Lithium-ion batteries are indispensable power sources for a wide range of modern electronic devices. However, battery lifespan remains a critical limitation, directly affecting the sustainability and user experience. Conventional battery failure analysis in controlled lab settings may not capture the complex interactions and environmental factors encountered in real-world, in-device operating conditions. This study analyzes the failure of commercial wireless earbud batteries as a model system within their intended usage context. Through multiscale and multimodal characterizations, the degradations from the material level to the device level are correlated, elucidating a failure pattern that is closely tied to the specific device configuration and operating conditions. The findings indicate that the ultimate failure mode is determined by the interplay of battery materials, cell structural design, and the in-device microenvironment, such as temperature gradients and their fluctuations. This holistic, in-device perspective on environmental influences provides critical insights for battery integration design, enhancing the reliability of modern electronics.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1002/adma.202416915 | DOI Listing |
Adv Mater
March 2025
Walker Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX, 78712, USA.
Lithium-ion batteries are indispensable power sources for a wide range of modern electronic devices. However, battery lifespan remains a critical limitation, directly affecting the sustainability and user experience. Conventional battery failure analysis in controlled lab settings may not capture the complex interactions and environmental factors encountered in real-world, in-device operating conditions.
View Article and Find Full Text PDFACS Appl Mater Interfaces
March 2025
College of Energy, Soochow University, Suzhou 215006, P. R. China.
Flexible aqueous zinc-ion batteries (AZIBs) are considered one of the most attractive flexible devices owing to their high theoretical capacity, low cost, and high security. However, the formation of Zn dendrites and the poor flexibility of the Zn material greatly impede the application of wearable AZIBs. Herein, by transferring graphene onto the surface of polyethylene terephthalate-indium tin oxide (PET-ITO-G), a substrate combining excellent flexibility and dendrite suppression ability was prepared.
View Article and Find Full Text PDFSmall
March 2025
School of Advanced Materials, Peking University Shenzhen Graduate School, Shenzhen, 518055, P. R. China.
Hard carbon is the sole anode material employed in commercial sodium-ion batteries. However, its intrinsic defects and impurities will lead to battery failure, diminishing further development of sodium batteries in energy storage. Here, an acrylonitrile copolymer and poly(ethylene oxide) (LA/PEO) composite binder is developed to address these challenges in biomass-derived hard carbon.
View Article and Find Full Text PDFNano Lett
March 2025
College of Physics and Energy, Fujian Normal University, Fuzhou 350117, China.
Combined solid electrolytes address cathode-anode compatibility in all-solid-state Li-ion batteries (ASSLBs), yet interface stability and ion transport mechanisms between different electrolytes remain unclear. Herein, we investigate LiPSCl (LPSC), LiInCl (LIC), and LiZrOCl (LZOC) composite electrolytes through electrochemical analysis and operando X-ray photoelectron spectroscopy. Our results reveal that the electrostatic potential difference between LPSC and LIC inhibits Li migration, leading to the decomposition of LIC into InCl and LiCl, causing battery failure.
View Article and Find Full Text PDFAdv Mater
March 2025
School of Future Technology, State Key Laboratory for Mechanical Behavior of Materials, Shaanxi International Research Center for Soft Matter, Xi'an Jiaotong University, Xi'an, 710049, China.
All-solid-state batteries (ASSBs) are promising candidates for next-generation energy storage devices due to their high energy density and enhanced safety. Binder plays an irreplaceable role in stabilizing the electrode structure, enhancing carrier transport and modulating solid electrolyte interfaces by connecting each component of the electrode. The development of functional binders is seen as a key strategy to achieve higher energy densities of ASSBs.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!