iScience
School of Information Science and Technology, Hangzhou Normal University, Hangzhou 311121, China.
Published: February 2025
Atomic spin gyroscopes (ASGs) based on spin-exchange relaxation-free (SERF) co-magnetometers represent a new generation of ultra-high-precision inertial sensors. However, their long-term stability is significantly constrained by the stability of electron spin polarization. Despite its critical importance, current research lacks effective methods for and real-time measurement of electron spin polarization. This paper addresses this gap by developing a model for pump laser propagation within the vapor cell and proposing an Euler-particle swarm optimization (PSO) algorithm to estimate the model's unknown parameters. By utilizing artificial neural networks, we derive an output equation for electron spin polarization, using transmitted laser power and cell temperature as independent variables. Comparative experiments validate the accuracy of the proposed method, and perturbation experiments demonstrate its real-time capability. The proposed real-time measurement method for electron spin polarization lays a solid foundation for improving closed-loop control and enhancing the long-term stability of ASGs.
Download full-text PDF |
Source |
---|---|
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC11791252 | PMC |
http://dx.doi.org/10.1016/j.isci.2025.111757 | DOI Listing |
Adv Mater
March 2025
Department of Chemical and Biomolecular Engineering, National University of Singapore, Singapore, 117585, Republic of Singapore.
Tuning transition metal spin states potentially offers a powerful means to control electrocatalyst activity. However, implementing such a strategy in electrochemical CO reduction (COR) is challenging since rational design rules have yet to be elucidated. Here we show how the addition of P dopants to a ferromagnetic element (Fe, Co, and Ni) single-atom catalyst (SAC) can shift its spin state.
View Article and Find Full Text PDFMaterials (Basel)
February 2025
Centre for Quantum Physics, Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement (MOE), School of Physics, Beijing Institute of Technology, Beijing 100081, China.
A topological insulator with large bulk-insulating behavior and high electron mobility of the surface state is needed urgently, not only because it would be a good platform for studying topological surface states but also because it is a prerequisite for potential future applications. In this work, we demonstrated that tin (Sn) or indium (In) dopants could be introduced into a BiSbTeSe single crystal. The impacts of the dopants on the bulk-insulating property and electron mobility of the surface state were systematically investigated by electrical transport measurements.
View Article and Find Full Text PDFInt J Mol Sci
February 2025
Departamento de Física, Universidad Nacional de Colombia, Carrera 30 No. 45-03, Bogota 111321, Colombia.
Energy levels associated with several crystalline defects, such as zinc (V) and oxygen (V) vacancies, Zn and O interstitials (Zn and O respectively), Zn and O antisite defects, and charged oxygen vacancies Vo-, among others, are generated by the introduction of cobalt (Co) into the structure. The effective introduction of Co into the Zn occupancy site was evaluated by XRD and electron paramagnetic resonance. The EPR spectra remain consistent across all doping concentrations of Co ions and revealed intriguing features linked to four distinct Co paramagnetic centers; among them, a pair of Co ions exhibited ferromagnetic coupling.
View Article and Find Full Text PDFMolecules
February 2025
Key Laboratory of Spin Electron and Nanomaterials of Anhui Higher Education Institutes, School of Mechanical and Electronic Engineering, Suzhou University, Suzhou 234000, China.
Sodium-ion batteries (SIBs) are a promising electrochemical energy storage system but face great challenges in developing fast-charging anodes. MXene-based composites are a new class of two-dimensional materials that are expected to be widely used in SIB energy storage due to their excellent electrical conductivity and stable structure. However, MXenes tend to experience interlayer stacking during preparation, which can result in poor electrochemical performance and a lower actual capacity compared to the theoretical value.
View Article and Find Full Text PDFJ Chem Theory Comput
March 2025
Department of Chemistry, Chicago Center for Theoretical Chemistry, University of Chicago, Chicago, Illinois 60637, United States.
Single-molecule magnets (SMMs) are promising candidates for molecular-scale data storage and processing due to their strong magnetic anisotropy and long spin relaxation times. However, as the temperature rises, interactions between electronic states and lattice vibrations accelerate spin relaxation, significantly limiting their practical applications. Recently, ab initio simulations have made it possible to advance our understanding of phonon-induced magnetic relaxation, but significant deviations from the experiments have often been observed.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!
© LitMetric 2025. All rights reserved.