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Transport of a comb-like polymer across a nanochannel subject to a pulling force. | LitMetric

Transport of a comb-like polymer across a nanochannel subject to a pulling force.

J Phys Condens Matter

Department of Mathematics, Physics, and Statistics, Addis Ababa Science and Technology University, Addis Ababa, Ethiopia.

Published: October 2024

AI Article Synopsis

Article Abstract

We investigate the dynamics of comb-like polymer translocation through a nanochannel using three-dimensional Langevin dynamics simulations based on a coarse-grained chain model. A comprehensive set of simulations are performed to examine the effects of system parameters such as the grafting densityof the side chains, the polymer chain length, the nanochannel dimensions, and the magnitude of the pulling force on the translocation dynamics. For a given polymer chain length, keeping the backbone length is constant while varying, we have found that the dependence of the mean translocation time⟨τ⟩onis non-monotonic, with a maximum translocation time for a specificat which the translocation is the slowest. The simulation results also show that⟨τ⟩is not significantly affected by the channel width above a certain radius, while the comb-like polymer translocation is hindered by a narrower channel due to increased interactions between the chain monomers and the channel. In addition,⟨τ⟩increases linearly with the nanochannel length. A linear scaling relationship between the mean translocation time⟨τ⟩and the chain lengthof polymer is obtained,⟨τ⟩∼N. Similarly, the dependence of⟨τ⟩on the backbone chain sizeNbbhas a quasi-linear dependence,⟨τ⟩∼Nbb. On the other hand, the translocation velocityfollows a power-law relationship with the polymer chain lengthasv∼N-1. The mean translocation time also shows an inverse linear relationship with the magnitude of the pulling force,⟨τ⟩∼F-1. The power-law relationships discovered in this study contribute to the fundamental understanding of the comb polymer translocation dynamics and to establishing a framework for further investigations in this field.

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Source
http://dx.doi.org/10.1088/1361-648X/ad7e70DOI Listing

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