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The realization of higher coupling strengths between coupled resonant modes enables exploration of compelling phenomena in diverse fields of physics and chemistry. In this study, we focus on the modal coupling between localized surface plasmon resonance (LSPR) of Au nanoparticles (Au-NPs) and Fabry-Pérot mode (p-NiO/Au film). The effects of nanoparticle size, projected surface coverage (PSC), interparticle distance (IPD), and arrangement to the coupling strength between the two modes are theoretically investigated using finite-difference time-domain (FDTD) method. Au-NPs/p-NiO/Au film (ANA) nanostructures with NPs size of 10 nm, 30 nm, and 50 nm are considered. Numerical calculations point to larger size and higher projected surface coverage (also smaller IPD) of NPs as pre-eminent factors in enhancing the strength of modal coupling. ANA nanostructure with NPs size of 30 nm (ANA-30) and 50 nm (ANA-50) are experimentally fabricated via a facile air-liquid interface self-assembly. The fabricated nanodevices exhibit immense Rabi splitting energies of 655 meV (ANA-30) and 770 meV (ANA-50), and thus fulfill the ultrastrong coupling condition with remarkable splitting energy to bare (plasmon) energy ratio of 0.35 (ANA-30) and 0.4 (ANA-50). The physical insights presented in this study, together with the simple and scalable fabrication process, establish a viable approach to realize stronger coupling between LSPR and Fabry-Pérot mode in metal NPs/dielectric/metal film systems. This will be vital to take advantage of the promising performance enhancements of plasmonic-based nanostructures under strongly coupled regimes in areas such as solar to fuel conversion, sensing, opto-electronics, and quantum applications.
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http://www.ncbi.nlm.nih.gov/pmc/articles/PMC11636521 | PMC |
http://dx.doi.org/10.1515/nanoph-2023-0763 | DOI Listing |
Hum Brain Mapp
December 2024
Research Group Cognition and Plasticity, Max Planck Institute for Human Cognitive and Brain Sciences, Leipzig, Germany.
The ability to integrate semantic information into the context of a sentence is essential for human communication. Several studies have shown that the predictability of a final keyword based on the sentence context influences semantic integration on the behavioral, neurophysiological, and neural level. However, the architecture of the underlying network interactions for semantic integration across the lifespan remains unclear.
View Article and Find Full Text PDFHuman mesenchymal stromal cells (MSCs) are attractive for both medical practice and biomedical research. Nonfreezing short-term storage may provide safe and simple transportation and promote the practical use of MSCs. We aimed to determine the duration of efficient storage at ambient temperature (22°C) of human dermal MSCs in different three-dimensional organization and to investigate the role of cell metabolic mode in the resistance to the ambient storage damaging factors.
View Article and Find Full Text PDFObservational studies and clinical trials indicate a link between arterial stiffness (AS) and sarcopenia (SAR), yet the causal relationship between these remains unclear. The study aims to investigate the causal connection from AS to SAR by Mendelian randomization (MR). We analyzed Genome-Wide Association Studies data for AS indicators: pulse wave arterial stiffness index (PWASI) and pulse wave peak-to-peak time (PPT), and SAR indicators: low hand grip strength (LHGS), usual walking pace (UWP), moderate-to-vigorous physical activity levels (MVPA), and walk or cycle unassisted for 10 minutes.
View Article and Find Full Text PDFFront Neurosci
December 2024
Basic Medical School, Guizhou University of Traditional Chinese Medicine, Guiyang, Guizhou, China.
Background: Neuropathic pain (NeP) presents considerable challenges in terms of effective management and significantly impacts the quality of life for affected patients. The current treatment options for NeP are limited, highlighting the need for alternative therapeutic approaches. Dahuang Fuzi Decoction (DF), a formula from traditional Chinese medicine, has shown potential in relieving pain symptoms associated with various types of NeP.
View Article and Find Full Text PDFFront Psychol
December 2024
Department of Humanities and Social Sciences, Mid Sweden University, Östersund, Sweden.
Introduction: Sport and outdoor activities have benefits on people's health and well-being but may also increase the frequency of unsustainable behaviors. The present study explores drivers of travel mode choice and consumption of material (clothes and equipment) associated with physical activity to clarify the extent to which an active and sustainable lifestyle is compatible. The role of identity and varying levels of internalized motivation for pro-environmental behaviors (autonomous and controlled environmental motivation) and engagement in physical activity (autonomous and controlled activity motivation) was examined.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!