Metal-halide perovskite nanowire array photodetectors based on the solution method are valuable in the field of polarized light detection because of their unique one-dimensional array structure and excellent photoelectric performance. However, the limited wettability of liquids poses challenges for achieving large-scale and high-quality perovskite nanowire arrays. To address this issue, we develop a facile method utilizing capillary condensation to grow high-quality centimeter-scale perovskite nanowire arrays. Based on these nanowires, the fabricated photodetector showcases specific detectivities of 1.95 × 10 jones, surpassing commercially available silicon detectors in weak-light detection capabilities. The weak-light imaging capability of our nanowire photodetectors has been successfully demonstrated at intensities below 54 nW/cm. Moreover, the nanowire arrays also display excellent polarization absorption characteristics, promising applications in polarized light detection. Notably, the perovskite nanowire arrays can be grown on flexible substrates by employing capillary condensation, which retains 83% of their properties after 2000 bending cycles. This research enhances the potential of perovskite nanowire arrays photodetector in practical applications.
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http://dx.doi.org/10.1038/s41377-024-01680-2 | DOI Listing |
Light Sci Appl
January 2025
State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, International Center of Future Science, Jilin University, Changchun, 130012, China.
Metal-halide perovskite nanowire array photodetectors based on the solution method are valuable in the field of polarized light detection because of their unique one-dimensional array structure and excellent photoelectric performance. However, the limited wettability of liquids poses challenges for achieving large-scale and high-quality perovskite nanowire arrays. To address this issue, we develop a facile method utilizing capillary condensation to grow high-quality centimeter-scale perovskite nanowire arrays.
View Article and Find Full Text PDFACS Omega
December 2024
Synchrotron Radiation Research and NanoLund, Department of Physics, Lund University, Box 124, Lund 22100, Sweden.
Metal halide perovskite nanowires are widely studied due to their unique electronic and optical characteristics, making them promising for light emitting and detection applications. We developed a ligand-free method to grow vertically aligned free-standing CsPbBr nanowires from anodized aluminum oxide nanopore substrates. Here, we investigate the growth process using microscopy with ultraviolet and visible light excitation, revealing a highly dynamic process with pronounced fluorescence at locations where high-density free-standing nanowires could be found.
View Article and Find Full Text PDFAdv Sci (Weinh)
December 2024
Zhejiang Lab, Hangzhou, 311121, China.
ACS Nano
December 2024
Division of Synchrotron Radiation Research, Department of Physics, Lund University, 221 00 Lund, Sweden.
Metal-halide perovskites (MHPs) have gained substantial interest in the energy and optoelectronics field. MHPs in nanostructure forms, such as nanocrystals and nanowires (NWs), have further expanded the horizons for perovskite nanodevices in geometry and properties. A partial anion exchange within the nanostructure, creating axial heterojunctions, has significantly augmented the potential applications.
View Article and Find Full Text PDFNanoscale
January 2025
Department of Chemistry, Ben-Gurion University of the Negev, Beer-Sheva, 8410501, Israel.
Halide perovskites (HPs), particularly at the nanoscale, attract attention due to their unique optical properties compared to other semiconductors. They exhibit bright emission, defect tolerance, and a broad tunable band gap. The ability to directly transport charge carriers along the HPs nanowires (NWs) has led to the development of methods for their synthesis.
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