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Activation and Catalysis of Methane over Metal-Organic Framework Materials.
Acc Mater Res
January 2025
Department of Chemistry, University of Manchester, Manchester M13 9PL, U.K.
Methane (CH), which is the main component of natural gas, is an abundant and widely available carbon resource. However, CH has a low energy density of only 36 kJ L under ambient conditions, which is significantly lower than that of gasoline (. 34 MJ L).
View Article and Find Full Text PDFThe Role of Surfactant in Electrocatalytic Carbon Dioxide Reduction in the Absence of Metal Cations.
ACS Electrochem
January 2025
Stephenson Institute for Renewable Energy (SIRE) and the Department of Chemistry, University of Liverpool, Liverpool L69 7ZF, United Kingdom.
Carbon dioxide electroreduction does not occur on Au when metal cations are absent from the electrode surfaces. Here we show that the electroreduction can be enabled without metal cations, albeit with low efficiency, by the presence of cationic surfactants on Au. The findings demonstrate that in addition to possibly stabilizing CO reduction intermediates the presence of surfactants plays a role in suppressing the competing reactions.
View Article and Find Full Text PDFResonances in Low-Energy Electron Collisions with Salicylic Acid.
J Phys Chem A
January 2025
Departamento de Física, Universidade Federal do Paraná, Caixa Postal 19044, 81531-980 Curitiba, Paraná, Brazil.
In this work, we report elastic integral, differential, and momentum-transfer cross sections for the scattering of low-energy electrons by salicylic acid. The cross sections were calculated with the Schwinger multichannel method implemented with norm-conserving pseudopotential within the static-exchange and static-exchange plus polarization (SEP) approximations for energies up to 15 eV. In the SEP approximation, four π* resonances were found at around 0.
View Article and Find Full Text PDFOptimized Interface Engineering Enhances Carrier and Phonon Scattering for Superior Thermoelectric Performance in Yb-Filled Skutterudites.
ACS Appl Mater Interfaces
January 2025
Key Laboratory of Radiation Physics and Technology, Ministry of Education, Institute of Nuclear Science and Technology, Sichuan University, Chengdu 610064, China.
Thermoelectric (TE) performance in materials is often constrained by the strong coupling between carrier and phonon transport, necessitating trade-offs between electrical and thermal properties that limit improvements in the figure of merit (). Herein, a novel strategy is proposed to achieve simultaneous energy filtering and enhanced phonon scattering, effectively optimizing the TE properties of CoSb-based skutterudites. By introducing CuTe nanoprecipitates into the YbCoSb matrix, interfacial barriers are formed, which selectively filter low-energy charge carriers, significantly improving the Seebeck coefficient while maintaining high carrier mobility.
View Article and Find Full Text PDFAttix free-air chamber correction factors computed using EGSnrc.
Med Phys
January 2025
Department of Medical Physics, School of Medicine and Public Health, University of Wisconsin-Madison, Madison, Wisconsin, USA.
Background: A cylindrical free-air chamber, the Attix FAC, is used for absolute air-kerma measurements of low-energy photon beams at the University of Wisconsin Medical Radiation Research Center. Correction factors for air-kerma measurements of specific beams were determined in the 1990s. In order to measure air-kerma rates of beams in development, new correction factors must be computed.
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