Quantum sensing is crucial for precision measurements, yet quantum sensor sensitivity is often limited by the coherence time of the quantum system. Here, we demonstrate a method to enhance coherence time through cooperative spins. Using a tunable feedback circuit, we induce cooperation among noble-gas ^{129}Xe spins, resulting in an impressive 18-fold coherence enhancement. Moreover, we show that the cooperative ^{129}Xe spins can significantly amplify magnetic signals by at least 3 orders of magnitude. Magnetic field sensing assisted with such a cooperative spin amplifier realizes the sensitivity of 4 fT/Hz^{1/2} and surpasses the spin-projection noise of the embedded ^{87}Rb spin gas magnetometer. These results pave the way for a new class of "cooperative quantum sensors," and open up exciting prospects in fundamental physics.
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http://dx.doi.org/10.1103/PhysRevLett.133.133202 | DOI Listing |
Materials (Basel)
January 2025
Laboratory for Heteroepitaxial Growth of Functional Materials & Devices, Department of Chemical & Biological Engineering, State University of New York (SUNY) at Buffalo, Buffalo, NY 14260, USA.
This study analyzes the calculation of the critical current density by means of Bean's critical state model, using the equation formulated by Gyorgy et al. and other similar equations derived from it reported in the literature. While estimations of using Bean's model are widely performed, improper use of different equations with different magnetic units and pre-factors leads to confusion and to significant errors in the reported values of .
View Article and Find Full Text PDFJ Chem Phys
January 2025
Université Paris-Saclay, UVSQ, CNRS, GEMaC, 45 Avenue des Etats Unis, 78035 Versailles, France.
Among the large family of spin-crossover (SCO) solids, recent investigations focused on polynuclear SCO materials, whose specific molecular configurations allow the presence of multi-step transitions and elastic frustration. In this contribution, we develop the first elastic modeling of thermal and dynamical properties of trinuclear SCO solids. For that, we study a finite SCO open chain constituted of successive elastically coupled trinuclear (A=B=C) blocks, in which each site (A, B, and C) may occupy two electronic configurations, namely, low-spin (LS) and high-spin (HS) states, accompanied with structural changes.
View Article and Find Full Text PDFRheumatol Int
January 2025
Department of Diagnostic and Interventional Radiology, University Hospital Wuerzburg, Oberduerrbacher Strasse 6, 97080, Wuerzburg, Germany.
Background: Diagnosis of Giant Cell Arteritis (GCA) and Polymyalgia rheumatica (PMR) may be challenging as many patients present with non-specific symptoms. Superficial cranial arteries are predilection sites of inflammatory affection. Ultrasound is typically the diagnostic tool of first choice supplementary to clinical and laboratory examination.
View Article and Find Full Text PDFSci Rep
December 2024
Mads Clausen Institute, NanoSYD, University of Southern Denmark, Alsion 2, 6400, Sønderborg, Denmark.
Highly porous, self-supported 3D interconnected network-based nanomaterials hold immense promise in revolutionizing the field of catalysis. These materials combine two critical features; a large accessible surface and an overall active surface that leads to substantial catalytic effects. In this study, we developed a novel class of 3D composite material composed of zinc oxide tetrapods (ZOT) and polyethylene glycol (PEG) polymer, specifically designed for photocatalysis.
View Article and Find Full Text PDFChemistry
December 2024
Departamento de Química Orgánica, Facultad de Química, Universidad Complutense, 28040-, Madrid, Spain.
The synthesis and characterization of novel compounds (5-8) as mimetics of [FeFe]-hydrogenase, combining two distinct systems capable of participating in hydrogen evolution reactions (HER): the [(μ-adt)Fe(CO)] fragment and M-salen complexes (salen=N,N'-bis(salicylidene)ethylenediamine) (M=Zn, Ni, Fe, Mn), is reported. These complexes were synthesized in high yields via a three-step procedure from N,N'-bis(4-R-salicylidene)ethanediamine) 4 [R=Fe(CO)(μ-SCH)NCOCHO]. Structural analysis through spectroscopic, spectrometric, and computational (DFT) methods confirmed distorted tetrahedral and square-planar geometries for Zn-salen and Ni-salen complexes (5 and 6) respectively, while complexes Fe-salen 7 and Mn-salen 8 exhibit square-based pyramidal structures typical of Fe(III) and Mn(III) high-spin salen-complexes.
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