The Peach-Koehler force between disclination lines was originally formulated in the study of crystalline solids, and has since been adopted to provide a notion of interactions between disclination lines in nematic liquid crystals. Here, we argue that the standard formulation of this interaction force seemingly fails for materials where there is a symmetry-broken ground state, and suggest that this is due to the interaction between disclination lines and merons: non-singular yet non-trivial topological solitons. We examine this in the context of chiral nematic (cholesteric) liquid crystals, which provide a natural setting for studying these interactions due to their energetic preference for meron tubes in the form of double-twist cylinders. Through a combination of theory and simulation we demonstrate that, for sufficiently strong chirality, defects of +1/2 winding will change their winding through the emission of a meron line, and that interactions between the merons and defects dominate over defect-defect interactions. Instead of the Peach-Koehler framework, we employ a method based on contact topology-the Gray stability theorem-to directly calculate the velocity field of the material. We apply our framework to point defects as well as disclination lines. Our results have implications not just for chiral materials, but also for other phases with modulated ground states, such as the twist-bend and splay-bend nematics.
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http://dx.doi.org/10.1039/d4sm01478b | DOI Listing |
Soft Matter
February 2025
School of Physics, UNSW, Sydney, NSW 2052, Australia.
The Peach-Koehler force between disclination lines was originally formulated in the study of crystalline solids, and has since been adopted to provide a notion of interactions between disclination lines in nematic liquid crystals. Here, we argue that the standard formulation of this interaction force seemingly fails for materials where there is a symmetry-broken ground state, and suggest that this is due to the interaction between disclination lines and merons: non-singular yet non-trivial topological solitons. We examine this in the context of chiral nematic (cholesteric) liquid crystals, which provide a natural setting for studying these interactions due to their energetic preference for meron tubes in the form of double-twist cylinders.
View Article and Find Full Text PDFSci Adv
February 2025
Department of Physics, University of Science and Technology of China, Hefei, Anhui 230026, China.
In soft matter systems, there is a wealth of topological phenomena, such as singular disclination lines and nonsingular defects of skyrmions and hopfions. In a liquid crystal (LC), the topological nature of disclination lines and colloids induces chiral colloidal entanglements. How the chirality of the entanglements is deterministically created and how the chirality conversion is actuated in the disclinations with Möbius strip topology have never been explored.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
February 2025
Department of Applied Physics, Yale University, New Haven, CT 06511.
We have studied the magnetic moments of artificial spin ice arrays of nanomagnets in both undistorted square arrays and in arrays with a topological defect induced by a single disclination. We confirm that the disclination induces global, macroscopic changes in the low-energy collective states of the nanomagnet moment configuration. Specifically, the disclination leads to Faraday lines of effective magnetic flux that run from the center all the way to the edge of the arrays.
View Article and Find Full Text PDFACS Appl Mater Interfaces
February 2025
European Laboratory for Non-Linear Spectroscopy (LENS), Via Nello Carrara 1, 50019 Sesto Fiorentino, Italy.
Materials that can visually report changes in the surrounding environments are essential for future portable sensors that monitor temperature and detect hazardous chemicals. Ideal responsive materials for optical sensors are defined by a rapid response and readout, high selectivity, the ability to operate at room temperature, and simple microfabrication. However, because of the lack of viable materials and approaches, compact, passive, and multipurpose practical devices are still beyond reach.
View Article and Find Full Text PDFSoft Matter
February 2025
Department of Mechanical and Energy Engineering, Southern University of Science and Technology, Shenzhen, 518055, China.
We report an experimental study on how topological defects induced by cylindrical air inclusions in the ferroelectric nematic liquid crystal RM734 are influenced by ionic doping, including an ionic surfactant and ionic polymer. Our results show that subtle differences in molecular structure can lead to distinct surface alignments and topological defects. The ionic surfactant induces a planar alignment, with two -1/2 line defects adhering to the cylindrical bubble surface.
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