The motional sideband asymmetry of a mechanical oscillator interacting with a laser field can be observed when approaching the quantum ground state, where the zero-point energy of the mechanical oscillator becomes a sizable contribution to its motion. In the context of quantum optomechanics, it allows, in principle, calibration-free inference of the thermal equilibrium of a macroscopic mechanical resonator with its optical bath. At room temperature, this phenomenon has been observed in pioneering experiments using levitated nanoparticles. Measuring this effect with solid-state mechanical resonators has been compounded by thermal intermodulation noise, mirror frequency noise and low quantum cooperativity. Here, we sideband-cool a membrane-in-the-middle system close to the quantum ground state from room temperature and observe motional sideband asymmetry in a dual-homodyne measurement. Sideband thermometry yields a minimum phonon occupancy of n[over ¯]_{eff}=9.5. Our work provides insights into nonlinear optomechanical dynamics at room temperature and facilitates accessible optomechanical quantum technologies without the need for complex feedback control and cryogenic cooling.
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http://dx.doi.org/10.1103/PhysRevLett.134.073602 | DOI Listing |
Small Methods
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School of Materials and Energy, Lanzhou University, Lanzhou, 730000, P. R. China.
Solid polymer electrolytes (SPEs) have garnered significant attention from both academic and industrial communities due to their high safety feature and high energy density in combination with lithium(Li) metal anode. Nevertheless, their practical applications remain constrained by the relatively low room-temperature ionic conductivity and interface issues. Anion-derived cation-anion aggregates (AGGs), derived from high-concentration liquid electrolytes, promote a stable solid-electrolyte interphase layer, which have gradually propelled their application in SPEs.
View Article and Find Full Text PDFAdv Mater
March 2025
Institut de Physique et Chimie des Matériaux de Strasbourg, Université de Strasbourg, CNRS, UMR 7504, Strasbourg, F-67000, France.
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Department of Chemistry, Colorado State University, Fort Collins, CO 80523, USA.
A new deep-blue emitting and highly fluorescent anthracene (ANTH) derivative containing perfluorobenzyl (Bn) groups, 9,10-ANTH(Bn), was synthesized in a single step reaction of ANTH or ANTH(Br) with BnI, using either a high-temperature Cu-/NaSO-promoted reaction or via a room-temperature photochemical reaction. Its structure was elucidated by NMR spectroscopy and single crystal X-ray diffractometry. The latter revealed no π-π interaction between neighboring ANTH cores.
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Instituto Universitario CINQUIMA y Departamento de Química Orgánica, Facultad de Ciencias, Universidad de Valladolid, Paseo Belén 7, 47011-Valladolid, Spain.
The pharmaceutical chemical industry has long used kinetic resolution to obtain high-value compounds. Organocatalysis has recently been added to this strategy, allowing for the resolution of racemic mixtures with low catalyst loadings and mild reaction conditions. This research focuses on the kinetic resolution of 1,5-dicarbonyl compounds using a retro-Michael reaction, co-catalyzed at room temperature with 20 mol % of the Jørgensen-Hayashi catalyst and PNBA.
View Article and Find Full Text PDFBeilstein J Nanotechnol
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Ion Beam Centre, Department of Physics, Kurukshetra University, Kurukshetra-136119, India.
In this study, zinc telluride (ZnTe) films were grown on quartz substrates at room temperature, 300 °C, 400 °C, 500 °C, and 600 °C using RF sputtering. The thickness of the films has been found to decrease from 940 nm at room temperature to 200 nm at 600 °C with increasing substrate temperature. The structural investigation using grazing incidence angle X-ray diffraction revealed that films deposited at room temperature are amorphous; those deposited at other substrate temperatures are polycrystalline with a cubic zincblende structure and a preferred orientation along the [111] direction.
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