We propose a mechanism for generating single photons in the mid-infrared (MIR) using a solid-state or molecular quantum emitter. The scheme uses cavity quantum electrodynamics (QED) effects to selectively enhance a Frank-Condon transition, deterministically preparing a single Fock state of a polar phonon mode. By coupling the phonon mode to an antenna, the resulting excitation is then radiated to the far field as a single photon with a frequency matching the phonon mode. By combining macroscopic QED calculations with methods from open quantum system theory, we show that optimal parameters to generate these MIR photons occur for modest light-matter coupling strengths, which are achievable with state-of-the-art technologies. Combined, the cascaded system we propose provides a quasi-deterministic source of heralded single photons in a regime of the electromagnetic spectrum where this previously was not possible.

Download full-text PDF

Source
http://dx.doi.org/10.1126/sciadv.adr9239DOI Listing

Publication Analysis

Top Keywords

phonon mode
12
quantum system
8
system propose
8
single photons
8
on-demand heralded
4
heralded mir
4
mir single-photon
4
single-photon source
4
source cascaded
4
quantum
4

Similar Publications

We propose a mechanism for generating single photons in the mid-infrared (MIR) using a solid-state or molecular quantum emitter. The scheme uses cavity quantum electrodynamics (QED) effects to selectively enhance a Frank-Condon transition, deterministically preparing a single Fock state of a polar phonon mode. By coupling the phonon mode to an antenna, the resulting excitation is then radiated to the far field as a single photon with a frequency matching the phonon mode.

View Article and Find Full Text PDF

While coupling between optical, electronic, and mechanical domains is paramount for high-frequency acoustic devices, materials that offer tunability in the degree of such coupling can be crucially enabling in expanding device functionality. Here, we show that the interaction of photons with coherent acoustic phonons confined in 2D layered semiconducting cavities can be controlled through either modifying the material state via a thermally induced electronic bandgap shift (EBS) or altering the polarization state of the incoming photons when optical birefringence is present in the cavity. We demonstrate temperature-driven EBS as an effective tool to engineer the WSe cavity readout as it allows one to sweep the excitonic energy relative to a chosen probe wavelength.

View Article and Find Full Text PDF

Strain-Induced Enhancement of the Charge Density Wave in the Kagome Metal ScV_{6}Sn_{6}.

Phys Rev Lett

February 2025

Istituto Officina dei Materiali, Consiglio Nazionale delle Ricerche, Trieste I-34149, Italy.

The kagome geometry is an example of a frustrated configuration in which rich physics takes place, including the emergence of superconductivity and charge density wave (CDW). Among the kagome metals, ScV_{6}Sn_{6} hosts an unconventional CDW, with its electronic order showing a different periodicity from the leading lattice instability. In this material, a CDW-softened flat phonon band has a second-order collapse at the same time that the first-order transition occurs.

View Article and Find Full Text PDF

Stimulated Brillouin scattering (SBS) provides a robust and versatile foundation for the development of mode-locked lasers, microwave signal generators, and optical gyroscopes across diverse optical platforms. Nonetheless, the relatively low efficacy of Brillouin interactions in traditional silicon photonic waveguides presents a barrier to the advances of silicon-based Brillouin laser technology. The emergence of hybrid photonic-phononic waveguides has brought to light the robust and adaptable nature of Brillouin interactions in silicon, marking a significant advancement.

View Article and Find Full Text PDF

Two-dimensional conjugated metal-organic frameworks (2D c-MOFs) have emerged as an intriguing class of quantum materials due to their high crystallinity, persistent spin centers, and tunable structures and topologies. However, it remains unclear how to achieve long spin relaxation time at room temperature in 2D c-MOFs via a bottom-up design strategy. Herein, we design a hexahydroxytrithiatruxene ligand (HHTH) to minimize the influence of nuclear spin on electron spin relaxation while weakening -π conjugation to construct a "spin docking" for preserving spin centers, which enables the resulting 2D c-MOFs, NiHHTH, to exhibit quantum coherence and Rabi oscillations at room temperature.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!