Transverse thermoelectric conversion holds significant potential in addressing complex challenges faced by classical Seebeck/Peltier modules. A promising transverse thermoelectric phenomenon is the anomalous Nernst effect originating from nontrivial band structures in magnetic topological materials. However, the currently reported performance of the anomalous Nernst effect in topological materials, e.g., CoMnGa, remains insufficient for practical thermoelectric applications. Here, we unveil an unconventional availability of the anomalous Nernst effect by integrating magnetic topological materials into artificially tilted multilayers, known to exhibit the structure-induced transverse thermoelectric conversion due to the off-diagonal Seebeck effect. Our experiments reveal that the transverse thermoelectric performance in CoMnGa-based artificially tilted multilayers is improved through the hybrid action of the anomalous Nernst and off-diagonal Seebeck effects, with the magnetization-dependent performance modulation being one order of magnitude greater than the performance achievable with the anomalous Nernst effect alone. This synergy underscores the importance of hybrid transverse thermoelectric conversion and paves a way for advancing thermoelectric applications using magnetic materials.
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http://dx.doi.org/10.1038/s41467-024-53723-2 | DOI Listing |
Nanoscale Horiz
December 2024
Electrical and Computer Engineering, The Grainger College of Engineering, University of Illinois Urbana-Champaign, Urbana, USA.
Antiferromagnetic materials have several unique properties, such as a vanishingly small net magnetization, which generates weak dipolar fields and makes them robust against perturbation from external magnetic fields and rapid magnetization dynamics, as dictated by the geometric mean of their exchange and anisotropy energies. However, experimental and theoretical techniques to detect and manipulate the antiferromagnetic order in a fully electrical manner must be developed to enable advanced spintronic devices with antiferromagnets as their active spin-dependent elements. Among the various antiferromagnetic materials, conducting antiferromagnets offer high electrical and thermal conductivities and strong electron-spin-phonon interactions.
View Article and Find Full Text PDFAdv Sci (Weinh)
November 2024
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing, 100190, China.
The large anomalous Nernst effect in magnetic Weyl semimetals is one of the most intriguing transport phenomena, which draws significant attention for its potential applications in topological thermoelectrics. Despite frequent reports of substantial anomalous Nernst conductivity (ANC), methods to optimize Nernst thermoelectrics remain limited. The research reveals that the magnitude of the ANC is directly related to the sum of the anomalous Nernst and Hall angles.
View Article and Find Full Text PDFNat Commun
November 2024
National Institute for Materials Science, Tsukuba, 305-0047, Japan.
Transverse thermoelectric conversion holds significant potential in addressing complex challenges faced by classical Seebeck/Peltier modules. A promising transverse thermoelectric phenomenon is the anomalous Nernst effect originating from nontrivial band structures in magnetic topological materials. However, the currently reported performance of the anomalous Nernst effect in topological materials, e.
View Article and Find Full Text PDFJ Phys Condens Matter
November 2024
Institut für Physik, Martin-Luther Universität Halle-Wittenberg, D-06099 Halle, Germany.
Monolayer jacutingaite (PtHgSe) exhibits remarkable properties, including significant spin-orbit coupling (SOC) and a tunable band gap, attributed to its buckled honeycomb geometry and the presence of heavy atoms. In this study, we explore the spin- and valley-dependent anomalous Nernst effect (ANE) in jacutingaite under the influence of a vertical electric field, off-resonance circularly polarized light (OCPL), and an antiferromagnetic exchange field. Our findings, within the low-energy approximation, reveal the emergence of a perfectly spin-polarized ANE with the application of appropriate OCPL and a perfectly valley-polarized ANE under an antiferromagnetic exchange field.
View Article and Find Full Text PDFACS Nano
November 2024
Max Planck Institute of Microstructure Physics, Weinberg 2, Halle 06120, Germany.
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