Sliding-Induced Rehydration in Hydrogels for Restoring Lubrication and Anticreeping Capability.

Fluid exudation in cartilage under normal loading can be counteracted by a sliding-induced rehydration phenomenon, which has a hydrodynamic origin related to a wedge effect at the contact inlet. Similar to cartilage, hydrogels also exhibit tribological rehydration properties, and we mimic this phenomenon to restore hydration lubrication and overcome creeping. It occurs within a specific velocity range and is mainly dependent on the applied load and hydrogel network structures. Crucially, a certain velocity in the mixed lubrication regime can produce a hydrodynamic pressure peak at the wedge and drive the rehydration inflow to overcome the extrusion. At lower sliding velocities in the boundary lubrication regime, inflows are insufficient to counteract fluid exudation, whereas at higher velocities in the hydrodynamic lubrication regime, the inlet wedge effect would diminish. These results suggest that tribological rehydration offers a novel approach to enhancing load-bearing capacity and maintaining lubrication in the hydrogels.