Exciton polaritons formed by the strong coupling between excitons and photons have been extensively studied in transition metal disulfides (TMDs) for their potential to inherit ultralong radiation lifetime and remarkable nonlinearity. Many studies have achieved strong coupling at room temperature. However, the systems in these studies generally lack orderly characteristics and precise controllability, and their tunability also remains rather limited. Here, we demonstrate a plasmonic grating with a bound state in the continuum (BIC) as a highly tunable platform for generating exciton polaritons in monolayer WS at room temperature. We characterized the polariton modes and determined an energy splitting of 93 meV. This validates strong coupling in our system. Our research offers a new approach for exploring exciton polaritons in 2D semiconductors, opening doors for room-temperature optoelectronic and quantum computing applications.
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http://dx.doi.org/10.1021/acs.nanolett.4c06464 | DOI Listing |
Nat Commun
March 2025
Key Laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing, China.
An exciton-polariton condensate is a state of matter with collective coherence leading to many fascinating macroscopic quantum effects. Recently, optical bound states in the continuum (BICs) have been demonstrated as peculiar topological states capable of imparting novel characteristics onto the polariton condensates. Organic semiconductors featuring robust Frenkel excitons and high physicochemical tunability potentially offer a promising platform to explore topologically engineering of BIC polariton condensates at room temperature.
View Article and Find Full Text PDFACS Nano
March 2025
School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332, United States.
Exciton-polariton condensation offers a promising path to low-threshold coherent light sources, impacting fields from communications to healthcare. These hybrid quasiparticles, arising from strong exciton-photon coupling, combine the low effective mass from their photonic component and the strong nonlinear interactions from excitons. While polariton condensation has been achieved in a range of inorganic and organic materials, many systems still face significant challenges despite fulfilling the main properties requirements.
View Article and Find Full Text PDFPhys Rev Lett
February 2025
Carl von Ossietzky Universität Oldenburg, Institut für Physik, Fakultät V, 26129 Oldenburg, Germany.
MoTe_{2} monolayers and bilayers are unique within the family of van der Waals materials since they pave the way toward atomically thin infrared light-matter quantum interfaces, potentially reaching the important telecommunication windows. Here, we report emergent exciton polaritons based on MoTe_{2} monolayers and bilayers in a low-temperature open microcavity in a joint experiment-theory study. Our experiments clearly evidence both the enhanced oscillator strength and enhanced luminescence of MoTe_{2} bilayers, signified by a 38% increase of the Rabi splitting and a strongly enhanced relaxation of polaritons to low-energy states.
View Article and Find Full Text PDFNature
March 2025
CNR Nanotec, Institute of Nanotechnology, Lecce, Italy.
A supersolid is a counter-intuitive phase of matter in which its constituent particles are arranged into a crystalline structure, yet they are free to flow without friction. This requires the particles to share a global macroscopic phase while being able to reduce their total energy by spontaneous, spatial self-organization. The existence of the supersolid phase of matter was speculated more than 50 years ago.
View Article and Find Full Text PDFNano Lett
March 2025
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
Exciton polaritons formed by the strong coupling between excitons and photons have been extensively studied in transition metal disulfides (TMDs) for their potential to inherit ultralong radiation lifetime and remarkable nonlinearity. Many studies have achieved strong coupling at room temperature. However, the systems in these studies generally lack orderly characteristics and precise controllability, and their tunability also remains rather limited.
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