We consider the quantum dynamics of a pair of coupled quantum oscillators coupled to a common correlated dissipative environment. The resulting equations of motion for both the operator moments and covariances can be integrated analytically using the Lyapunov equations. We find that for fully correlated and fully anti-correlated environments, the oscillators relax into a phase-synchronized state that persists for long-times when the two oscillators are nearly resonant and (essentially) forever if the two oscillators are in resonance. We identify an exceptional point that indicates the onset of broken symmetry between an unsynchronized and synchronized dynamical phase of the system as correlations within the environment are increased. We also show that the environmental noise correlation leads to quantum entanglement, and all the correlations between the two oscillators are purely quantum mechanical in origin. This work provides a robust mathematical foundation for understanding how long-lived exciton coherences can be linked to vibronic correlation effects.
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http://dx.doi.org/10.1063/5.0246275 | DOI Listing |
J Am Chem Soc
March 2025
Spin-X Institute, School of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 511442, China.
The electric control of magnetism has been considered to be promising for molecular spintronics and quantum information. However, the spin-electric coupling strength appears to be insufficient for application in most cases. Two major factors capable of amplifying the relative effect are spin-orbit coupling and ferroelectricity.
View Article and Find Full Text PDFSci Adv
March 2025
Department of Electrical and Photonics Engineering, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark.
We propose a mechanism for generating single photons in the mid-infrared (MIR) using a solid-state or molecular quantum emitter. The scheme uses cavity quantum electrodynamics (QED) effects to selectively enhance a Frank-Condon transition, deterministically preparing a single Fock state of a polar phonon mode. By coupling the phonon mode to an antenna, the resulting excitation is then radiated to the far field as a single photon with a frequency matching the phonon mode.
View Article and Find Full Text PDFSci Adv
March 2025
Department of Physics and Guangdong Basic Research Center of Excellence for Quantum Science, Southern University of Science and Technology, Shenzhen, 518055, P. R. China.
Developing high-performance photothermal materials and unraveling the underlying mechanism are essential for photothermal applications. Here, photothermal performance improved by strong interaction between plasmon and topological surface state (TSS) is demonstrated in BiSe/CuS nanowires. This hybrid, which CuS nanosheets were grown on BiSe nanowires, leverages the plasmon resonance and TSS-induced optical property, generating wide and efficient light absorption.
View Article and Find Full Text PDFRadiol Phys Technol
March 2025
Center for Frontier Medical Engineering, Chiba University, Chiba, Japan.
Positron emission tomography (PET) is a valuable tool for diagnosing malignant tumors. Intraoperative PET imaging is expected to allow the more accurate localization of tumors that need resections. However, conventional devices feature a large detector ring that obstructs surgical procedures, preventing their intraoperative application.
View Article and Find Full Text PDFNanomaterials (Basel)
March 2025
Department of Optical Engineering, School of Opto-Electronic Engineering, Changchun University of Science and Technology, Changchun 130022, China.
Wet etching is the mainstream fabrication method for single-bar quantum cascade lasers (QCLs). Different etching solutions result in varying etching effects on III-V semiconductor materials. In this study, an efficient and nearly ideal etching solution ratio was proposed for simultaneously etching both InP and GaInAs/AlInAs, and the surface chemical reactions induced by each component of the etching solution during the process were investigated.
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