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Additive Manufacturing (AM) was evaluated as a promising technology for constructing photocatalytic reactors due to its inherent ability to produce complex geometries with high precision and customization. In this work, a 3D structure was designed to achieve a good light distribution inside a cylindrical batch reactor and printed using the stereolithography (SLA) technique. A hybrid material composed of a commercial photoreactive resin (Formlabs Clear V4) and the benchmark photocatalyst TiO P25 Evonik (1 wt%) was prepared and characterized by scanning electron microscopy (SEM) and rheological and mechanical methods.

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Methane, the major component of natural and shale gas, is a significant carbon source for chemical synthesis. The direct partial oxidation of methane to liquid oxygenates under mild conditions is an attractive pathway, but the molecule's inertness makes it challenging to achieve simultaneously high conversion and high selectivity towards a single target product. This difficulty is amplified when aiming for more valuable products that require C-C coupling.

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Solar-based technologies for removing potentially toxic metals from water sources: a review.

Environ Sci Pollut Res Int

January 2025

Departamento de Ciência E Tecnologia de Alimentos, Universidade Federal de Santa Catarina, Rod. Admar Gonzaga, 1346, Itacorubi, Florianópolis, Santa Catarina, 88034-001, Brazil.

Technological advances have led to a proportional increase in the deposition of contaminants across various environmental compartments, including water sources. Heavy metals, also known as potentially toxic metals, are of particular concern due to their significant harmful impacts on environmental and human health. Among the available methods for mitigating the threat of these metals in water, solar radiation-based technologies stand out for their cleanliness, cost-effectiveness, and efficiency in removing or reducing the toxicity of heavy metals.

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Bioinspired Photo-Thermal Catalytic System Using Covalent Organic Framework-Based Aerogel for Synchronous Seawater Desalination and HO Production.

Angew Chem Int Ed Engl

January 2025

School of Materials Science and Engineering, National Institute for, Advanced Materials, TKL of Metal and Molecule-Based Material Chemistry, Nankai University, Tianjin, 300350, P. R. China.

Efficient utilization of solar energy is widely regarded as a crucial solution to addressing the energy crisis and reducing reliance on fossil fuels. Coupling photothermal and photochemical conversion can effectively improve solar energy utilization yet remains challenging. Here, inspired by the photosynthesis system in green plants, we report herein an artificial solar energy converter (ASEC) composed of light-harvesting units as solar collector and oriented ionic hydrophilic channels as reactors and transporters.

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Mechanism, Performance, and Application of g-CN-Coupled TiO as an S-Scheme Heterojunction Photocatalyst for the Abatement of Gaseous Benzene.

ACS Appl Mater Interfaces

January 2025

Department of Civil and Environmental Engineering, Hanyang University, 222 Wangsimni-ro, Seongdong-Gu, Seoul 04763, Republic of Korea.

In this research, S-scheme heterojunction photocatalysts are prepared through the hybridization of nitrogen-rich g-CN with TiO (coded as TCN-(): as the weight ratio of TiO:g-CN). The photocatalytic potential of TCN-() is evaluated against benzene (1-5 ppm) across varying humidity levels using a dynamic flow packed-bed photocatalytic reactor. Among the prepared composites, TCN-(10) exhibits the highest synergy between g-CN and TiO at "" ratio of 10%, showing superior best benzene degradation performance (e.

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