Polydopamine-functionalized capsules: From design to applications.

In recent years, polydopamine (PDA)-functionalized capsules have garnered significant interest from researchers in the field of materials, owing to its remarkable properties of adhesion, biocompatibility, photothermal conversion capabilities, chemical reactivity, and so on. At present, numerous studies have reported various structures and morphologies of PDA-functionalized capsules fabricated via diverse strategies, that have found applications across a broad spectrum of disciplines. However, there are few comprehensive and systematic reviews focusing on various preparation strategies of PDA-functionalized capsules with various structures. This paper systematically reviewed the preparation strategies and related applications of PDA-functionalized capsules. These strategies of PDA-functionalized capsules were discussed in detail from four parts including PDA-functionalized capsules based on hollow PDA, mesoporous PDA (MPDA), directly encapsulating emulsion, and surface modification of capsules. Then the review outlined the applications of PDA-functionalized capsules in biomedicine, energy, textiles, and the environment. Furthermore, this review summarized the current research findings on PDA-functionalized capsules and outlines their future development directions. Overall, we aim for this review to inspire researchers and offer valuable guidance for the synthesis and application of advanced PDA-functionalized capsules.