Effects of stir-frying on chemical profile, sensory quality and antioxidant activity of Chrysanthemi Flos: A metabolomics and sensory study.

Chrysanthemi Flos has been consumed as floral tea for centuries, but the effects of stir-frying on its chemical profile, sensory characteristics, and bioactivity remain unclear. This study used untargeted metabolomics, sensory assessment (E-eye, E-nose, E-tongue), and antioxidant activity evaluation to investigate compositional changes and their effects. In the metabolomics analysis, a total of 101 non-volatile and 306 volatile differential metabolites were identified. During stir-frying of Chrysanthemi Flos, glycosidic bond rupture in flavonoid glycosides, thermal decomposition of caffeoylquinic acid, Maillard, and caramelization reactions occurred. This led to the formation of 4 flavonoid glycosides (luteolin, diosmetin, apigenin, and quercetin) and 33 roasted aroma compounds like pyrazines, furans, 2-methylbutanal, and 2-furanmethanol. The Spearson's correlation analysis of metabolomics, E-eye, and E-tongue data showed that these compositional changes not only resulted in darkening and scorching of the color of Chrysanthemi Flos after stir-frying, but also improved the bitter and astringent taste of Chrysanthemi Flos tea broths, and enhanced the antioxidant activity of Chrysanthemi Flos. These findings will provide new perspectives on the selection of processing methods for Chrysanthemi Flos.