Membrane-based gas separation provides an energy-efficient approach for the simultaneous CO and HS removal from sour natural gas. The fluorinated polyimide (PI) membranes exhibited a promising balance between permeability and permselectivity for sour natural gas separation. To further improve the separation efficiency of fluorinated PI membranes, a melamine-copolymerization synthetic approach is devised that aims to incorporate melamine motifs with high sour gas affinity into the structure of the PI membranes. The fluorinated copolyimide membranes that are structurally engineered exhibited excellent solution-processability and enhanced sweet-mixed gas selectivity compared to their original PI membranes. Additionally, under a five-component sour mixed-gas feed, these melamine-copolymerized fluorinated PI membranes provided superior combined HS and CO removal efficiency in comparison to conventional glassy polymer membranes. The melamine-copolymerization strategy provides an easily operable and generally effective approach to developing performance-enhancing PI membranes for sour natural gas separation.
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http://dx.doi.org/10.1002/advs.202416109 | DOI Listing |
Adv Sci (Weinh)
January 2025
Aramco Americas, Boston Research Center, Cambridge, MA, 02139, USA.
Membrane-based gas separation provides an energy-efficient approach for the simultaneous CO and HS removal from sour natural gas. The fluorinated polyimide (PI) membranes exhibited a promising balance between permeability and permselectivity for sour natural gas separation. To further improve the separation efficiency of fluorinated PI membranes, a melamine-copolymerization synthetic approach is devised that aims to incorporate melamine motifs with high sour gas affinity into the structure of the PI membranes.
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January 2025
College of Food and Chemical Engineering, Shaoyang University, Shaoshui Road, Shaoyang 422000, China.
Endogenous peptides in Baijiu have primarily focused on finished liquor research, with limited attention given to the peptides in base liquor prior to blending. Liquid chromatography-tandem mass spectrometry (LC-MS) was employed to identify endogenous peptides in the distillates from the first to seventh rounds of soy sauce-flavored Baijiu. Two hundred and five oligopeptides were identified from these distillates, all of which had molecular weights below 1000 Da and were composed of amino acid residues associated with flavor (sweet, sour, and bitter) and biological activity.
View Article and Find Full Text PDFPlant Cell Environ
January 2025
College of Horticulture, Hebei Agricultural University, Baoding, Hebei, China.
Jujube (Ziziphus ujuba Mill.) holds great importance as a fruit tree in China, with strong tolerance to drought and saline stress, but its growth is limited by vulnerability to cold stress. Consequently, the role of MAPK cascades in mediating jujube cold stress response remains unclear, with the specific function of ZjMAPKK4 in this context yet to be fully elucidated.
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December 2024
Smell & Taste Clinic, Department of Otorhinolaryngology, Technische Universität Dresden, 01307 Dresden, Germany.
The umami taste is well validated in Asian culture but remains less recognized and accepted in European cultures despite its presence in natural local products. This study explored the sensory and emotional perceptions of umami in 233 Austrian participants who had lived in Austria for most of their lives. Using blind tasting, participants evaluated monosodium glutamate (MSG) dissolved in water, providing open-ended verbal descriptions, pleasantness ratings, and comparisons to a sodium chloride (NaCl) solution.
View Article and Find Full Text PDFItal J Food Saf
November 2024
Plant Pathology and Postharvest Quality Laboratory, Regional Center for Agronomical Research of Kenitra, Morocco.
Biotic stress significantly challenges the global citrus industry. Major post-harvest issues include diseases caused by , and . The negative impact of chemical fungicides on the environment and health necessitates eco-friendly alternatives.
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