between different brain regions. Specifically, global phase synchronization (GPS) characterizes the degree of PS among multivariate neural signals. In recent years, several GPS methods have been proposed.
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