In this paper, a vanadium dioxide (VO)-based terahertz device is proposed to realize the conversion between broadband absorption and broadband transmission functions, including the VO bottom layer, dielectric layer and VO pattern layer in a three-layer structure. With the change of the VO conductivity, the terahertz metamaterial device can switch between broadband absorption and broadband transmission. When the device exhibits broadband transmission, it has a high transmittance of 90% for terahertz waves in the 5.6 THz to 8.7 THz frequency band. When the device exhibits broadband absorption, it has a high 90% absorption of terahertz waves in the 3.66 THz to 9.98 THz frequency band. Furthermore, with increasing VO conductivity, the peak transmittance of the device decreases from 93.8% to 0% and the absorption increases from 1% to 99.5%. The impedance matching theory is invoked and the physical mechanism of the device is elucidated by analyzing the surface electric field of the device. By studying the absorption characteristics for different incidence and polarization angles, the device is insensitive to polarization and has good absorption performance over large incidence angles. Compared with other absorbers of terahertz metamaterials, the device structure proposed in this study has a unique design and diverse functions and can play an important role in various fields such as communications, electromagnetic stealth, sensors, and thermal emission devices.
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http://dx.doi.org/10.1039/d5dt00153f | DOI Listing |
Adv Mater
March 2025
Laboratory of Organic Electronics, Department of Science and Technology (ITN), Linköping University, Norrköping, SE-601 74, Sweden.
Chiral-specific interaction of light with organic materials is important but typically arises from circular polarization-dependent absorption of specific optical transitions, resulting in narrow effective wavelength ranges. This study presents a scalable and universal concept for broadband circular dichroism (CD) enabled by strained conducting polymer thin films that possess in-plane hyperbolic optical behavior (i.e.
View Article and Find Full Text PDFNanomaterials (Basel)
March 2025
Advanced Laser Technology Laboratory of Anhui Province, College of Electronic Engineering, National University of Defense Technology, Hefei 230037, China.
The compatibility of low infrared emission and wideband microwave absorption has drawn extensive attention, both theoretically and practically. In this paper, an infrared-radar-compatible stealth metasurface is designed using transparent conductive materials, namely indium tin oxide (ITO) and poly methacrylimide (PMI). The designed structure is a combination of a radar-absorbing layer (RAL) and a low-infrared-emission layer (IRSL), with an overall thickness of about 1.
View Article and Find Full Text PDFMater Horiz
March 2025
School of Applied & Interdisciplinary Sciences, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032, India.
Lead halide perovskites are widely recognized for their exceptional defect tolerance, setting the benchmark for high-performance optoelectronic applications. Conversely, low-toxicity perovskite-inspired materials (PIMs) typically exhibit suboptimal optoelectronic performance, primarily due to their intrinsic susceptibility to defects. In this study, we address this limitation by exploring the effects of halide vacancies in PIMs through the synthesis of non-stoichiometric CsBiBrI microcrystals (MCs) with a trigonal crystal structure, incorporating iodine vacancies.
View Article and Find Full Text PDFInorg Chem
March 2025
Materials Science and Technology Division, CSIR─National Institute for Interdisciplinary Science and Technology, Thiruvananthapuram, Kerala 695019, India.
Phosphor-converted white light-emitting diodes (pc-WLEDs) with a supreme color rendering index (CRI) remain challenging, particularly due to the limited accessibility of efficient cyan-green-emitting phosphors in the 480-520 nm emission range. Herein, a novel rare earth-free cyan-green-emitting Ta-substituted CsVO phosphor that exhibits a VO charge transfer enabled cyan-green emission band centered at ∼520 nm under the 370 nm near UV (n-UV) light is reported with an internal quantum efficiency of 93.9%.
View Article and Find Full Text PDFNanoscale
March 2025
School of Electrical Engineering, Ben-Gurion University of the Negev, Beer-Sheva 84105, Israel.
Broadband and omnidirectional absorption is the first requirement for any solar energy harvesting technology. For example, the realization of silicon thin-film photovoltaics is hampered by the low absorption coefficient of silicon. This work introduces a nano-light-mixer (NLM) array to address this hurdle.
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