High-Performance Gate-Voltage-Tunable Photodiodes Based on NbPdSe/WSe Mixed-Dimensional Heterojunctions.

ACS Appl Mater Interfaces

Key Laboratory of Materials Physics, Anhui Key Laboratory of Nanomaterials and Nanotechnology, Institute of Solid State Physics, Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei 230031, China.

Published: November 2024

AI Article Synopsis

  • The development of a mixed-dimensional van der Waals heterojunction using 1D NbPdSe nanowires and 2D WSe nanosheets shows promise for advanced photodetectors due to its unique photoelectric properties and compatibility.
  • By adjusting the Fermi level with gate voltage, the heterojunction achieves tunable rectification characteristics, enhancing its performance.
  • Under 685 nm laser light, it exhibits impressive self-powered photodetection with a photoresponsivity of 1.45 A/W, a detectivity of 6.8 × 10^9 Jones, and a rapid response time, along with the capability to detect wavelengths from 255 to 1064 nm.

Article Abstract

The mixed-dimensional (MD) van der Waals (vdWs) heterojunction for photodetectors has garnered significant attention owing to its exceptional compatibility and superior quality. Low-dimensional material heterojunctions exhibit unique photoelectric properties attributed to their nanoscale thickness and vdWs contact surfaces. In this work, a novel MD vdWs heterojunction composed of one-dimensional (1D) NbPdSe nanowires and two-dimensional (2D) WSe nanosheets is proposed. The heterojunction's energy band engineering is accomplished by manipulating the Fermi level of the bipolar 2D material via gate voltage, resulting in a rectification characteristic that can be adjusted with gate voltage. Under 685 nm laser irradiation, it demonstrates exceptional self-powered photodetection performance, attaining a photoresponsivity of 1.45 A W, an ultrahigh detectivity of 6.8 × 10 Jones, and an ultrafast response time of 37/64 μs at zero bias. In addition, a broadband photodetector from 255 to 1064 nm is realized. These results demonstrate the great potential of NbPdSe/WSe MD heterostructures for advanced electronic and optoelectronic devices.

Download full-text PDF

Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC11583975PMC
http://dx.doi.org/10.1021/acsami.4c09682DOI Listing

Publication Analysis

Top Keywords

vdws heterojunction
8
gate voltage
8
high-performance gate-voltage-tunable
4
gate-voltage-tunable photodiodes
4
photodiodes based
4
based nbpdse/wse
4
nbpdse/wse mixed-dimensional
4
mixed-dimensional heterojunctions
4
heterojunctions mixed-dimensional
4
mixed-dimensional van
4

Similar Publications

Broadband detection technology is crucial in the fields of astronomy and environmental surveying. Two dimensional (2D) materials have emerged as promising candidates for next-generation broadband photodetectors with the characteristics of high integration, multi-dimensional sensing, and low power consumption. Among these, 2D tellurium (Te) is particularly noteworthy due to its excellent mobility, tunable bandgap, and air stability.

View Article and Find Full Text PDF

High-Performance Gate-Voltage-Tunable Photodiodes Based on NbPdSe/WSe Mixed-Dimensional Heterojunctions.

ACS Appl Mater Interfaces

November 2024

Key Laboratory of Materials Physics, Anhui Key Laboratory of Nanomaterials and Nanotechnology, Institute of Solid State Physics, Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei 230031, China.

Article Synopsis
  • The development of a mixed-dimensional van der Waals heterojunction using 1D NbPdSe nanowires and 2D WSe nanosheets shows promise for advanced photodetectors due to its unique photoelectric properties and compatibility.
  • By adjusting the Fermi level with gate voltage, the heterojunction achieves tunable rectification characteristics, enhancing its performance.
  • Under 685 nm laser light, it exhibits impressive self-powered photodetection with a photoresponsivity of 1.45 A/W, a detectivity of 6.8 × 10^9 Jones, and a rapid response time, along with the capability to detect wavelengths from 255 to 1064 nm.
View Article and Find Full Text PDF

van der Waals (vdW) heterostructures constructed by low-dimensional (0D, 1D, and 2D) materials are emerging as one of the most appealing systems in next-generation flexible photodetection. Currently, hand-stacked vdW-type photodetectors are not compatible with large-area-array fabrication and show unimpressive performance in self-powered mode. Herein, vertical 1D GaN nanorods arrays (NRAs)/2D MoS/PEDOT:PSS in wafer scale have been proposed for self-powered flexible photodetectors arrays firstly.

View Article and Find Full Text PDF

One-dimensional van der Waals (vdWs) heterostructures are celebrated for their exceptional thermal management capabilities, garnering significant research interest. Consequently, our research focused on the one-dimensional vdWs heterojunction comprising carbon nanotube half-wrapped in boron nitride nanotube (BNCNT), specifically their thermal rectification (TR) properties. We employed non-equilibrium molecular dynamics to explore the TR mechanism and assess the impacts of temperature, strain, and coupling strength on heat flux and TR ratio.

View Article and Find Full Text PDF

High-Spike Barrier Photodiodes Based on 2D Te/WS Heterostructures.

ACS Nano

July 2024

Academy for Advanced Interdisciplinary Science and Technology, Key Laboratory of Advanced Materials and Devices for Post-Moore Chips Ministry of Education, State Key Laboratory for Advanced Metals and Materials, University of Science and Technology Beijing, Beijing 100083, P. R. China.

Article Synopsis
  • Two-dimensional van der Waals heterojunctions are being researched for their potential in fast and low-power photodiodes due to their smooth interfaces and quick charge transfer.
  • The study introduces a high-spike barrier photodiode using Te/WS heterojunctions, which effectively reduces dark current while maintaining a fast response by manipulating band alignment.
  • The Te/WS photodiode achieves impressive performance metrics with an ultralow dark current of 8 × 10 A and a rapid photoresponse of 10/13 μs, while also demonstrating a visible-light imager with a pixel resolution of 100 × 40.
View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!