Smart surfaces with switchable adhesion have garnered significant attention in wearable devices, robotics, and biological detection. However, achieving universal switchable adhesion at both solid and liquid interfaces is still challenging. Here, we report a thermo-induced biomimetic switchable slippery interface (TBSSI) with robust solid and liquid adhesion, inspired by octopus tentacles and slippery mussels. Relying on femtosecond laser drilling on soft PDMS sheets and the infusion of phase-change paraffin, a smart surface of the TBSSI is fabricated. Liquid adhesion is achieved at room temperature, while solid adhesion is achieved through the phase transition of paraffin excited by Joule heating, exhibiting a robust adhesion strength of ≈142 kPa. Mechanical abrasion tests demonstrate the exceptional self-repairing capability and excellent retainability of the surface adhesion strength. This work should provide new insights into the designs of universal adhesive surfaces and advance related fields, such as ultrafast laser microfabrication and soft robotics.
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http://dx.doi.org/10.1021/acs.nanolett.4c05723 | DOI Listing |
Nano Lett
March 2025
CAS Key Laboratory of Mechanical Behavior and Design of Materials, Department of Precision Machinery and Precision Instrumentation, University of Science and Technology of China, Hefei, 230027, P. R. China.
Smart surfaces with switchable adhesion have garnered significant attention in wearable devices, robotics, and biological detection. However, achieving universal switchable adhesion at both solid and liquid interfaces is still challenging. Here, we report a thermo-induced biomimetic switchable slippery interface (TBSSI) with robust solid and liquid adhesion, inspired by octopus tentacles and slippery mussels.
View Article and Find Full Text PDFChemistry
December 2021
State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, 130021, P. R. China.
The polymorphs of 2ClChMe-4 in Form I (ribbon-like crystal) and Form II (block-like crystal) were prepared, and they exhibited curling/flipping and expansion upon heating on account of single-crystal-to-single-crystal transformations. The irreversible phase transformations occurred separately at 53.2 °C and 57.
View Article and Find Full Text PDFAdv Sci (Weinh)
December 2021
State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou, 730000, China.
Directional transportation of objects has important applications from energy transfer and intelligent robots to biomedical devices. Although breakthroughs in liquid migration on 2D surfaces or 3D tubular devices have been achieved, realizing smooth/on-demand transportation of constrained solids within a 3D cavity environment under harsh pressurized environment still remains a daunting challenge, where strong interface friction force becomes the main obstacle restricting the movement of solids. Inspired by typical feeding mechanism in natural esophagus system which synergistically couples a lubricating mucosa surface with the peristaltic contraction deformation of the cavity, herein, this challenge is addressed by constructing an esophagus-inspired layered tubular actuator with a slippery inner surface and responsive hydrogel matrix to realize spherical solid propulsion by photo(thermo)-induced cavity deformation.
View Article and Find Full Text PDFBiomimetics (Basel)
February 2019
School of Materials Science, Japan Advanced Institute of Science and Technology, 1-1 Asahidai, Nomi, Ishikawa 923-1292, Japan.
Capsaicin is a natural compound that produces a warm sensation and is known for its remarkable medicinal properties. Understanding the interaction between capsaicin with lipid membranes is essential to clarify the molecular mechanisms behind its pharmacological and biological effects. In this study, we investigated the effect of capsaicin on thermoresponsiveness, fluidity, and phase separation of liposomal membranes.
View Article and Find Full Text PDFSmall
March 2015
Radboud University Nijmegen, Institute for Molecules and Materials (IMM), Heyendaalseweg 135, 6525, AJ, Nijmegen, The Netherlands.
Diphenylalanine peptide nano- and microtubes formed by self-assembly demonstrate strongly enhanced and tunable single-photon and two-photon luminescence in the visible range, which appears after heat- or laser treatment of these self-organized peptide microtubes. This process significantly extends the functionality of these microstructures and can trigger a new interest in the optical properties of structures based on short peptides.
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