The surge of flexible, biointegrated electronics has inspired continued research efforts in designing and developing chip-less and wireless devices as soft and mechanically compliant interfaces to the living systems. In recent years, innovations in materials, devices, and systems have been reported to address challenges surrounding this topic to empower their reliable operation for monitoring physiological signals. This perspective provides a brief overview of recent works reporting various chip-less electronics for sensing and actuation in diverse application scenarios. We summarize wireless signal/data/power transmission strategies, key considerations in materials design and selection, as well as successful demonstrations of sensors and actuators in wearable and implantable forms. The final section provides an outlook to the future direction down the road for performance improvement and optimization. These versatile, inexpensive, and low-power device concepts can serve as alternative strategies to existing digital wireless electronics, which will find broad applications as bidirectional biointerfaces in basic biomedical research and clinical practices.
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http://dx.doi.org/10.1021/acsmaterialsau.4c00106 | DOI Listing |
ACS Appl Mater Interfaces
January 2025
State Key Laboratory of New Textile Materials and Advanced Processing Technologies, College of Textile Science and Engineering, Wuhan Textile University, Wuhan 430200, P. R. China.
Carbon fiber (CF) has been widely used in aerospace, military, infrastructure, sports, and leisure fields owing to its excellent mechanical properties, superior corrosion and friction resistances, excellent thermal stability, and lightweight. However, the ultrablack appearance derived from the extremely strong absorption of light throughout the entire visible region makes it difficult to satisfy the aesthetic and pleasurable demands of the colorful world and limits their applications in a broader field. Herein, inspired by the , a double-layer ultrathin AlO/TiO composite structure was fabricated on CFs by the atomic layer deposition method.
View Article and Find Full Text PDFSci Bull (Beijing)
December 2024
State Key Laboratory of Advanced Fiber Materials, Institute of Functional Materials, College of Materials Science and Engineering, Research Base of Textile Materials for Flexible Electronics and Biomedical Applications (China Textile Engineering Society), Shanghai Engineering Research Center of Nano-Biomaterials and Regenerative Medicine, Shanghai Key Laboratory of Lightweight Composite, Donghua University, Shanghai 201620, China. Electronic address:
It remains a challenge for a simple and scalable method to fabricate ultrathin porous Janus membranes for stretchable on-skin electronics. Here, we propose a one-step droplet spreading phase separation strategy to prepare an ultrathin and easily collected Janus thermoplastic polyurethane (TPU) membrane within seconds. The metal-ion solvation structure mitigated migration kinetics to delay TPU solution demixing, promoting the further penetration of the coagulating solvent.
View Article and Find Full Text PDFACS Mater Au
January 2025
Department of Materials Science and Engineering, The Ohio State University, Columbus, Ohio 43210, United States.
The surge of flexible, biointegrated electronics has inspired continued research efforts in designing and developing chip-less and wireless devices as soft and mechanically compliant interfaces to the living systems. In recent years, innovations in materials, devices, and systems have been reported to address challenges surrounding this topic to empower their reliable operation for monitoring physiological signals. This perspective provides a brief overview of recent works reporting various chip-less electronics for sensing and actuation in diverse application scenarios.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
Institute of Chemical Engineering Sciences, Foundation of Research and Technology- Hellas (FORTH/ICE-HT), Stadiou Street, Platani, Patras 26504, Greece.
Due to their outstanding electrical and thermal properties, graphene and related materials have been proposed as ideal candidates for the development of lightweight systems for thermoelectric applications. Recently, the nanolaminate architecture that entails alternation of continuous graphene monolayers and ultrathin polymer films has been proposed as an efficient route for the development of composites with impressive physicochemical properties. In this work, we present a novel layer-by-layer approach for the fabrication of highly ordered, flexible, heat-resistant, and electrically conductive freestanding graphene/polymer nanolaminates through alternating Marangoni-driven self-assembly of reduced graphene oxide (rGO) and poly(ether imide) (PEI) films.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2024
Department of Chemical Engineering, National Taiwan University, Taipei 10617, Taiwan.
The research on photonic synapses holds immense promise for various applications, such as robotics and artificial intelligence. Pursuing lightweight, miniaturized, and low-energy consumption designs is crucial for enhancing efficiency and adaptability in evolving technological environments. To achieve this goal, this work designs a series of conjugated self-assembled molecules with photoactive pyrene, benzo-naphthol-thiophene (BNT), perylene, and benzothieno-benzothiophene cores to develop ultrathin (<3 nm) charge-trapping self-assembled monolayers (SAMs).
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