Magnetic structure plays a pivotal role in the functionality of antiferromagnets (AFMs), which not only can be employed to encode digital data but also yields novel phenomena. Despite its growing significance, visualizing the antiferromagnetic domain structure remains a challenge, particularly for non-collinear AFMs. Currently, the observation of magnetic domains in non-collinear antiferromagnetic materials is feasible only in MnSn, underscoring the limitations of existing techniques that necessitate distinct methods for in-plane and out-of-plane magnetic domain imaging. In this study, we present a versatile method for imaging the antiferromagnetic domain structure in a series of non-collinear antiferromagnetic materials by utilizing the anomalous Ettingshausen effect (AEE), which resolves both the magnetic octupole moments parallel and perpendicular to the sample surface. Temperature modulation due to AEE originating from different magnetic domains is measured by lock-in thermography, revealing distinct behaviors of octupole domains in different antiferromagnets. This work delivers an efficient technique for the visualization of magnetic domains in non-collinear AFMs, which enables comprehensive study of the magnetization process at the microscopic level and paves the way for potential advancements in applications.
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http://dx.doi.org/10.1093/nsr/nwad308 | DOI Listing |
Natl Sci Rev
June 2024
International Center for Quantum Design of Functional Materials (ICQD), School of Emerging Technology, University of Science and Technology of China, Hefei 230026, China.
Nanoscale Horiz
September 2024
Department of Materials Science and Engineering, Monash University, Clayton, Victoria 3800, Australia.
Nat Commun
August 2024
Laboratoire de Physique et d'Etude de Matériaux (CNRS), ESPCI Paris, PSL Research University, 75005, Paris, France.
Nature
August 2024
Department of Physics and Center for Complex Quantum Systems, The University of Texas at Austin, Austin, TX, USA.
Helical spin structures are expressions of magnetically induced chirality, entangling the dipolar and magnetic orders in materials. The recent discovery of helical van der Waals multiferroics down to the ultrathin limit raises prospects of large chiral magnetoelectric correlations in two dimensions. However, the exact nature and magnitude of these couplings have remained unknown so far.
View Article and Find Full Text PDFAdv Mater
June 2024
Paul Scherrer Institut, Villigen PSI, 5232, Switzerland.
Understanding the magnetic and ferroelectric ordering of magnetoelectric multiferroic materials at the nanoscale necessitates a versatile imaging method with high spatial resolution. Here, soft X-ray ptychography is employed to simultaneously image the ferroelectric and antiferromagnetic domains in an 80 nm thin freestanding film of the room-temperature multiferroic BiFeO (BFO). The antiferromagnetic spin cycloid of period 64 nm is resolved by reconstructing the corresponding resonant elastic X-ray scattering in real space and visualized together with mosaic-like ferroelectric domains in a linear dichroic contrast image at the Fe L edge.
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