Perfluorooctanoic acid (PFOA), a novel contaminant, is extensively found in aquatic environments. However, the capability of the denitrifying phosphorus removal process to treat PFOA-containing wastewater, as well as its response mechanisms, are unclear. This study used batch experiments to assess the short-term impact of PFOA on denitrifying phosphorus removal systems. During a single cycle, the addition of PFOA predominantly enhanced phosphate removal in the system mainly by the anaerobic phosphorus release pathway, but had no substantial effect on nitrogen removal. COD removal efficiency has a substantial positive correlation with C6-HSL and C8-HSL concentrations. As the PFOA concentration increased, the ROS concentration and enzyme activity also increased, while the PN/PS ratio decreased, causing the sludge to become looser. At the beginning of the second cycle, the impact of PFOA on phosphorus removal efficiency shifted from promotion to inhibition. These findings shed fresh light on the influence of PFOA on the denitrifying phosphorus removal mechanism, potentially furthering its use in the treatment of fluoride-containing wastewater.
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http://dx.doi.org/10.1016/j.jes.2024.08.004 | DOI Listing |
Nanomaterials (Basel)
February 2025
College of Materials Science and Engineering, Xi'an University of Science and Technology, Xi'an 710054, China.
With the advancement of industrial production and urban modernization, pollution from heavy metal ions and the accumulation of solid waste have become critical global environmental challenges. Establishing an effective recycling system for solid waste and removing heavy metals from wastewater is essential. Coal gangue was used in this study as the primary material for the synthesis of a fully coal gangue-based phosphorus-silicon-aluminum (SAPO-5) molecular sieve through a hydrothermal process.
View Article and Find Full Text PDFNanomaterials (Basel)
February 2025
College of Materials Science and Engineering, Xi'an University of Science and Technology, Xi'an 710054, China.
The accumulation of organic pollutants and solid waste is one of the major environmental challenges faced globally. Establishing an efficient recycling system for solid waste and designing cost-effective, high-performance photocatalysts are urgent tasks for the removal of organic pollutants from water. This study utilizes coal gangue as the precursor to synthesize a coal gangue-based phosphorus-silicon-aluminum molecular sieve (SAPO-5) via hydrothermal synthesis.
View Article and Find Full Text PDFJ Environ Manage
March 2025
Hubei Three Gorges Laboratory, Yichang, Hubei, 443000, China.
Phosphogypsum (PG), a byproduct of phosphate fertilizer production, poses environmental pollution risks due to the potential release of impurities such as phosphorus, fluoride, and organic compounds, necessitating effective treatment and remediation. Among various methodologies, flotation has emerged as a key technique for separating impurities from PG. Although extensive research has been conducted on the separation and reuse of PG, studies focusing specifically on organic impurity separation and collector optimization are still limited.
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
March 2025
State Key Laboratory of Pollution Control and Resource Reuse, Key Laboratory of Aquatic Ecosystem Health in the Middle and Lower Reaches of Yangtze River, School of Environment, Nanjing University, Nanjing, 210023, China.
Cyanobacterial blooms, which carry a lot of nitrogen (N) and phosphorus (P), have emerged as one of the most severe environmental issues in freshwater ecosystems. However, there are few studies on the effect of organic matters released during cyanobacterial decomposition in promoting N release from lake sediments that remain underexplored. An essential step is to eliminate the impact of the N contributions from cyanobacteria when evaluating sedimentary N release.
View Article and Find Full Text PDFJ Environ Manage
March 2025
UCD Dooge Centre for Water Resources Research, School of Civil Engineering, University College Dublin, Newstead Building, Belfield, Dublin 4, Ireland.
Efficient hydraulic performance is critical for Constructed Wetlands (CWs), since poor hydraulic performance can reduce treatment efficiency by altering the actual residence time relative to the design value. However, no quantitative studies on the relationship between Hydraulic Efficiency (HE) and treatment efficiency in CWs have been reported to date. This study assessed the extent to which baffled-induced improvements in HE translated into improvements in pollutant removal efficiency.
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