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Polarizability, plasmons and damping in pseudospin-1 gapped materials with a flat band.
J Phys Condens Matter
December 2024
Space Vehicles Directorate, US Air Force Research Laboratory, Kirtland Air Force Base, Albuquerque, NM 87117, United States of America.
The subject of our present investigation is the collective electronic properties of various types of pseudospin-1 Dirac-cone materials with a flat band and finite bandgaps in their low-energy spectra. Specifically, we have calculated the dynamical polarization, plasmon dispersions, as well as their decay rates due to Landau damping and presented the closed-form analytical expressions for the wave function overlaps for both the gapped dice lattice and the Lieb lattice. The gapped dice lattice is a special case of the more general-T3model such that its band structure is symmetric and the flat band remains dispersionless.
View Article and Find Full Text PDFStrongly coupled magneto-exciton condensates in large-angle twisted double bilayer graphene.
Nat Commun
June 2024
National Laboratory of Solid-State Microstructures, School of Physics, Nanjing University, Nanjing, 210093, China.
Excitons, pairs of electrons and holes, undergo a Bose-Einstein condensation at low temperatures. An important platform to study excitons is double-layer two-dimensional electron gases, with two parallel planes of electrons and holes separated by a thin insulating layer. Lowering this separation (d) strengthens the exciton binding energy, however, leads to the undesired interlayer tunneling, resulting in annihilation of excitons.
View Article and Find Full Text PDFIdentification of the interchromophore interaction in the electronic absorption and circular dichroism spectra of bis-phenanthrenes.
Phys Chem Chem Phys
February 2024
State Key Laboratory of Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, Fujian Provincial Key Laboratory of Theoretical and Computational Chemistry, and Department of Chemistry, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, P. R. China.
We characterize the low-lying excited electronic states of a series of bis-phenanthrenes using our newly developed diabatic scheme called the fragment particle-hole density (FPHD) method and calculate both the electronic absorption and circular dichroism (ECD) spectra using the time-dependent density functional theory (TDDFT) and the FPHD-based exciton model which couples intrachromophore local excitations (LEs) and the interchromophore charge-transfer excitations (CTEs). TDDFT treats each bis-phenanthrene as a single molecule while the mixed LE-CTE exciton model partitions the molecule into two phenanthrene-based aromatic moieties, and then applies the electronic coupling between the various quasi-diabatic states to cover the interactions. It is found that TDDFT and the mixed LE-CTE model reproduce all experimentally observed trends in the spectral profiles, and the hybridization between LE and CTE states is displayed differently in absorption and ECD spectral intensities, as it usually decreases the absorption maxima and affects the positive/negative extrema of the ECD irregularly.
View Article and Find Full Text PDFQuantum Phase Transition in Magnetic Nanographenes on a Lead Superconductor.
Nano Lett
November 2023
Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), TD Lee Institute, Shenyang National Laboratory for Materials Science, School of Physics and Astronomy, Shanghai Jiao Tong University, 800 Dongchuan Road, Shanghai 200240, China.
Quantum spins, also known as spin operators that preserve SU(2) symmetry, lack a specific orientation in space and are hypothesized to display unique interactions with superconductivity. However, spin-orbit coupling and crystal field typically cause a significant magnetic anisotropy in d/f shell spins on surfaces. Here, we fabricate atomically precise = 1/2 magnetic nanographenes on Pb(111) through engineering sublattice imbalance in the graphene honeycomb lattice.
View Article and Find Full Text PDFTopological Circular Dichroism in Chiral Multifold Semimetals.
Phys Rev Lett
September 2023
Department of Physics, Northeastern University, Boston, Massachusetts 02115, USA.
Uncovering the physical contents of the nontrivial topology of quantum states is a critical problem in condensed matter physics. Here, we study the topological circular dichroism in chiral semimetals using linear response theory and first-principles calculations. We show that, when the low-energy spectrum respects emergent SO(3) rotational symmetry, topological circular dichroism is forbidden for Weyl fermions, and thus is unique to chiral multifold fermions.
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