Cometary comae are a mixture of gas and ice-covered dust. Processing on the surface and in the coma change the composition of ice on dust grains relative to that of the nucleus. As the ice on dust grains sublimates, the local coma composition changes. Rosetta observations of 67P/Churyumov-Gerasimenko previously reported one of the highest D/H values for a comet. However, reanalysis of more than 4000 water isotope measurements over the full mission shows that dust markedly increases local D/H. The isotope ratio measured at a distance from the nucleus where the gas is well mixed is close to terrestrial, like that of other Jupiter family comets. This lower D/H has implications for understanding comet formation and the role of comets in delivering water to Earth.
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http://dx.doi.org/10.1126/sciadv.adp2191 | DOI Listing |
Sci Adv
January 2025
New Cornerstone Science Laboratory, State Key Laboratory of Extreme Photonics and Instrumentation, College of Optical Science and Engineering, Zhejiang University, Hangzhou 310027, China.
Small organic molecules are essential building blocks of our universe, from cosmic dust to planetary surfaces to life. Compared to their well-known gaseous and liquid forms that have been extensively studied, small organic molecules in the form of ice at low temperatures receive much less attention. Here, we show that supercooled small-molecule droplets can be drawn into highly uniform amorphous ice microfibers with lengths up to 5 cm and diameters down to 200 nm.
View Article and Find Full Text PDFEnviron Sci Technol
January 2025
Xi'an AMS Center, State Key Laboratory of Loess Science, Shaanxi Key Laboratory of Accelerator Mass Spectrometry Technology and Application, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, P. R. China.
There has been a sharp rise in the extent and scale of human activities since the mid-20th century, termed the "Great Acceleration", and nuclear activities are one of the defining technological processes for this period. Pu released by atmospheric nuclear weapons tests provides an ideal chronostratigraphic marker for labeling this change due to its global fallout feature, temporal mutation, and long half-lives. However, the accumulation dynamics of plutonium from atmospheric deposition to preservation in the sediment is still controversial.
View Article and Find Full Text PDFPhotochem Photobiol Sci
January 2025
Institute of Meteorology and Climate Research Atmospheric Trace Gases and Remote Sensing, Karlsruhe Institute of Technology, Karlsruhe, Germany.
For a given solar elevation, the levels of solar ultraviolet radiation at the Earth's surface are determined by the amounts of ozone, aerosols, and clouds, as well as by the reflectivity of the surface. Here, we study the evolution of these factors for three selected decades in the period 1950-2100 using results from simulations with Earth-System models (ESMs) participating in the 6 phase of the Coupled Model Intercomparison Project (CMIP6). The simulations for the future are based on three Shared Socioeconomic Pathways: SSP1-2.
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
December 2024
Amrita School for Sustainable Futures, Amrita Vishwa Vidyapeetham, Amritapuri, 690525, Kerala, India.
The 'Third Pole', home to numerous glaciers, serves as vital water reserves for a significant portion of the Asian population and has garnered global attention within the context of climate change due to their highly vulnerable nature. While a general decline in global glacial extent has been observed in recent decades, the pronounced regional imbalances across the Third Pole present a perplexing anomaly. To assess the impact of glacier mass changes in the Gangotri basin, we conducted a comprehensive analysis using remote sensing data to estimate spatially resolved mass changes from 2000 to 2023.
View Article and Find Full Text PDFEnviron Sci Technol
January 2025
Climate and Environmental Physics, Physics Institute, and Oeschger Centre for Climate Change Research, University of Bern, Sidlerstrasse 5, Bern 3012, Switzerland.
This study presents the integration of the single-particle extinction and scattering (SPES) method in a continuous flow analysis (CFA) setup. Continuous measurements with the instrument allow for the characterization of water-insoluble particles in ice cores at high resolution with a minimized risk of contamination. The SPES method can be used to investigate particles smaller than 1 μm, which previously could not be detected by instruments typically used in CFA.
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