In the presence of a magnetic field, a liquid crystal (LC) director can be distorted from a ground state set by a combination of LC elasticity and surface anchoring at any relevant interfaces. Uniform magnetic fields are often used to produce simple LC distortions on demand, but producing more spatially complex distortions is practically challenging. We develop a strategy for the spatially resolved control of the LC director by leveraging field patterns induced by ferromagnetic materials. Patterned magnetic fields are generated from high-permeability ferromagnetic microstructures embedded into nematic liquid crystals (NLCs) to manipulate the LC director's orientation. Each ferromagnetic microstructure produces a unique spatially varying magnetic field. In turn, tuning magnetic field strength in competition with NLC elasticity can pattern a range of spatially complex director configurations. Simulations relate the spatial variation induced in a magnetic field by a ferromagnetic geometry and the resultant director. Our predictive models can inform the inverse design of ferromagnetic microstructures to generate bespoke director patterns. We also link changes in the magnetic field to the migration of elastically driven periodic extinctions in birefringence near the edges of ferromagnetic structures.
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http://dx.doi.org/10.1021/acsami.4c17546 | DOI Listing |
Adv Mater
January 2025
School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, 200240, China.
Van der Waals (vdWs) materials are promising candidates for hetero-integration with silicon photonics toward miniaturization and integration. VdWs materials like molybdenum telluride and black phosphorus, despite being prominent, exhibit air sensitivity, and their room temperature emissions can be significantly broadened by tens of meV. Here, a self-encapsulation strategy is developed to scalably synthesize robust 2D vdWs ErOCl with sub-meV narrow emissions at the telecom C-band.
View Article and Find Full Text PDFAdv Mater
January 2025
State Key Laboratory for Manufacturing Systems Engineering, Electronic Materials Research Laboratory, Key Laboratory of the Ministry of Education, School of Electronic Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, China.
Large low-field magnetoresistance (LFMR, < 1 T), related to the spin-disorder scattering or spin-polarized tunneling at boundaries of polycrystalline manganates, holds considerable promise for the development of low-power and ultrafast magnetic devices. However, achieving significant LFMR typically necessitates extremely low temperatures due to diminishing spin polarization as temperature rises. To address this challenge, one strategy involves incorporating Ruddlesden-Popper structures (ABO):AO, which are layered derivatives of perovskite structure capable of potentially inducing heightened magnetic fluctuations at higher temperatures.
View Article and Find Full Text PDFSmall
January 2025
School of Energy Science and Engineering, Indian Institute of Technology Kharagpur, Kharagpur, 721302, India.
Inducing magnetic ordering in a non-ferrous layered double hydroxides (LDHs) instigates higher spin polarization, which leads to enhanced efficiency during oxygen evolution reaction (OER). In nano-sized magnetic materials, the concept of elongated grains drives domain alignment under the application of an external magnetic field. Hence, near the solid electrode interface, modified magnetohydrodynamics (MHD) positively impacts the electrocatalytic ability of non-ferrous nanocatalysts.
View Article and Find Full Text PDFAdv Mater
January 2025
Department of Applied Physics, University of Tokyo, Bunkyo-ku, Tokyo, 113-8656, Japan.
Antiferromagnets with broken time-reversal ( ) symmetry ( -odd antiferromagnets) have gained extensive attention, mainly due to their ferromagnet-like behavior despite the absence of net magnetization. However, certain types of -odd antiferromagnets remain inaccessible by the typical ferromagnet-like phenomena (e.g.
View Article and Find Full Text PDFPhys Rev B
January 2018
Quantum Electromagnetics Division, National Institute of Standards and Technology, Boulder, CO 80305, U.S.A.
Understanding the evolution of spin-orbit torque (SOT) with increasing heavy-metal thickness in ferromagnet/normal metal (FM/NM) bilayers is critical for the development of magnetic memory based on SOT. However, several experiments have revealed an apparent discrepancy between damping enhancement and damping-like SOT regarding their dependence on NM thickness. Here, using linewidth and phase-resolved amplitude analysis of vector network analyzer ferromagnetic resonance (VNA-FMR) measurements, we simultaneously extract damping enhancement and both field-like and damping-like inverse SOT in NiFe/Pt bilayers as a function of Pt thickness.
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