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Understanding water reaction pathways to control the hydrolytic reactivity of a Zn metal-organic framework.
Nat Commun
December 2024
Department of Chemistry, University of Western Ontario, London, Ontario, N6A 5B7, Canada.
Metal-organic frameworks (MOFs) are a class of porous materials that are of topical interest for their utility in water-related applications. Nevertheless, molecular-level insight into water-MOF interactions and MOF hydrolytic reactivity remains understudied. Herein, we report two hydrolytic pathways leading to either structural stability or framework decomposition of a MOF (ZnMOF-1).
View Article and Find Full Text PDFRapid and well-controlled degradation of polylactic acid materials with bio-based GEL(pectin/α-cellulose/SiO/CaCl).
Int J Biol Macromol
December 2024
College of Chemical Engineering and Materials Science, Tianjin University of Science & Technology, Tianjin 300457, China. Electronic address:
Polylactic acid (PLA) has been a subject of considerable interest as a degradable polymer. However, the degradation process is slow and uncontrollable. In this work, controlled degradable PLA/bio-based GEL (pectin/α-cellulose/SiO/CaCl) hydrophilic plasticizer composite material was successfully prepared by solution blending process.
View Article and Find Full Text PDFNovel frontiers through nitrogen substitution at 6th, 10th and 11th position of artemisinin: Synthetic approaches and antimalarial activity.
Eur J Med Chem
January 2025
Department of Chemistry, Banasthali University, Banasthali Newai, 304022, Rajasthan, India; Department of Education in Science and Mathematics (DESM), Regional Institute of Education (NCERT), Bhubaneshwar, 751022, India. Electronic address:
Malaria pertains to an array of catastrophic illnesses spurred on by the Plasmodium spp. Artemisinin (ART) is currently prescribed in conjunction with another medication as part of therapeutic regimens for acute malaria. These currently prescribed pharmaceuticals have been around for a while, even after lack of required thermos-metabolic stabilities, alongside fresh proclaims about surfacing resistance and neurotoxicity linked with sequential administration of such combination therapies.
View Article and Find Full Text PDFImproved volatile fatty acid production in anaerobic digestion via simultaneous temperature regulation and persulfate activation by biochar: Chemical and biological response mechanisms.
Environ Res
January 2025
Beijing Key Laboratory of Farmland Soil Pollution Prevention and Remediation, College of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, China. Electronic address:
Increasing volatile fatty acid (VFA) production via persulfate activation (i.e., chemical effect) in anaerobic digestion (AD) is an emerging resource utilization method.
View Article and Find Full Text PDFA novel CBM serving as a module for efficiently decomposing xanthan by modifying the processivity of hydrolase.
Carbohydr Polym
January 2025
School of Biological Engineering, Dalian Polytechnic University, Ganjingziqu, Dalian, PR China. Electronic address:
The inefficient decomposition of polysaccharides, particularly branched polysaccharides limits their large-scale industrial applications. Further understanding and modification of glycoside hydrolases (GHs) processivity is expected to overcome this limitation. Here, a novel xanthan-binding CBM (MiXBM), which was supposed to alter the processivity of GHs, was systematically characterized.
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