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Regulating Chlorine and Hydrogen Atom Transfer for Selective Photoelectrochemical C─C Coupling by Cu-coordination Effect at Semiconductor/Electrolyte Interfaces.
Adv Sci (Weinh)
December 2024
Key Laboratory of Photochemistry, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, P. R. China.
Semiconductor-based photoelectrochemical (PEC) organic transformations usually show radical characteristics, in which the reaction selectivity is often difficult to precisely control due to the nonselectivity of radicals. Accordingly, several simple organic reactions (e.g.
View Article and Find Full Text PDFZirconium-Coated β-Cyclodextrin Nanomaterials for Biofilm Eradication.
ACS Appl Bio Mater
December 2023
Department of Chemistry, Faculty of Exact Sciences, Bar-Ilan University, Ramat-Gan 5290002, Israel.
Under alkaline treatment, zirconyl chloride (ZrOCl.8HO) became a zirconia gel and formed a stable complex with beta-cyclodextrin (βCD). This complex was highly active in reactive oxygen species (ROS) formation via HO decomposition.
View Article and Find Full Text PDFImpact of Bicarbonate Interference on Routine Ion-Selective Electrode Chloride Measurements.
Ann Lab Med
September 2022
Department of Laboratory Medicine, AZ Groeninge Hospital, Kortrijk, Belgium.
Article Synopsis
- Chloride measurement is essential for determining the anion gap, yet bicarbonate can interfere with these measurements, leading to inaccuracies depending on the type of electrode used.
- Different electrodes showed varying levels of non-selectivity towards bicarbonate, with some becoming more biased over time while others gained selectivity.
- Adjusting calibrator bicarbonate concentrations significantly improved measurement accuracy, highlighting the need for laboratories to recognize and manage bicarbonate's impact on chloride assessments.
Electrochemical Oxidation of Monosaccharides at Nanoporous Gold with Controlled Atomic Surface Orientation and Non-Enzymatic Galactose Sensing.
Sensors (Basel)
October 2020
Bioproduction Research Institute, National Institute of Advanced Industrial Science and Technology (AIST), Sapporo 062-8517, Japan.
Non-enzymatic saccharide sensors are of great interest in diagnostics, but their non-selectivity limits their practical diagnostic abilities. In this study, we investigated the electrochemical oxidation of monosaccharides at nanoporous gold (NPG) catalysts with different contributions of surface crystallographic orientations. Fructose elicited no clear electrochemical response, but glucose, galactose, and mannose produced clear oxidative current.
View Article and Find Full Text PDFComparative study on degradation of propranolol and formation of oxidation products by UV/HO and UV/persulfate (PDS).
Water Res
February 2019
State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology, Harbin, 150090, China.
The frequent detection of propranolol, a widely used β-blocker, in wastewater effluents and surface waters has raised serious concern, due to its adverse effects on organisms. UV/hydrogen peroxide (UV/HO) and UV/persulfate (UV/PDS) processes are efficient in eliminating propranolol in various waters, but the formation of oxidation products in these processes, as well as the assessment of their toxicity, has not been systematically addressed. In this study, we identified and compared transformation products of propranolol produced by hydroxyl radical (OH) and sulfate radical (SO).
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