Plastic is a widely used material across various industries, including construction, packaging, healthcare, and automotive, among others. Global plastic production was estimated at 311 million tonnes in 2014 and is expected to double within two decades, continuing to rise towards 2050. As plastic pollution poses significant environmental and health risks, effective recycling and upcycling strategies are crucial for sustainable waste management. This paper explores the impact of plastic waste on public health and ecosystems, reviews chemical, mechanical, and biological recycling methods, and examines upcycling approaches. It also addresses key challenges such as limitations in chemical upcycling, scaling up carbonization, and inefficiencies in sorting and processing for mechanical recycling. Additionally, recent innovations-including enzymatic depolymerization for PET recycling, upcycling plastic waste into advanced carbon materials like graphene and carbon nanotubes, photochemical and photocatalytic upcycling, PVC recycling via Cl-transfer systems, and advancements in mechanical recycling for multi-layer plastics-are discussed to highlight emerging solutions in plastic waste management. By addressing these challenges and gaps, this paper provides valuable insights into advancing plastic waste management through innovative recycling and upcycling technologies, paving the way for more sustainable and environmentally friendly solutions to combat global plastic pollution.
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http://dx.doi.org/10.1016/j.jenvman.2025.124867 | DOI Listing |
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March 2025
Engineering Laboratory for AgroBiomass Recycling & Valorizing, College of Engineering, China Agricultural University, Beijing, 100083, China.
Chemical upcycling of plastic waste to produce green H has emerged as a promising avenue. Highly efficient and robust NiAlO catalysts with dual active nanocomposite (NiO-NiAlO) through a facile electronic configuration modulation strategy are synthesized for the decomposition-catalytic steam reforming (DCSR) of plastic wastes for enhancing H production while alleviating carbon deposition. Of these dual-active nanocomposite catalysts, NiAlO-800 presents the highest proportions of Ni cations and oxygen vacancies, contributing to the enhance structural stability and catalytic activity.
View Article and Find Full Text PDFNanomaterials (Basel)
February 2025
Zhongyuan Critical Metal Laboratory, School of Chemical Engineering, Zhengzhou University, Zhengzhou 450001, China.
The excessive utilization and emission of waste plastics have caused serious damage to the environment, and it is of great significance to explore high-value utilization methods for these waste plastics. To address this challenge, functional nano cobalt-loaded porous carbon materials (CoPC) with excellent antibiotic wastewater removal properties were prepared by one-step pyrolysis using waste PET plastics as a carbon source, a process described in this paper. Characterization revealed that the obtained CoPC-2 catalysts had a high degree of defects, a large specific surface area (343.
View Article and Find Full Text PDFMetab Eng Commun
June 2025
The Novo Nordisk Foundation Center for Biosustainability, Technical University of Denmark, Kemitorvet, Building 220, 2800, Kgs. Lyngby, Denmark.
Whole-cell biocatalysis facilitates the production of a wide range of industrially and pharmaceutically relevant molecules from sustainable feedstocks such as plastic wastes, carbon dioxide, lignocellulose, or plant-based sugar sources. The identification and use of efficient enzymes in the applied biocatalyst is key to establishing economically feasible production processes. The generation and selection of favorable enzyme variants in adaptive laboratory evolution experiments using growth as a selection criterion is facilitated by tightly coupling enzyme catalytic activity to microbial metabolic activity.
View Article and Find Full Text PDFRSC Adv
March 2025
Department of Chemistry, Dwaraka Doss Goverdhan Doss Vaishnav College (Autonomous) (Affiliated to the University of Madras, Chennai) 833, Gokul Bagh, E.V.R. Periyar Road, Arumbakkam Chennai 600 106 Tamil Nadu India +919677146579.
This research introduces a Mn/Zn-activated carbon (AC) bimetallic catalyst for hydroprocessing polypropylene pyrolysis oil (PPO) into hydroprocessed polypropylene pyrolysis oil blend (HPPO-B), which closely mimics commercial diesel. Under optimized conditions (70 bar, 350 °C), the catalyst efficiently converts PPO into iso-alkanes, -alkanes, and aromatics, achieving a 95% compositional match with diesel. HPPO-B meets European EN590 diesel standards, with viscosity (3.
View Article and Find Full Text PDFEcotoxicol Environ Saf
March 2025
Finnish Institute of Occupational Health, Helsinki 00250, Finland; Department of Anatomy, Embryology and Genetics, University of Zaragoza, Zaragoza 50013, Spain. Electronic address:
The increasing use of plastic polymers in 3D printing applications may lead to human exposure to micro- and nanoplastics (MNPLs), raising concerns regarding adverse health consequences such as cancer induction. Little attention has been given to MNPLs originated at the end of the life cycle of 3D-printed objects because of the mechanical and environmental degradation of plastic waste. This study assessed the carcinogenic potential of secondary MNPLs generated through cryomilling of 3D objects using the validated in vitro Bhas 42 cell transformation assay (CTA).
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