We investigate the thermoelectric response of an Abrikosov vortex in type-II superconductors in the deep quantum limit. We consider two thermoelectric geometries, a type-II superconductor-insulator-normal-metal (S-I-N) junction and a local scanning tunneling microscope (STM)-tip normal metal probe over the superconductor. We exploit the strong breaking of particle-hole symmetry in vortex-bound states at subgap energies within the superconducting vortex to realize a giant thermoelectric response in the presence of fluxons. We predict a thermovoltage of a few mV/K at subkelvin temperatures using both semianalytic and numerical self-consistent solutions of the Bogoliubov-de Gennes equations. Relevant thermoelectric coefficients and figures of merit ZT are found within our models, both in linear and nonlinear regimes. ZT of the S-I-N junction is around 1, rising to above 3 for the STM junction centered at the vortex core. We also discuss how this system can be used as a sensitive low-temperature thermocouple, or a localized bolometer to detect low-energy single photons.
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http://dx.doi.org/10.1103/PhysRevLett.133.256002 | DOI Listing |
Nat Mater
January 2025
Max Planck Institute for Chemical Physics of Solids, Dresden, Germany.
High thermoelectric performance is generally achieved by synergistically optimizing two or even three of the contradictorily coupled thermoelectric parameters. Here we demonstrate magneto-thermoelectric correlation as a strategy to achieve simultaneous gain in an enhanced Seebeck coefficient and reduced thermal conductivity in topological materials. We report a large magneto-Seebeck effect and high magneto-thermoelectric figure of merit of 1.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Department of Physics and Astronomy, University of Rochester, Rochester, New York 14627, USA.
ACS Appl Mater Interfaces
December 2024
Institute of Chemical Engineering Sciences, Foundation of Research and Technology- Hellas (FORTH/ICE-HT), Stadiou Street, Platani, Patras 26504, Greece.
Due to their outstanding electrical and thermal properties, graphene and related materials have been proposed as ideal candidates for the development of lightweight systems for thermoelectric applications. Recently, the nanolaminate architecture that entails alternation of continuous graphene monolayers and ultrathin polymer films has been proposed as an efficient route for the development of composites with impressive physicochemical properties. In this work, we present a novel layer-by-layer approach for the fabrication of highly ordered, flexible, heat-resistant, and electrically conductive freestanding graphene/polymer nanolaminates through alternating Marangoni-driven self-assembly of reduced graphene oxide (rGO) and poly(ether imide) (PEI) films.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2024
School of Science, and Ministry of Industry and Information Technology Key Lab of Micro-Nano Optoelectronic Information System, Harbin Institute of Technology, Shenzhen 518055, China.
As semiconductor technology advances toward miniaturization and portability, thin films with excellent thermoelectric performance have garnered increasing attention, particularly for applications in self-powered devices and temperature-responsive sensors. The high Seebeck coefficient of SnSe thin films makes them promising for temperature sensing, but their poor electrical conductivity limits their potential as thermoelectric generators. In this work, high-quality -axis oriented SnSe thin films were deposited on quartz substrates by using magnetron sputtering.
View Article and Find Full Text PDFACS Nano
December 2024
Sauvage Laboratory for Smart Materials, School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen), Shenzhen 518055, China.
Featuring the capabilities of self-power, low dark current, and broadband response, photothermoelectric (PTE) detection demonstrates great potential for application in the military and civilian fields. The development of materials with an intrinsically high efficiency for PTE energy conversion and the in-depth study of its thermoelectric properties on the device performance are of great significance. Here, we reported a quasi-one-dimensional (quasi-1D) van der Waals (vdW) TaSe crystal as a promising material candidate for PTE detection.
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