Neutron-induced reaction cross sections of short-lived nuclei are imperative to understand the origin of heavy elements in stellar nucleosynthesis and for societal applications, but their measurement is extremely complicated due to the radioactivity of the targets involved. One way of overcoming this issue is to combine surrogate reactions with the unique possibilities offered by heavy-ion storage rings. In this work, we describe the first surrogate-reaction experiment in inverse kinematics, which we successfully conducted at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, using the ^{208}Pb(p,p^{'}) reaction as a surrogate for neutron capture on ^{207}Pb. Thanks to the outstanding detection efficiencies possible at the ESR, we were able to measure for the first time the neutron-emission probability as a function of the excitation energy of ^{208}Pb. We have used this probability to select different descriptions of the γ-ray strength function and nuclear level density, and provide reliable results for the neutron-induced radiative capture cross section of ^{207}Pb at energies for which no experimental data exist.
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http://dx.doi.org/10.1103/PhysRevLett.134.072501 | DOI Listing |
Phys Rev Lett
February 2025
Université de Bordeaux, CNRS, LP2I Bordeaux, 33170 Gradignan, France.
Neutron-induced reaction cross sections of short-lived nuclei are imperative to understand the origin of heavy elements in stellar nucleosynthesis and for societal applications, but their measurement is extremely complicated due to the radioactivity of the targets involved. One way of overcoming this issue is to combine surrogate reactions with the unique possibilities offered by heavy-ion storage rings. In this work, we describe the first surrogate-reaction experiment in inverse kinematics, which we successfully conducted at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, using the ^{208}Pb(p,p^{'}) reaction as a surrogate for neutron capture on ^{207}Pb.
View Article and Find Full Text PDFPhys Rev Lett
July 2024
Sino-French Institute of Nuclear Engineering and Technology, Sun Yat-sen University, Zhuhai 519082, China.
We investigated decays of ^{51,52,53}K at the ISOLDE Decay Station at CERN in order to understand the mechanism of the β-delayed neutron-emission (βn) process. The experiment quantified neutron and γ-ray emission paths for each precursor. We used this information to test the hypothesis, first formulated by Bohr in 1939, that neutrons in the βn process originate from the structureless "compound nucleus.
View Article and Find Full Text PDFPhys Rev Lett
October 2022
Department of Physics and Astronomy, University of Tennessee, Knoxville, Tennessee 37996, USA.
The β-delayed one- and two-neutron emission probabilities (P_{1n} and P_{2n}) of 20 neutron-rich nuclei with N≥82 have been measured at the RIBF facility of the RIKEN Nishina Center. P_{1n} of ^{130,131}Ag, ^{133,134}Cd, ^{135,136}In, and ^{138,139}Sn were determined for the first time, and stringent upper limits were placed on P_{2n} for nearly all cases. β-delayed two-neutron emission (β2n) was unambiguously identified in ^{133}Cd and ^{135,136}In, and their P_{2n} were measured.
View Article and Find Full Text PDFRadiat Prot Dosimetry
August 2022
Slovak University of Technology in Bratislava, Faculty of Electrical Engineering and Information Technology, Ilkovičova 3, 81219 Bratislava, Slovakia.
The manganese sulphate bath is a globally recognized method for determining emission of neutrons from radionuclide since 1959. In combination with the measurement of neutron emission anisotropy, this method is standardly used for the primary standardization of dosimetry quantities of neutron radiation. To achieve results at the metrology level, it is essential to have all quantities which contribute to the overall uncertainty properly determined and contributing uncertainty minimized.
View Article and Find Full Text PDFPhys Rev Lett
April 2022
Riken Nishina Center for Accelerator-Based Science, Wako, Saitama 351-0198, Japan.
The Rare-RI Ring (R3) is a recently commissioned cyclotronlike storage ring mass spectrometer dedicated to mass measurements of exotic nuclei far from stability at Radioactive Isotope Beam Factory (RIBF) in RIKEN. The first application of mass measurement using the R3 mass spectrometer at RIBF is reported. Rare isotopes produced at RIBF-^{127}Sn, ^{126}In, ^{125}Cd, ^{124}Ag, ^{123}Pd-were injected in R3.
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