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| http://dx.doi.org/10.1021/acscentsci.4c02221 | DOI Listing |
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Quantum Thermodynamic Derivation of the Energy Resolution Limit in Magnetometry.
Phys Rev Lett
December 2024
University of Crete, Department of Physics, Heraklion 70013, Greece.
It was recently demonstrated that a multitude of realizations of several magnetic sensing technologies satisfy the energy resolution limit, which connects a quantity composed by the variance of the magnetic field estimate, the sensor volume and the measurement time, and having units of action, with ℏ. A first-principles derivation of this limit is still elusive. We here present such a derivation based on quantum thermodynamic arguments.
View Article and Find Full Text PDFMorphological Control of Y6 Thin Films Reveals Charge Transfer Is Facilitated by Co-facial Interactions.
J Phys Chem Lett
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School of Chemical and Physical Sciences, Victoria University of Wellington, Wellington 6012, New Zealand.
The organic semiconductor Y6 has been extensively used as an acceptor in organic photovoltaic devices, yielding high efficiencies. Its unique properties include a high refractive index, intrinsic exciton dissociation, and barrierless charge generation in bulk heterojunctions. However, the direct impact of the crystal packing morphology on the photophysics of Y6 has remained elusive, hindering further development of heterojunction and homojunction devices.
View Article and Find Full Text PDFEnzymes in a human cytoplasm model organize into submetabolon complexes.
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Department of Chemistry, University of Illinois Urbana-Champaign, Urbana, IL 61801.
Enzyme-enzyme interactions are fundamental to the function of cells. Their atomistic mechanisms remain elusive mainly due to limitations of in-cell measurements. We address this challenge by atomistically modeling, for a total of ≈80 μs, a slice of the human cell cytoplasm that includes three successive enzymes along the glycolytic pathway: glyceraldehyde-3-phosphate dehydrogenase (GAPDH), phosphoglycerate kinase (PGK), and phosphoglycerate mutase (PGM).
View Article and Find Full Text PDFMedialization of shaft of humerus to provide medial buttress and prevent varus collapse in 3- and 4-part proximal humerus fractures: review of the surgical technique.
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